Dynamic Modeling of the Sulfur Cycle in Urban Sewage Pipelines Under High-Temperature and High-Salinity Conditions

This study addresses the microbial corrosion of cement-based materials in coastal urban sewer networks, systematically investigating the kinetic mechanisms of sulfur biogeochemical cycling under seawater infiltration conditions. Through dynamic monitoring of sulfide concentrations and environmental...

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Main Authors: Zhiwei Cao, Zhen Xu, Yufeng Chen, Bingxuan Zhao, Chenxu Wang, Zuozhou Yu, Jingya Zhou
Format: Article
Language:English
Published: MDPI AG 2025-06-01
Series:Microorganisms
Subjects:
Online Access:https://www.mdpi.com/2076-2607/13/7/1534
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author Zhiwei Cao
Zhen Xu
Yufeng Chen
Bingxuan Zhao
Chenxu Wang
Zuozhou Yu
Jingya Zhou
author_facet Zhiwei Cao
Zhen Xu
Yufeng Chen
Bingxuan Zhao
Chenxu Wang
Zuozhou Yu
Jingya Zhou
author_sort Zhiwei Cao
collection DOAJ
description This study addresses the microbial corrosion of cement-based materials in coastal urban sewer networks, systematically investigating the kinetic mechanisms of sulfur biogeochemical cycling under seawater infiltration conditions. Through dynamic monitoring of sulfide concentrations and environmental parameter variations in anaerobic pipelines, a multiphase coupled kinetic model integrating liquid-phase, gas-phase, and biofilm metabolic processes was developed. The results demonstrate that moderate salinity enhances the activity of sulfate-reducing bacteria (SRB) and accelerates sulfate reduction rates, whereas excessive sulfide accumulation inhibits SRB activity. At 35 °C, the mathematical model coefficient “a” for sulfate reduction in the reactor with 3 g/L salinity was significantly higher than those in reactors with 19 g/L and 35 g/L salinities, with no significant difference observed between the latter two. Overall, high sulfate concentrations do not act as limiting factors for sulfide oxidation under anaerobic conditions; instead, they enhance the reaction within specific concentration ranges. The refined kinetic model enables prediction of sulfur speciation in tropical coastal urban sewer pipelines, providing a scientific basis for corrosion risk assessment.
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publishDate 2025-06-01
publisher MDPI AG
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series Microorganisms
spelling doaj-art-aac4ecf09a5646b79bdaf6a69109053f2025-08-20T03:07:55ZengMDPI AGMicroorganisms2076-26072025-06-01137153410.3390/microorganisms13071534Dynamic Modeling of the Sulfur Cycle in Urban Sewage Pipelines Under High-Temperature and High-Salinity ConditionsZhiwei Cao0Zhen Xu1Yufeng Chen2Bingxuan Zhao3Chenxu Wang4Zuozhou Yu5Jingya Zhou6Department of Agricultural Resources and Environment, College of Agriculture, Yanbian University, Yanji 133002, ChinaCollege of Geography and Ocean Sciences, Yanbian University, Yanji 133002, ChinaKey Laboratory of Biology and Genetic Resources of Tropical Crops, Ministry of Agriculture, Institute of Tropical Bioscience and Biotechnology, Chinese Academy of Tropical Agricultural Sciences, Haikou 571101, ChinaDepartment of Biological, Geological, and Environmental Sciences, University of Bologna, Via Sant’Alberto 163, 48123 Ravenna, ItalyDepartment of Environmental Science, College of Geography and Ocean Sciences, Yanbian University, Yanji 133002, ChinaDepartment of Environmental Science, College of Geography and Ocean Sciences, Yanbian University, Yanji 133002, ChinaDepartment of Agricultural Resources and Environment, College of Agriculture, Yanbian University, Yanji 133002, ChinaThis study addresses the microbial corrosion of cement-based materials in coastal urban sewer networks, systematically investigating the kinetic mechanisms of sulfur biogeochemical cycling under seawater infiltration conditions. Through dynamic monitoring of sulfide concentrations and environmental parameter variations in anaerobic pipelines, a multiphase coupled kinetic model integrating liquid-phase, gas-phase, and biofilm metabolic processes was developed. The results demonstrate that moderate salinity enhances the activity of sulfate-reducing bacteria (SRB) and accelerates sulfate reduction rates, whereas excessive sulfide accumulation inhibits SRB activity. At 35 °C, the mathematical model coefficient “a” for sulfate reduction in the reactor with 3 g/L salinity was significantly higher than those in reactors with 19 g/L and 35 g/L salinities, with no significant difference observed between the latter two. Overall, high sulfate concentrations do not act as limiting factors for sulfide oxidation under anaerobic conditions; instead, they enhance the reaction within specific concentration ranges. The refined kinetic model enables prediction of sulfur speciation in tropical coastal urban sewer pipelines, providing a scientific basis for corrosion risk assessment.https://www.mdpi.com/2076-2607/13/7/1534dynamic modelsulfur cyclephased reaction processsewage pipelinescorrosion
spellingShingle Zhiwei Cao
Zhen Xu
Yufeng Chen
Bingxuan Zhao
Chenxu Wang
Zuozhou Yu
Jingya Zhou
Dynamic Modeling of the Sulfur Cycle in Urban Sewage Pipelines Under High-Temperature and High-Salinity Conditions
Microorganisms
dynamic model
sulfur cycle
phased reaction process
sewage pipelines
corrosion
title Dynamic Modeling of the Sulfur Cycle in Urban Sewage Pipelines Under High-Temperature and High-Salinity Conditions
title_full Dynamic Modeling of the Sulfur Cycle in Urban Sewage Pipelines Under High-Temperature and High-Salinity Conditions
title_fullStr Dynamic Modeling of the Sulfur Cycle in Urban Sewage Pipelines Under High-Temperature and High-Salinity Conditions
title_full_unstemmed Dynamic Modeling of the Sulfur Cycle in Urban Sewage Pipelines Under High-Temperature and High-Salinity Conditions
title_short Dynamic Modeling of the Sulfur Cycle in Urban Sewage Pipelines Under High-Temperature and High-Salinity Conditions
title_sort dynamic modeling of the sulfur cycle in urban sewage pipelines under high temperature and high salinity conditions
topic dynamic model
sulfur cycle
phased reaction process
sewage pipelines
corrosion
url https://www.mdpi.com/2076-2607/13/7/1534
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AT yufengchen dynamicmodelingofthesulfurcycleinurbansewagepipelinesunderhightemperatureandhighsalinityconditions
AT bingxuanzhao dynamicmodelingofthesulfurcycleinurbansewagepipelinesunderhightemperatureandhighsalinityconditions
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