Long-term migration of 137Cs in Swedish grassland soil profiles following the Chornobyl accident

This study presents long-term findings (1987–2008) on the vertical migration of 137Cs from the Chornobyl accident in undisturbed grassland soils in central and northern Sweden. We examined five mineral and three organic soils, with 137Cs deposition in 1986 ranging from 16 to 190 kBq m2. 137Cs activi...

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Main Authors: Klas Rosén, Ingrid Öborn, Mykhailo Vinichuk
Format: Article
Language:English
Published: Elsevier 2025-09-01
Series:Geoderma
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Online Access:http://www.sciencedirect.com/science/article/pii/S0016706125003209
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author Klas Rosén
Ingrid Öborn
Mykhailo Vinichuk
author_facet Klas Rosén
Ingrid Öborn
Mykhailo Vinichuk
author_sort Klas Rosén
collection DOAJ
description This study presents long-term findings (1987–2008) on the vertical migration of 137Cs from the Chornobyl accident in undisturbed grassland soils in central and northern Sweden. We examined five mineral and three organic soils, with 137Cs deposition in 1986 ranging from 16 to 190 kBq m2. 137Cs activities were measured in 1 cm slices at depths of 0–10 cm and in 2.5 cm slices at 10–50 cm. Distribution (kBq m2) was calculated for different soil horizons, and migration rates were determined based on observed depths. During the initial period after the fallout (1987–1992), 137Cs was primarily located in the upper 0–2 cm layers of both mineral and organic soils, comprising 77 % to 94 % of the radionuclide. During the intermediate period (1994–2003), the average migration depth was 4.0 cm in mineral soils and 5.5 cm in the organic soils while during the later period (2004–2008) it was 4.4 and 7.0 cm, respectively. After about 20 years, approximately 80 % of the 137Cs activity was found in the upper 0–6 cm at five out of eight sites, and 75–78 % within 0–9 cm at two sites regardless of soil type. The average radionuclide migration rate of 137Cs in the period 1987 to 2008 across various sites was 0.31 cm yr−1. In mineral soils, the average migration rate was 0.28 cm yr−1 (range 0.13–0.47) and in organic soils it was 0.3 cm yr−1 (range 0.17–0.76). There was no significant relationship between soil clay content in mineral soils and the average migration depth of the radionuclide during the study period (P = 0.423).
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spelling doaj-art-a7c60fa17e504b709ad824135c17ad2b2025-08-20T04:03:22ZengElsevierGeoderma1872-62592025-09-0146111747910.1016/j.geoderma.2025.117479Long-term migration of 137Cs in Swedish grassland soil profiles following the Chornobyl accidentKlas Rosén0Ingrid Öborn1Mykhailo Vinichuk2Department of Soil and Environment, Swedish University of Agricultural Sciences, Box 7014, Uppsala SE-750 07, SwedenDepartment of Crop Production Ecology, Swedish University of Agricultural Sciences, Box 7043, Uppsala SE-750 07, SwedenDepartment of Soil and Environment, Swedish University of Agricultural Sciences, Box 7014, Uppsala SE-750 07, Sweden; Department of Ecology and Environmental Protection Technologies, Zhytomyr Polytechnic State University, 103 Chudnivska str., Zhytomyr 10005, Ukraine; Corresponding author at: Department of Soil and Environment, Swedish University of Agricultural Sciences, Box 7014, Uppsala SE-750 07, Sweden.This study presents long-term findings (1987–2008) on the vertical migration of 137Cs from the Chornobyl accident in undisturbed grassland soils in central and northern Sweden. We examined five mineral and three organic soils, with 137Cs deposition in 1986 ranging from 16 to 190 kBq m2. 137Cs activities were measured in 1 cm slices at depths of 0–10 cm and in 2.5 cm slices at 10–50 cm. Distribution (kBq m2) was calculated for different soil horizons, and migration rates were determined based on observed depths. During the initial period after the fallout (1987–1992), 137Cs was primarily located in the upper 0–2 cm layers of both mineral and organic soils, comprising 77 % to 94 % of the radionuclide. During the intermediate period (1994–2003), the average migration depth was 4.0 cm in mineral soils and 5.5 cm in the organic soils while during the later period (2004–2008) it was 4.4 and 7.0 cm, respectively. After about 20 years, approximately 80 % of the 137Cs activity was found in the upper 0–6 cm at five out of eight sites, and 75–78 % within 0–9 cm at two sites regardless of soil type. The average radionuclide migration rate of 137Cs in the period 1987 to 2008 across various sites was 0.31 cm yr−1. In mineral soils, the average migration rate was 0.28 cm yr−1 (range 0.13–0.47) and in organic soils it was 0.3 cm yr−1 (range 0.17–0.76). There was no significant relationship between soil clay content in mineral soils and the average migration depth of the radionuclide during the study period (P = 0.423).http://www.sciencedirect.com/science/article/pii/S0016706125003209Chornobyl falloutField studyGrasslandMigration rateRadiocaesiumSoil type
spellingShingle Klas Rosén
Ingrid Öborn
Mykhailo Vinichuk
Long-term migration of 137Cs in Swedish grassland soil profiles following the Chornobyl accident
Geoderma
Chornobyl fallout
Field study
Grassland
Migration rate
Radiocaesium
Soil type
title Long-term migration of 137Cs in Swedish grassland soil profiles following the Chornobyl accident
title_full Long-term migration of 137Cs in Swedish grassland soil profiles following the Chornobyl accident
title_fullStr Long-term migration of 137Cs in Swedish grassland soil profiles following the Chornobyl accident
title_full_unstemmed Long-term migration of 137Cs in Swedish grassland soil profiles following the Chornobyl accident
title_short Long-term migration of 137Cs in Swedish grassland soil profiles following the Chornobyl accident
title_sort long term migration of 137cs in swedish grassland soil profiles following the chornobyl accident
topic Chornobyl fallout
Field study
Grassland
Migration rate
Radiocaesium
Soil type
url http://www.sciencedirect.com/science/article/pii/S0016706125003209
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