Green-based anti-biofilm nanoformulations against bacterial contaminations in nosocomial environments

α-amylase enzyme molecules were conjugated to biocompatible and biodegradable ad-hoc synthetized polycaprolactone (PCL) nanoparticles, in order to fabricate an effective and innovative nanoplatform for the treatment of nosocomial Staphylococcus aureus contaminations. Indeed, PCL was chosen as the po...

Full description

Saved in:
Bibliographic Details
Main Authors: Giovanni Lo Bello, Elena Dellacasa, Giacomo Damonte, Debora Caviglia, Anna Maria Schito, Roberto Raiteri, Orietta Monticelli, Marina Sartini, Maria Luisa Cristina, Laura Pastorino
Format: Article
Language:English
Published: Elsevier 2025-02-01
Series:Heliyon
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2405844025013155
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1850078469323489280
author Giovanni Lo Bello
Elena Dellacasa
Giacomo Damonte
Debora Caviglia
Anna Maria Schito
Roberto Raiteri
Orietta Monticelli
Marina Sartini
Maria Luisa Cristina
Laura Pastorino
author_facet Giovanni Lo Bello
Elena Dellacasa
Giacomo Damonte
Debora Caviglia
Anna Maria Schito
Roberto Raiteri
Orietta Monticelli
Marina Sartini
Maria Luisa Cristina
Laura Pastorino
author_sort Giovanni Lo Bello
collection DOAJ
description α-amylase enzyme molecules were conjugated to biocompatible and biodegradable ad-hoc synthetized polycaprolactone (PCL) nanoparticles, in order to fabricate an effective and innovative nanoplatform for the treatment of nosocomial Staphylococcus aureus contaminations. Indeed, PCL was chosen as the polymer matrix due to its features and the easy scalability of its synthesis, which enables to obtain a linear or star-shaped architecture with high functionality as in the polymer used.The developed nanoformulation underwent extensive structural and functional characterization to evaluate nanoparticles size and morphology before and after enzyme immobilization. Its antibiofilm effectiveness was then validated against bacterial strains isolated from hospital surfaces, demonstrating its potential for practical anti-biofilm applications. The obtained results demonstrated that the system prepared from the enzyme-conjugated nanoparticles exhibited a significant enzymatic activity and an efficient ability to degrade the protective bacterial biofilm. The proposed nanoformulation can therefore be considered an effective and completely environmentally friendly material for surface disinfection in healthcare facilities, which can be safely used in different environment (e.g. sinks and pipes) or medical equipment surfaces (e.g. touch screens).
format Article
id doaj-art-accc7166840c47cd9775d8965630ca65
institution DOAJ
issn 2405-8440
language English
publishDate 2025-02-01
publisher Elsevier
record_format Article
series Heliyon
spelling doaj-art-accc7166840c47cd9775d8965630ca652025-08-20T02:45:33ZengElsevierHeliyon2405-84402025-02-01114e4293410.1016/j.heliyon.2025.e42934Green-based anti-biofilm nanoformulations against bacterial contaminations in nosocomial environmentsGiovanni Lo Bello0Elena Dellacasa1Giacomo Damonte2Debora Caviglia3Anna Maria Schito4Roberto Raiteri5Orietta Monticelli6Marina Sartini7Maria Luisa Cristina8Laura Pastorino9Department of Informatics, Bioengineering, Robotics, and System Engineering, University of Genova, Via Opera Pia 13, 16145, Genova, ItalyDepartment of Informatics, Bioengineering, Robotics, and System Engineering, University of Genova, Via Opera Pia 13, 16145, Genova, ItalyDepartment of Chemistry and Industrial Chemistry, University of Genova, Via Dodecaneso 31, 16146, Genova, ItalyDepartment of Integrated Surgical and Diagnostical Sciences, University of Genoa, Viale Benedetto XV 6, 16132, Genoa, ItalyDepartment of Integrated Surgical and Diagnostical Sciences, University of Genoa, Viale Benedetto XV 6, 16132, Genoa, ItalyDepartment of Informatics, Bioengineering, Robotics, and System Engineering, University of Genova, Via Opera Pia 13, 16145, Genova, ItalyDepartment of Chemistry and Industrial Chemistry, University of Genova, Via Dodecaneso 31, 16146, Genova, ItalyDepartment of Health Science, University of Genova, Via Pastore 1, 16132, Genova, Italy; E.O. Ospedali Galliera, Hygiene Unit, Via Mura delle Cappuccine 14, 16128, Genova, ItalyDepartment of Health Science, University of Genova, Via Pastore 1, 16132, Genova, Italy; E.O. Ospedali Galliera, Hygiene Unit, Via Mura delle Cappuccine 14, 16128, Genova, ItalyDepartment of Informatics, Bioengineering, Robotics, and System Engineering, University of Genova, Via Opera Pia 13, 16145, Genova, Italy; Corresponding author.