Synthesis and Characterization of Acrylamide-Based Anionic Copolymer and Investigation of Solution Properties

The copolymer of acrylamide (AM) and 2-acrylamido-2-methyl-1-propane sulfonic acid (AMPS) was synthesized through radical solution polymerization by potassium persulfate as initiator. By changing the AMPS feed ratio from 10 to 70%, and keeping other reaction conditions constant, different copolymers...

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Main Authors: H. Jamshidi, A. Rabiee
Format: Article
Language:English
Published: Wiley 2014-01-01
Series:Advances in Materials Science and Engineering
Online Access:http://dx.doi.org/10.1155/2014/728675
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author H. Jamshidi
A. Rabiee
author_facet H. Jamshidi
A. Rabiee
author_sort H. Jamshidi
collection DOAJ
description The copolymer of acrylamide (AM) and 2-acrylamido-2-methyl-1-propane sulfonic acid (AMPS) was synthesized through radical solution polymerization by potassium persulfate as initiator. By changing the AMPS feed ratio from 10 to 70%, and keeping other reaction conditions constant, different copolymers were synthesized. The techniques of Fourier transform infrared (FTIR) and nuclear magnetic resonance (1H- 13C-NMR) spectroscopy were used for identification of functional groups and confirmation of copolymers’ structure. Intrinsic and apparent viscosity of samples were measured in aqueous sodium chloride solution under standard conditions. The anionic degree of copolymers was determined by back titration method and by 13C-NMR spectroscopy. Molecular weight of copolymers was determined by the Mark-Houwink relationship. The measured molecular weight of samples showed that we have acquired a high molecular weight product. The effect of different range of shear rates on solution viscosity was evaluated. The copolymer solutions showed non-Newtonian shear thinning behavior. The performance of copolymers with respect to shear resistance and molecular weight was evaluated from industry application standpoint.
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spelling doaj-art-ab5158a1e8734e29b8ee2625f3a23f692025-08-20T03:39:39ZengWileyAdvances in Materials Science and Engineering1687-84341687-84422014-01-01201410.1155/2014/728675728675Synthesis and Characterization of Acrylamide-Based Anionic Copolymer and Investigation of Solution PropertiesH. Jamshidi0A. Rabiee1Iran Polymer and Petrochemical Institute, P.O. Box 14965/115, Tehran, IranIran Polymer and Petrochemical Institute, P.O. Box 14965/115, Tehran, IranThe copolymer of acrylamide (AM) and 2-acrylamido-2-methyl-1-propane sulfonic acid (AMPS) was synthesized through radical solution polymerization by potassium persulfate as initiator. By changing the AMPS feed ratio from 10 to 70%, and keeping other reaction conditions constant, different copolymers were synthesized. The techniques of Fourier transform infrared (FTIR) and nuclear magnetic resonance (1H- 13C-NMR) spectroscopy were used for identification of functional groups and confirmation of copolymers’ structure. Intrinsic and apparent viscosity of samples were measured in aqueous sodium chloride solution under standard conditions. The anionic degree of copolymers was determined by back titration method and by 13C-NMR spectroscopy. Molecular weight of copolymers was determined by the Mark-Houwink relationship. The measured molecular weight of samples showed that we have acquired a high molecular weight product. The effect of different range of shear rates on solution viscosity was evaluated. The copolymer solutions showed non-Newtonian shear thinning behavior. The performance of copolymers with respect to shear resistance and molecular weight was evaluated from industry application standpoint.http://dx.doi.org/10.1155/2014/728675
spellingShingle H. Jamshidi
A. Rabiee
Synthesis and Characterization of Acrylamide-Based Anionic Copolymer and Investigation of Solution Properties
Advances in Materials Science and Engineering
title Synthesis and Characterization of Acrylamide-Based Anionic Copolymer and Investigation of Solution Properties
title_full Synthesis and Characterization of Acrylamide-Based Anionic Copolymer and Investigation of Solution Properties
title_fullStr Synthesis and Characterization of Acrylamide-Based Anionic Copolymer and Investigation of Solution Properties
title_full_unstemmed Synthesis and Characterization of Acrylamide-Based Anionic Copolymer and Investigation of Solution Properties
title_short Synthesis and Characterization of Acrylamide-Based Anionic Copolymer and Investigation of Solution Properties
title_sort synthesis and characterization of acrylamide based anionic copolymer and investigation of solution properties
url http://dx.doi.org/10.1155/2014/728675
work_keys_str_mv AT hjamshidi synthesisandcharacterizationofacrylamidebasedanioniccopolymerandinvestigationofsolutionproperties
AT arabiee synthesisandcharacterizationofacrylamidebasedanioniccopolymerandinvestigationofsolutionproperties