Adjusting Hirshfeld charge of TEMPO catholytes for stable all-organic aqueous redox flow batteries

Adjusting Hirshfeld charge of TEMPO catholytes for stable all-organic aqueous redox flow batteries

Abstract 2,2,6,6-tetramethylpiperidine-1-oxyl (TEMPO) derivatives are typical catholytes in aqueous organic redox flow batteries (AORFBs), but reported lifetime of them is limited. We find that the increase of Hirshfeld charge decreases the Gibbs free energy change (ΔG) values of side reactions of T...

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Bibliographic Details
Main Authors: Gonggen Tang, Wenyi Wu, Yahua Liu, Kang Peng, Peipei Zuo, Zhengjin Yang, Tongwen Xu
Format: Article
Language:English
Published: Nature Portfolio 2025-01-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-024-55244-4
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