New Insight Into the Source and Sink of 227Ac in the Ocean

Abstract Actinium‐227 (227Ac) has been used as a powerful tracer of diapycnal mixing in the ocean, assuming that it is conservative and originates mainly from deep‐sea sediments. However, here we show an unexpectedly large source (continental margin) and sink (scavenging) of 227Ac in the ocean, base...

Full description

Saved in:
Bibliographic Details
Main Authors: Hojong Seo, Hanbyul Lee, Guebuem Kim
Format: Article
Language:English
Published: Wiley 2024-01-01
Series:Geophysical Research Letters
Subjects:
Online Access:https://doi.org/10.1029/2023GL105853
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1850205132262735872
author Hojong Seo
Hanbyul Lee
Guebuem Kim
author_facet Hojong Seo
Hanbyul Lee
Guebuem Kim
author_sort Hojong Seo
collection DOAJ
description Abstract Actinium‐227 (227Ac) has been used as a powerful tracer of diapycnal mixing in the ocean, assuming that it is conservative and originates mainly from deep‐sea sediments. However, here we show an unexpectedly large source (continental margin) and sink (scavenging) of 227Ac in the ocean, based on high‐resolution 227Ac distributions obtained for the first time by mooring Mn‐fibers in the East Sea (Japan Sea). Although we expected a decrease in radium‐228 (228Ra) to 227Ac ratios with depth owing to their different half‐lives, the ratios increased with depth in the upper layer, indicating efficient removal of 227Ac by particle scavenging. In addition, unusually high 227Ac activities (∼15 dpm m−3) were observed in the surface layer, likely due to the horizontal transport of 227Ac‐enriched shelf water. Thus, our results suggest refining our understanding of the geochemical cycle and application of 227Ac in the ocean.
format Article
id doaj-art-b036af60ae9147688dc17d6cb225b5df
institution OA Journals
issn 0094-8276
1944-8007
language English
publishDate 2024-01-01
publisher Wiley
record_format Article
series Geophysical Research Letters
spelling doaj-art-b036af60ae9147688dc17d6cb225b5df2025-08-20T02:11:09ZengWileyGeophysical Research Letters0094-82761944-80072024-01-01512n/an/a10.1029/2023GL105853New Insight Into the Source and Sink of 227Ac in the OceanHojong Seo0Hanbyul Lee1Guebuem Kim2School of Earth and Environmental Sciences Research Institute of Oceanography Seoul National University Seoul KoreaSchool of Earth and Environmental Sciences Research Institute of Oceanography Seoul National University Seoul KoreaSchool of Earth and Environmental Sciences Research Institute of Oceanography Seoul National University Seoul KoreaAbstract Actinium‐227 (227Ac) has been used as a powerful tracer of diapycnal mixing in the ocean, assuming that it is conservative and originates mainly from deep‐sea sediments. However, here we show an unexpectedly large source (continental margin) and sink (scavenging) of 227Ac in the ocean, based on high‐resolution 227Ac distributions obtained for the first time by mooring Mn‐fibers in the East Sea (Japan Sea). Although we expected a decrease in radium‐228 (228Ra) to 227Ac ratios with depth owing to their different half‐lives, the ratios increased with depth in the upper layer, indicating efficient removal of 227Ac by particle scavenging. In addition, unusually high 227Ac activities (∼15 dpm m−3) were observed in the surface layer, likely due to the horizontal transport of 227Ac‐enriched shelf water. Thus, our results suggest refining our understanding of the geochemical cycle and application of 227Ac in the ocean.https://doi.org/10.1029/2023GL105853actinium‐227continental shelf waterparticle scavengingEast Sea (Japan Sea)mooring Mn‐fibers
spellingShingle Hojong Seo
Hanbyul Lee
Guebuem Kim
New Insight Into the Source and Sink of 227Ac in the Ocean
Geophysical Research Letters
actinium‐227
continental shelf water
particle scavenging
East Sea (Japan Sea)
mooring Mn‐fibers
title New Insight Into the Source and Sink of 227Ac in the Ocean
title_full New Insight Into the Source and Sink of 227Ac in the Ocean
title_fullStr New Insight Into the Source and Sink of 227Ac in the Ocean
title_full_unstemmed New Insight Into the Source and Sink of 227Ac in the Ocean
title_short New Insight Into the Source and Sink of 227Ac in the Ocean
title_sort new insight into the source and sink of 227ac in the ocean
topic actinium‐227
continental shelf water
particle scavenging
East Sea (Japan Sea)
mooring Mn‐fibers
url https://doi.org/10.1029/2023GL105853
work_keys_str_mv AT hojongseo newinsightintothesourceandsinkof227acintheocean
AT hanbyullee newinsightintothesourceandsinkof227acintheocean
AT guebuemkim newinsightintothesourceandsinkof227acintheocean