Synthesis of new surface-active ammonium-type complexes based on palmitic acid for removing thin petroleum films from water surface

Complexes based on palmitic acid and nitrogen-containing compounds (monoethanolamine and triethylenetetramine) were synthesized. The synthesized complexes were taken to react with different moles of propylene oxide (1, 2 and 3) to form propoxylated compounds (surfactants). Some of physico-chemical i...

Full description

Saved in:
Bibliographic Details
Main Authors: Ziyafaddin H. Asadov, Ahmed H. Tantawy, Ilhama A. Zarbaliyeva, Ravan A. Rahimov
Format: Article
Language:English
Published: Egyptian Petroleum Research Institute 2013-12-01
Series:Egyptian Journal of Petroleum
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S1110062113000536
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1849397792069386240
author Ziyafaddin H. Asadov
Ahmed H. Tantawy
Ilhama A. Zarbaliyeva
Ravan A. Rahimov
author_facet Ziyafaddin H. Asadov
Ahmed H. Tantawy
Ilhama A. Zarbaliyeva
Ravan A. Rahimov
author_sort Ziyafaddin H. Asadov
collection DOAJ
description Complexes based on palmitic acid and nitrogen-containing compounds (monoethanolamine and triethylenetetramine) were synthesized. The synthesized complexes were taken to react with different moles of propylene oxide (1, 2 and 3) to form propoxylated compounds (surfactants). Some of physico-chemical indices of the prepared compounds such as solubility, acid and amine numbers as well as electrical conductivity have been determined. Surface-active properties (interfacial tension) of the obtained complexes were investigated by the stalagmometric method. Surface properties studied included critical micelle concentration (CMC), maximum surface excess (Γmax), and minimum surface area (Amin). Free energies of micellization (ΔGmic°) and adsorption (ΔGads°) were calculated. Petroleum-collecting and dispersing properties of the synthesized and propoxylated complexes in diluted (5 wt.% aq. solution) and undiluted form in waters of varying salinity have been studied. FTIR spectra, C13 and H1NMR spectra confirm the compound structure.
format Article
id doaj-art-a70aaa3a69fe4279b6ea14bbf575ff8a
institution Kabale University
issn 1110-0621
language English
publishDate 2013-12-01
publisher Egyptian Petroleum Research Institute
record_format Article
series Egyptian Journal of Petroleum
spelling doaj-art-a70aaa3a69fe4279b6ea14bbf575ff8a2025-08-20T03:38:50ZengEgyptian Petroleum Research InstituteEgyptian Journal of Petroleum1110-06212013-12-0122226126710.1016/j.ejpe.2013.06.005Synthesis of new surface-active ammonium-type complexes based on palmitic acid for removing thin petroleum films from water surfaceZiyafaddin H. Asadov0Ahmed H. Tantawy1Ilhama A. Zarbaliyeva2Ravan A. Rahimov3Institute of Petrochemical Processes of Azerbaijan National Academy of Sciences, Hojaly Ave. 30, Az 1025, Baku, AzerbaijanInstitute of Petrochemical Processes of Azerbaijan National Academy of Sciences, Hojaly Ave. 30, Az 1025, Baku, AzerbaijanInstitute of Petrochemical Processes of Azerbaijan National Academy of Sciences, Hojaly Ave. 30, Az 1025, Baku, AzerbaijanInstitute of Petrochemical Processes of Azerbaijan National Academy of Sciences, Hojaly Ave. 30, Az 1025, Baku, AzerbaijanComplexes based on palmitic acid and nitrogen-containing compounds (monoethanolamine and triethylenetetramine) were synthesized. The synthesized complexes were taken to react with different moles of propylene oxide (1, 2 and 3) to form propoxylated compounds (surfactants). Some of physico-chemical indices of the prepared compounds such as solubility, acid and amine numbers as well as electrical conductivity have been determined. Surface-active properties (interfacial tension) of the obtained complexes were investigated by the stalagmometric method. Surface properties studied included critical micelle concentration (CMC), maximum surface excess (Γmax), and minimum surface area (Amin). Free energies of micellization (ΔGmic°) and adsorption (ΔGads°) were calculated. Petroleum-collecting and dispersing properties of the synthesized and propoxylated complexes in diluted (5 wt.% aq. solution) and undiluted form in waters of varying salinity have been studied. FTIR spectra, C13 and H1NMR spectra confirm the compound structure.http://www.sciencedirect.com/science/article/pii/S1110062113000536Palmitic acidNitrogen-containing compoundsComplexDispersing agentCollecting agentPropylene oxide
spellingShingle Ziyafaddin H. Asadov
Ahmed H. Tantawy
Ilhama A. Zarbaliyeva
Ravan A. Rahimov
Synthesis of new surface-active ammonium-type complexes based on palmitic acid for removing thin petroleum films from water surface
Egyptian Journal of Petroleum
Palmitic acid
Nitrogen-containing compounds
Complex
Dispersing agent
Collecting agent
Propylene oxide
title Synthesis of new surface-active ammonium-type complexes based on palmitic acid for removing thin petroleum films from water surface
title_full Synthesis of new surface-active ammonium-type complexes based on palmitic acid for removing thin petroleum films from water surface
title_fullStr Synthesis of new surface-active ammonium-type complexes based on palmitic acid for removing thin petroleum films from water surface
title_full_unstemmed Synthesis of new surface-active ammonium-type complexes based on palmitic acid for removing thin petroleum films from water surface
title_short Synthesis of new surface-active ammonium-type complexes based on palmitic acid for removing thin petroleum films from water surface
title_sort synthesis of new surface active ammonium type complexes based on palmitic acid for removing thin petroleum films from water surface
topic Palmitic acid
Nitrogen-containing compounds
Complex
Dispersing agent
Collecting agent
Propylene oxide
url http://www.sciencedirect.com/science/article/pii/S1110062113000536
work_keys_str_mv AT ziyafaddinhasadov synthesisofnewsurfaceactiveammoniumtypecomplexesbasedonpalmiticacidforremovingthinpetroleumfilmsfromwatersurface
AT ahmedhtantawy synthesisofnewsurfaceactiveammoniumtypecomplexesbasedonpalmiticacidforremovingthinpetroleumfilmsfromwatersurface
AT ilhamaazarbaliyeva synthesisofnewsurfaceactiveammoniumtypecomplexesbasedonpalmiticacidforremovingthinpetroleumfilmsfromwatersurface
AT ravanarahimov synthesisofnewsurfaceactiveammoniumtypecomplexesbasedonpalmiticacidforremovingthinpetroleumfilmsfromwatersurface