Gate-Controlled Three-Terminal ZnO Nanoparticle Optoelectronic Synaptic Devices for In-Sensor Neuromorphic Memory Applications

This study reports a gate-tunable three-terminal optoelectronic synaptic device based on an Al/ZnO nanoparticles (NPs)/SiO<sub>2</sub>/Si structure for neuromorphic in-sensor memory applications. The ZnO NP film, fabricated via spin coating, exhibited strong UV-induced excitatory post-sy...

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Main Authors: Dabin Jeon, Seung Hun Lee, Sung-Nam Lee
Format: Article
Language:English
Published: MDPI AG 2025-06-01
Series:Nanomaterials
Subjects:
Online Access:https://www.mdpi.com/2079-4991/15/12/908
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author Dabin Jeon
Seung Hun Lee
Sung-Nam Lee
author_facet Dabin Jeon
Seung Hun Lee
Sung-Nam Lee
author_sort Dabin Jeon
collection DOAJ
description This study reports a gate-tunable three-terminal optoelectronic synaptic device based on an Al/ZnO nanoparticles (NPs)/SiO<sub>2</sub>/Si structure for neuromorphic in-sensor memory applications. The ZnO NP film, fabricated via spin coating, exhibited strong UV-induced excitatory post-synaptic current (EPSC) responses that were modulated by gate voltage through charge injection across the SiO<sub>2</sub> dielectric rather than by conventional field effect. Optical stimulation enabled short-term synaptic plasticity, with paired-pulse facilitation (PPF) values reaching 185% at a gate voltage of −5.0 V and decreasing to 180% at +5.0 V, confirming gate-dependent modulation of synaptic weight. Repeated stimulation enhanced learning efficiency and memory retention, as demonstrated by reduced pulse numbers for relearning and slower EPSC decay. Wickelgren’s power law analysis further revealed a decrease in the forgetting rate under negative gate bias, indicating improved long-term memory characteristics. A 3 × 3 synaptic device array visualized visual memory formation through EPSC-based color mapping, with darker intensities and slower fading observed under −5.0 V bias. These results highlight the critical role of gate-voltage-induced charge injection through the SiO<sub>2</sub> dielectric in controlling optical potentiation and electrical depression, establishing ZnO NP-based optoelectronic synaptic devices as promising platforms for energy-efficient, light-driven neuromorphic computing.
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spelling doaj-art-a6febb790b7146aabffbdacc8dceb1172025-08-20T03:27:25ZengMDPI AGNanomaterials2079-49912025-06-01151290810.3390/nano15120908Gate-Controlled Three-Terminal ZnO Nanoparticle Optoelectronic Synaptic Devices for In-Sensor Neuromorphic Memory ApplicationsDabin Jeon0Seung Hun Lee1Sung-Nam Lee2Department of IT Semiconductor Convergence Engineering, Tech University of Korea, Siheung 15073, Republic of KoreaDepartment of IT Semiconductor Convergence Engineering, Tech University of Korea, Siheung 15073, Republic of KoreaDepartment of IT Semiconductor Convergence Engineering, Tech University of Korea, Siheung 15073, Republic of KoreaThis study reports a gate-tunable three-terminal optoelectronic synaptic device based on an Al/ZnO nanoparticles (NPs)/SiO<sub>2</sub>/Si structure for neuromorphic in-sensor memory applications. The ZnO NP film, fabricated via spin coating, exhibited strong UV-induced excitatory post-synaptic current (EPSC) responses that were modulated by gate voltage through charge injection across the SiO<sub>2</sub> dielectric rather than by conventional field effect. Optical stimulation enabled short-term synaptic plasticity, with paired-pulse facilitation (PPF) values reaching 185% at a gate voltage of −5.0 V and decreasing to 180% at +5.0 V, confirming gate-dependent modulation of synaptic weight. Repeated stimulation enhanced learning efficiency and memory retention, as demonstrated by reduced pulse numbers for relearning and slower EPSC decay. Wickelgren’s power law analysis further revealed a decrease in the forgetting rate under negative gate bias, indicating improved long-term memory characteristics. A 3 × 3 synaptic device array visualized visual memory formation through EPSC-based color mapping, with darker intensities and slower fading observed under −5.0 V bias. These results highlight the critical role of gate-voltage-induced charge injection through the SiO<sub>2</sub> dielectric in controlling optical potentiation and electrical depression, establishing ZnO NP-based optoelectronic synaptic devices as promising platforms for energy-efficient, light-driven neuromorphic computing.https://www.mdpi.com/2079-4991/15/12/908ZnOnanoparticle3-terminalsynapseoptoelectronicneuromorphic
spellingShingle Dabin Jeon
Seung Hun Lee
Sung-Nam Lee
Gate-Controlled Three-Terminal ZnO Nanoparticle Optoelectronic Synaptic Devices for In-Sensor Neuromorphic Memory Applications
Nanomaterials
ZnO
nanoparticle
3-terminal
synapse
optoelectronic
neuromorphic
title Gate-Controlled Three-Terminal ZnO Nanoparticle Optoelectronic Synaptic Devices for In-Sensor Neuromorphic Memory Applications
title_full Gate-Controlled Three-Terminal ZnO Nanoparticle Optoelectronic Synaptic Devices for In-Sensor Neuromorphic Memory Applications
title_fullStr Gate-Controlled Three-Terminal ZnO Nanoparticle Optoelectronic Synaptic Devices for In-Sensor Neuromorphic Memory Applications
title_full_unstemmed Gate-Controlled Three-Terminal ZnO Nanoparticle Optoelectronic Synaptic Devices for In-Sensor Neuromorphic Memory Applications
title_short Gate-Controlled Three-Terminal ZnO Nanoparticle Optoelectronic Synaptic Devices for In-Sensor Neuromorphic Memory Applications
title_sort gate controlled three terminal zno nanoparticle optoelectronic synaptic devices for in sensor neuromorphic memory applications
topic ZnO
nanoparticle
3-terminal
synapse
optoelectronic
neuromorphic
url https://www.mdpi.com/2079-4991/15/12/908
work_keys_str_mv AT dabinjeon gatecontrolledthreeterminalznonanoparticleoptoelectronicsynapticdevicesforinsensorneuromorphicmemoryapplications
AT seunghunlee gatecontrolledthreeterminalznonanoparticleoptoelectronicsynapticdevicesforinsensorneuromorphicmemoryapplications
AT sungnamlee gatecontrolledthreeterminalznonanoparticleoptoelectronicsynapticdevicesforinsensorneuromorphicmemoryapplications