Theoretical fundamentals of mechanochemical reactions in the solid phase

Chemical reactions in the solid phase are characterized by many specificities. The study of such reactions, with regard to the condensed state, eliminates the need to introduce many approximations that are common when considering reactions in the liquid phase or heterogeneous reactions, other laws,...

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Main Authors: Đorđević Nataša, Mihajlović Slavica, Vlahović Milica, Kašić Vladan, Matijašević Srđan, Grubišić Mirko
Format: Article
Language:English
Published: Faculty of Mining and Geology, Belgrade 2025-01-01
Series:Podzemni Radovi
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Online Access:https://scindeks-clanci.ceon.rs/data/pdf/0354-2904/2025/0354-29042501101Q.pdf
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author Đorđević Nataša
Mihajlović Slavica
Vlahović Milica
Kašić Vladan
Matijašević Srđan
Grubišić Mirko
author_facet Đorđević Nataša
Mihajlović Slavica
Vlahović Milica
Kašić Vladan
Matijašević Srđan
Grubišić Mirko
author_sort Đorđević Nataša
collection DOAJ
description Chemical reactions in the solid phase are characterized by many specificities. The study of such reactions, with regard to the condensed state, eliminates the need to introduce many approximations that are common when considering reactions in the liquid phase or heterogeneous reactions, other laws, specific and inherent only to the solid state of matter. These make the scientific field of solid-state chemistry far more complex, due to the very strong need for a comprehensive multidisciplinary approach. The basic theoretical principles from the fields of physics, chemistry, physical chemistry and chemical technology are equally important. The article gives an example of mechanochemical synthesis of the neutralization type, and barium oxide as the base component and titanium oxide as the sisal component of the mixture are activated. In order to determine the changes that occur due to the mechanical activation of the starting materials, barium oxide and titanium oxide were ground in a stoichiometric ratio for 440 minutes. The analysis determined that a mechanochemical synthesis had taken place and that barium titanate with a degree of synthesis of 0.99 had been obtained. This was confirmed using X-ray structural analysis, which monitored the state of the activated material as a function of the time of activation.
format Article
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institution Kabale University
issn 0354-2904
2560-3337
language English
publishDate 2025-01-01
publisher Faculty of Mining and Geology, Belgrade
record_format Article
series Podzemni Radovi
spelling doaj-art-b025714df792457f8a86e04d29b6e7932025-08-20T03:56:38ZengFaculty of Mining and Geology, BelgradePodzemni Radovi0354-29042560-33372025-01-0120254610111610.5937/podrad2501101Q0354-29042501101QTheoretical fundamentals of mechanochemical reactions in the solid phaseĐorđević Nataša0https://orcid.org/0000-0002-2353-6751Mihajlović Slavica1https://orcid.org/0000-0003-0904-3878Vlahović Milica2https://orcid.org/0000-0002-7893-9101Kašić Vladan3https://orcid.org/0000-0002-4430-567XMatijašević Srđan4https://orcid.org/0000-0002-3897-8085Grubišić Mirko5https://orcid.org/0009-0007-9705-2796Institute for Technology of Nuclear and Other Row Materials, Belgrade, SerbiaInstitute for Technology of Nuclear and Other Row Materials, Belgrade, SerbiaUniversity of Belgrade, Institute of Chemistry, Technology and Metallurgy, National Institute of the Republic of Serbia, SerbiaInstitute for Technology of Nuclear and Other Row Materials, Belgrade, SerbiaInstitute for Technology of Nuclear and Other Row Materials, Belgrade, SerbiaInstitute for Technology of Nuclear and Other Row Materials, Belgrade, SerbiaChemical reactions in the solid phase are characterized by many specificities. The study of such reactions, with regard to the condensed state, eliminates the need to introduce many approximations that are common when considering reactions in the liquid phase or heterogeneous reactions, other laws, specific and inherent only to the solid state of matter. These make the scientific field of solid-state chemistry far more complex, due to the very strong need for a comprehensive multidisciplinary approach. The basic theoretical principles from the fields of physics, chemistry, physical chemistry and chemical technology are equally important. The article gives an example of mechanochemical synthesis of the neutralization type, and barium oxide as the base component and titanium oxide as the sisal component of the mixture are activated. In order to determine the changes that occur due to the mechanical activation of the starting materials, barium oxide and titanium oxide were ground in a stoichiometric ratio for 440 minutes. The analysis determined that a mechanochemical synthesis had taken place and that barium titanate with a degree of synthesis of 0.99 had been obtained. This was confirmed using X-ray structural analysis, which monitored the state of the activated material as a function of the time of activation.https://scindeks-clanci.ceon.rs/data/pdf/0354-2904/2025/0354-29042501101Q.pdfsolid statemechanochemical synthesisbarium titanate
spellingShingle Đorđević Nataša
Mihajlović Slavica
Vlahović Milica
Kašić Vladan
Matijašević Srđan
Grubišić Mirko
Theoretical fundamentals of mechanochemical reactions in the solid phase
Podzemni Radovi
solid state
mechanochemical synthesis
barium titanate
title Theoretical fundamentals of mechanochemical reactions in the solid phase
title_full Theoretical fundamentals of mechanochemical reactions in the solid phase
title_fullStr Theoretical fundamentals of mechanochemical reactions in the solid phase
title_full_unstemmed Theoretical fundamentals of mechanochemical reactions in the solid phase
title_short Theoretical fundamentals of mechanochemical reactions in the solid phase
title_sort theoretical fundamentals of mechanochemical reactions in the solid phase
topic solid state
mechanochemical synthesis
barium titanate
url https://scindeks-clanci.ceon.rs/data/pdf/0354-2904/2025/0354-29042501101Q.pdf
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AT kasicvladan theoreticalfundamentalsofmechanochemicalreactionsinthesolidphase
AT matijasevicsrđan theoreticalfundamentalsofmechanochemicalreactionsinthesolidphase
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