α-amylase enzyme molecules were conjugated to biocompatible and biodegradable ad-hoc synthetized polycaprolactone (PCL) nanoparticles, in order to fabricate an effective and innovative nanoplatform for the treatment of nosocomial Staphylococcus aureus contaminations. Indeed, PCL was chosen as the polymer matrix due to its features and the easy scalability of its synthesis, which enables to obtain a linear or star-shaped architecture with high functionality as in the polymer used.The developed nanoformulation underwent extensive structural and functional characterization to evaluate nanoparticles size and morphology before and after enzyme immobilization. Its antibiofilm effectiveness was then validated against bacterial strains isolated from hospital surfaces, demonstrating its potential for practical anti-biofilm applications. The obtained results demonstrated that the system prepared from the enzyme-conjugated nanoparticles exhibited a significant enzymatic activity and an efficient ability to degrade the protective bacterial biofilm. The proposed nanoformulation can therefore be considered an effective and completely environmentally friendly material for surface disinfection in healthcare facilities, which can be safely used in different environment (e.g. sinks and pipes) or medical equipment surfaces (e.g. touch screens).http://www.sciencedirect.com/science/article/pii/S2405844025013155Nosocomial infectionsStaphylococcus aureusα-amylasePCL nanoparticlesAntibiofilm nanoplatform
spellingShingle Giovanni Lo Bello
Elena Dellacasa
Giacomo Damonte
Debora Caviglia
Anna Maria Schito
Roberto Raiteri
Orietta Monticelli
Marina Sartini
Maria Luisa Cristina
Laura Pastorino
Green-based anti-biofilm nanoformulations against bacterial contaminations in nosocomial environments
Heliyon
Nosocomial infections
Staphylococcus aureus
α-amylase
PCL nanoparticles
Antibiofilm nanoplatform
title Green-based anti-biofilm nanoformulations against bacterial contaminations in nosocomial environments
title_full Green-based anti-biofilm nanoformulations against bacterial contaminations in nosocomial environments
title_fullStr Green-based anti-biofilm nanoformulations against bacterial contaminations in nosocomial environments
title_full_unstemmed Green-based anti-biofilm nanoformulations against bacterial contaminations in nosocomial environments
title_short Green-based anti-biofilm nanoformulations against bacterial contaminations in nosocomial environments
title_sort green based anti biofilm nanoformulations against bacterial contaminations in nosocomial environments
topic Nosocomial infections
Staphylococcus aureus
α-amylase
PCL nanoparticles
Antibiofilm nanoplatform
url http://www.sciencedirect.com/science/article/pii/S2405844025013155
work_keys_str_mv AT giovannilobello greenbasedantibiofilmnanoformulationsagainstbacterialcontaminationsinnosocomialenvironments
AT elenadellacasa greenbasedantibiofilmnanoformulationsagainstbacterialcontaminationsinnosocomialenvironments
AT giacomodamonte greenbasedantibiofilmnanoformulationsagainstbacterialcontaminationsinnosocomialenvironments
AT deboracaviglia greenbasedantibiofilmnanoformulationsagainstbacterialcontaminationsinnosocomialenvironments
AT annamariaschito greenbasedantibiofilmnanoformulationsagainstbacterialcontaminationsinnosocomialenvironments
AT robertoraiteri greenbasedantibiofilmnanoformulationsagainstbacterialcontaminationsinnosocomialenvironments
AT oriettamonticelli greenbasedantibiofilmnanoformulationsagainstbacterialcontaminationsinnosocomialenvironments
AT marinasartini greenbasedantibiofilmnanoformulationsagainstbacterialcontaminationsinnosocomialenvironments
AT marialuisacristina greenbasedantibiofilmnanoformulationsagainstbacterialcontaminationsinnosocomialenvironments
AT laurapastorino greenbasedantibiofilmnanoformulationsagainstbacterialcontaminationsinnosocomialenvironments