Metal-organic framework glass stabilizes high-voltage cathodes for efficient lithium-metal batteries

Abstract The rapid evolution of portable electronics and electric vehicles necessitates batteries with high energy density, robust cycling stability, and fast charging capabilities. High-voltage cathodes, like LiNi0.8Co0.1Mn0.1O2 (NCM-811), promise enhanced energy density but are hampered by poor st...

Full description

Saved in:
Bibliographic Details
Main Authors: Lishun Bai, Yan Xu, Yue Liu, Danni Zhang, Shibin Zhang, Wujie Yang, Zhi Chang, Haoshen Zhou
Format: Article
Language:English
Published: Nature Portfolio 2025-04-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-025-58639-z
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1850183880275918848
author Lishun Bai
Yan Xu
Yue Liu
Danni Zhang
Shibin Zhang
Wujie Yang
Zhi Chang
Haoshen Zhou
author_facet Lishun Bai
Yan Xu
Yue Liu
Danni Zhang
Shibin Zhang
Wujie Yang
Zhi Chang
Haoshen Zhou
author_sort Lishun Bai
collection DOAJ
description Abstract The rapid evolution of portable electronics and electric vehicles necessitates batteries with high energy density, robust cycling stability, and fast charging capabilities. High-voltage cathodes, like LiNi0.8Co0.1Mn0.1O2 (NCM-811), promise enhanced energy density but are hampered by poor stability and sluggish lithium-ion diffusion in conventional electrolytes. We introduce a metal-organic framework (MOF) liquid-infusion technique to fully integrate MOF liquid into the grain boundaries of NCM-811, creating a thoroughly coated cathode with a thin, rigid MOF Glass layer. The surface electrically non-conductive MOF Glass layer with 2.9 Å pore windows facilitating Li-ion pre-desolvation and enabling highly aggregative electrolyte formation inside the Glass channels, suppressing solvated Li-ion co-insertion and solvent decomposition. While the inner Glass layer composes of Li-ion conducting components and enhancing fast Li-ion diffusion. This functional structure effectively shields the cathode from particle cracking, CEI rupture, oxygen loss, and transition metal migration. As a result, Li | |Glass@NCM-811 cells demonstrate good rate capability and cycling stability even under high-charge rates and elevated voltages. Furthermore, we also achieve a 385 Wh kg-1 pouch-cell (19.579 g, for pouch-cell), showcasing the practical potential of this method. This straightforward and versatile strategy can be applied to other high-voltage cathodes like Li-rich manganese oxides and LiCoO2.
format Article
id doaj-art-ad51ceff912e411795da10720de6b341
institution OA Journals
issn 2041-1723
language English
publishDate 2025-04-01
publisher Nature Portfolio
record_format Article
series Nature Communications
spelling doaj-art-ad51ceff912e411795da10720de6b3412025-08-20T02:17:13ZengNature PortfolioNature Communications2041-17232025-04-0116111310.1038/s41467-025-58639-zMetal-organic framework glass stabilizes high-voltage cathodes for efficient lithium-metal batteriesLishun Bai0Yan Xu1Yue Liu2Danni Zhang3Shibin Zhang4Wujie Yang5Zhi Chang6Haoshen Zhou7School of Materials Science and Engineering, Key Laboratory of Electronic Packaging and Advanced Functional Materials of Hunan Province, Central South UniversitySchool of Materials Science and Engineering, Key Laboratory of Electronic Packaging and Advanced Functional Materials of Hunan Province, Central South UniversitySchool of Materials Science and Engineering, Key Laboratory of Electronic Packaging and Advanced Functional Materials of Hunan Province, Central South UniversitySchool of Materials Science and Engineering, Key Laboratory of Electronic Packaging and Advanced Functional Materials of Hunan Province, Central South UniversitySchool of Materials Science and Engineering, Key Laboratory of Electronic Packaging and Advanced Functional Materials of Hunan