Recent Advances in Zinc Complexes for Stereoselective Ring-Opening Polymerization and Copolymerization

Recent advances in zinc complexes for stereoselective ring-opening polymerization (ROP) and copolymerization (ROCOP) highlight their pivotal role in synthesizing biodegradable aliphatic polyesters and polycarbonates. These materials address the urgent demand for sustainable alternatives to petroleum...

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Main Authors: Xia Li, Yang Li, Gangqiang Zhang, Yat-Ming So, Yu Pan
Format: Article
Language:English
Published: MDPI AG 2025-06-01
Series:Inorganics
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Online Access:https://www.mdpi.com/2304-6740/13/6/185
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author Xia Li
Yang Li
Gangqiang Zhang
Yat-Ming So
Yu Pan
author_facet Xia Li
Yang Li
Gangqiang Zhang
Yat-Ming So
Yu Pan
author_sort Xia Li
collection DOAJ
description Recent advances in zinc complexes for stereoselective ring-opening polymerization (ROP) and copolymerization (ROCOP) highlight their pivotal role in synthesizing biodegradable aliphatic polyesters and polycarbonates. These materials address the urgent demand for sustainable alternatives to petroleum-based plastics, with stereochemical control directly impacting polymer crystallinity, thermal stability, and degradability. Zinc catalysts, leveraging low toxicity and versatile coordination chemistry, enable precise stereoregulation, whose performance is modulated by ligand steric/electronic effects, coordination geometry, and reaction conditions. This review summarizes the recent developments in zinc complexes for stereoselective ROP and ROCOP, focusing on ligand design strategies to enhance catalytic performance.
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id doaj-art-ae21f80aeee94a5e85747403ec4517c3
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publisher MDPI AG
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series Inorganics
spelling doaj-art-ae21f80aeee94a5e85747403ec4517c32025-08-20T02:21:02ZengMDPI AGInorganics2304-67402025-06-0113618510.3390/inorganics13060185Recent Advances in Zinc Complexes for Stereoselective Ring-Opening Polymerization and CopolymerizationXia Li0Yang Li1Gangqiang Zhang2Yat-Ming So3Yu Pan4Institute of Functional Textiles and Advanced Materials, College of Textiles and Clothing, State Key Laboratory of Bio-Fibers and Eco-Textiles, Qingdao University, Qingdao 266071, ChinaSchool of Chemical Engineering, Ocean and Life Sciences, Dalian University of Technology, Panjin 124221, ChinaInstitute of Functional Textiles and Advanced Materials, College of Textiles and Clothing, State Key Laboratory of Bio-Fibers and Eco-Textiles, Qingdao University, Qingdao 266071, ChinaDepartment of Chemistry, The Hong Kong University of Science and Technology, Hong Kong 999077, ChinaInstitute of Functional Textiles and Advanced Materials, College of Textiles and Clothing, State Key Laboratory of Bio-Fibers and Eco-Textiles, Qingdao University, Qingdao 266071, ChinaRecent advances in zinc complexes for stereoselective ring-opening polymerization (ROP) and copolymerization (ROCOP) highlight their pivotal role in synthesizing biodegradable aliphatic polyesters and polycarbonates. These materials address the urgent demand for sustainable alternatives to petroleum-based plastics, with stereochemical control directly impacting polymer crystallinity, thermal stability, and degradability. Zinc catalysts, leveraging low toxicity and versatile coordination chemistry, enable precise stereoregulation, whose performance is modulated by ligand steric/electronic effects, coordination geometry, and reaction conditions. This review summarizes the recent developments in zinc complexes for stereoselective ROP and ROCOP, focusing on ligand design strategies to enhance catalytic performance.https://www.mdpi.com/2304-6740/13/6/185zinc complexesring-opening polymerizationstereoselectivecopolymerizationligand designbiodegradable polymers
spellingShingle Xia Li
Yang Li
Gangqiang Zhang
Yat-Ming So
Yu Pan
Recent Advances in Zinc Complexes for Stereoselective Ring-Opening Polymerization and Copolymerization
Inorganics
zinc complexes
ring-opening polymerization
stereoselective
copolymerization
ligand design
biodegradable polymers
title Recent Advances in Zinc Complexes for Stereoselective Ring-Opening Polymerization and Copolymerization
title_full Recent Advances in Zinc Complexes for Stereoselective Ring-Opening Polymerization and Copolymerization
title_fullStr Recent Advances in Zinc Complexes for Stereoselective Ring-Opening Polymerization and Copolymerization
title_full_unstemmed Recent Advances in Zinc Complexes for Stereoselective Ring-Opening Polymerization and Copolymerization
title_short Recent Advances in Zinc Complexes for Stereoselective Ring-Opening Polymerization and Copolymerization
title_sort recent advances in zinc complexes for stereoselective ring opening polymerization and copolymerization
topic zinc complexes
ring-opening polymerization
stereoselective
copolymerization
ligand design
biodegradable polymers
url https://www.mdpi.com/2304-6740/13/6/185
work_keys_str_mv AT xiali recentadvancesinzinccomplexesforstereoselectiveringopeningpolymerizationandcopolymerization
AT yangli recentadvancesinzinccomplexesforstereoselectiveringopeningpolymerizationandcopolymerization
AT gangqiangzhang recentadvancesinzinccomplexesforstereoselectiveringopeningpolymerizationandcopolymerization
AT yatmingso recentadvancesinzinccomplexesforstereoselectiveringopeningpolymerizationandcopolymerization
AT yupan recentadvancesinzinccomplexesforstereoselectiveringopeningpolymerizationandcopolymerization