CO2 Capture by Using a Membrane-absorption Hybrid Process in the Nature Gas Combined Cycle Power Plants

Abstract This study’s main objective was to optimize the design parameters of the hybrid membrane-absorption CO2-capture process in natural gas steam cycle (NGCC) power plants. To calculate the CO2 concentration in the permeating gas and the required area for the separating membrane, a mass transfer...

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Main Authors: Wenfeng Dong, Mengxiang Fang, Tao Wang, Fei Liu, Ningtong Yi
Format: Article
Language:English
Published: Springer 2020-09-01
Series:Aerosol and Air Quality Research
Subjects:
Online Access:https://doi.org/10.4209/aaqr.2020.07.0374
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author Wenfeng Dong
Mengxiang Fang
Tao Wang
Fei Liu
Ningtong Yi
author_facet Wenfeng Dong
Mengxiang Fang
Tao Wang
Fei Liu
Ningtong Yi
author_sort Wenfeng Dong
collection DOAJ
description Abstract This study’s main objective was to optimize the design parameters of the hybrid membrane-absorption CO2-capture process in natural gas steam cycle (NGCC) power plants. To calculate the CO2 concentration in the permeating gas and the required area for the separating membrane, a mass transfer model of a membrane for separating CO2, N2 and H2O was developed in Aspen Plus. The effects of the CO2 recovery rate of the membrane, the ratio of the feed gas pressure to the permeating-side gas pressure and the flow rate of the flue gas on the required area for the membrane, the power consumption of the compressor and the heat duty for the solvent regeneration were then analyzed. The optimal feed-gas-to-permeating-side-gas pressure ratio and the flue gas flow rate were found to be 10:1 and 50%, respectively. Furthermore, compared to traditional chemical absorption, the solvent regeneration’s heat duty decreased by more than 20.7% when the gas flow rate and the CO2 recovery rate were 100% and 20%, respectively.
format Article
id doaj-art-aa3705499e5840e695d4f7c4aab9eb9c
institution Kabale University
issn 1680-8584
2071-1409
language English
publishDate 2020-09-01
publisher Springer
record_format Article
series Aerosol and Air Quality Research
spelling doaj-art-aa3705499e5840e695d4f7c4aab9eb9c2025-02-09T12:19:56ZengSpringerAerosol and Air Quality Research1680-85842071-14092020-09-0121311210.4209/aaqr.2020.07.0374CO2 Capture by Using a Membrane-absorption Hybrid Process in the Nature Gas Combined Cycle Power PlantsWenfeng Dong0Mengxiang Fang1Tao Wang2Fei Liu3Ningtong Yi4State Key Laboratory of Clean Energy Utilization, Zhejiang UniversityState Key Laboratory of Clean Energy Utilization, Zhejiang UniversityState Key Laboratory of Clean Energy Utilization, Zhejiang UniversityState Key Laboratory of Clean Energy Utilization, Zhejiang UniversityState Key Laboratory of Clean Energy Utilization, Zhejiang UniversityAbstract This study’s main objective was to optimize the design parameters of the hybrid membrane-absorption CO2-capture process in natural gas steam cycle (NGCC) power plants. To calculate the CO2 concentration in the permeating gas and the required area for the separating membrane, a mass transfer model of a membrane for separating CO2, N2 and H2O was developed in Aspen Plus. The effects of the CO2 recovery rate of the membrane, the ratio of the feed gas pressure to the permeating-side gas pressure and the flow rate of the flue gas on the required area for the membrane, the power consumption of the compressor and the heat duty for the solvent regeneration were then analyzed. The optimal feed-gas-to-permeating-side-gas pressure ratio and the flue gas flow rate were found to be 10:1 and 50%, respectively. Furthermore, compared to traditional chemical absorption, the solvent regeneration’s heat duty decreased by more than 20.7% when the gas flow rate and the CO2 recovery rate were 100% and 20%, respectively.https://doi.org/10.4209/aaqr.2020.07.0374Membrane-absorption processMass transfer modelNatural gas steam combined cycle power plantsCO2 captureMonoethanolamine
spellingShingle Wenfeng Dong
Mengxiang Fang
Tao Wang
Fei Liu
Ningtong Yi
CO2 Capture by Using a Membrane-absorption Hybrid Process in the Nature Gas Combined Cycle Power Plants
Aerosol and Air Quality Research
Membrane-absorption process
Mass transfer model
Natural gas steam combined cycle power plants
CO2 capture
Monoethanolamine
title CO2 Capture by Using a Membrane-absorption Hybrid Process in the Nature Gas Combined Cycle Power Plants
title_full CO2 Capture by Using a Membrane-absorption Hybrid Process in the Nature Gas Combined Cycle Power Plants
title_fullStr CO2 Capture by Using a Membrane-absorption Hybrid Process in the Nature Gas Combined Cycle Power Plants
title_full_unstemmed CO2 Capture by Using a Membrane-absorption Hybrid Process in the Nature Gas Combined Cycle Power Plants
title_short CO2 Capture by Using a Membrane-absorption Hybrid Process in the Nature Gas Combined Cycle Power Plants
title_sort co2 capture by using a membrane absorption hybrid process in the nature gas combined cycle power plants
topic Membrane-absorption process
Mass transfer model
Natural gas steam combined cycle power plants
CO2 capture
Monoethanolamine
url https://doi.org/10.4209/aaqr.2020.07.0374
work_keys_str_mv AT wenfengdong co2capturebyusingamembraneabsorptionhybridprocessinthenaturegascombinedcyclepowerplants
AT mengxiangfang co2capturebyusingamembraneabsorptionhybridprocessinthenaturegascombinedcyclepowerplants
AT taowang co2capturebyusingamembraneabsorptionhybridprocessinthenaturegascombinedcyclepowerplants
AT feiliu co2capturebyusingamembraneabsorptionhybridprocessinthenaturegascombinedcyclepowerplants
AT ningtongyi co2capturebyusingamembraneabsorptionhybridprocessinthenaturegascombinedcyclepowerplants