Province, Central South UniversityCenter of Energy Storage Materials & Technology, College of Engineering and Applied Sciences, National Laboratory of Solid State Micro-structures, Nanjing UniversitySchool of Materials Science and Engineering, Key Laboratory of Electronic Packaging and Advanced Functional Materials of Hunan Province, Central South UniversityCenter of Energy Storage Materials & Technology, College of Engineering and Applied Sciences, National Laboratory of Solid State Micro-structures, Nanjing UniversityAbstract The rapid evolution of portable electronics and electric vehicles necessitates batteries with high energy density, robust cycling stability, and fast charging capabilities. High-voltage cathodes, like LiNi0.8Co0.1Mn0.1O2 (NCM-811), promise enhanced energy density but are hampered by poor stability and sluggish lithium-ion diffusion in conventional electrolytes. We introduce a metal-organic framework (MOF) liquid-infusion technique to fully integrate MOF liquid into the grain boundaries of NCM-811, creating a thoroughly coated cathode with a thin, rigid MOF Glass layer. The surface electrically non-conductive MOF Glass layer with 2.9 Å pore windows facilitating Li-ion pre-desolvation and enabling highly aggregative electrolyte formation inside the Glass channels, suppressing solvated Li-ion co-insertion and solvent decomposition. While the inner Glass layer composes of Li-ion conducting components and enhancing fast Li-ion diffusion. This functional structure effectively shields the cathode from particle cracking, CEI rupture, oxygen loss, and transition metal migration. As a result, Li | |Glass@NCM-811 cells demonstrate good rate capability and cycling stability even under high-charge rates and elevated voltages. Furthermore, we also achieve a 385 Wh kg-1 pouch-cell (19.579 g, for pouch-cell), showcasing the practical potential of this method. This straightforward and versatile strategy can be applied to other high-voltage cathodes like Li-rich manganese oxides and LiCoO2.https://doi.org/10.1038/s41467-025-58639-z
spellingShingle Lishun Bai
Yan Xu
Yue Liu
Danni Zhang
Shibin Zhang
Wujie Yang
Zhi Chang
Haoshen Zhou
Metal-organic framework glass stabilizes high-voltage cathodes for efficient lithium-metal batteries
Nature Communications
title Metal-organic framework glass stabilizes high-voltage cathodes for efficient lithium-metal batteries
title_full Metal-organic framework glass stabilizes high-voltage cathodes for efficient lithium-metal batteries
title_fullStr Metal-organic framework glass stabilizes high-voltage cathodes for efficient lithium-metal batteries
title_full_unstemmed Metal-organic framework glass stabilizes high-voltage cathodes for efficient lithium-metal batteries
title_short Metal-organic framework glass stabilizes high-voltage cathodes for efficient lithium-metal batteries
title_sort metal organic framework glass stabilizes high voltage cathodes for efficient lithium metal batteries
url https://doi.org/10.1038/s41467-025-58639-z
work_keys_str_mv AT lishunbai metalorganicframeworkglassstabilizeshighvoltagecathodesforefficientlithiummetalbatteries
AT yanxu metalorganicframeworkglassstabilizeshighvoltagecathodesforefficientlithiummetalbatteries
AT yueliu metalorganicframeworkglassstabilizeshighvoltagecathodesforefficientlithiummetalbatteries
AT dannizhang metalorganicframeworkglassstabilizeshighvoltagecathodesforefficientlithiummetalbatteries
AT shibinzhang metalorganicframeworkglassstabilizeshighvoltagecathodesforefficientlithiummetalbatteries
AT wujieyang metalorganicframeworkglassstabilizeshighvoltagecathodesforefficientlithiummetalbatteries
AT zhichang metalorganicframeworkglassstabilizeshighvoltagecathodesforefficientlithiummetalbatteries
AT haoshenzhou metalorganicframeworkglassstabilizeshighvoltagecathodesforefficientlithiummetalbatteries