Studying the temporal bias of the steady-state approximation of 234Th-derived carbon export during phytoplankton blooms

The 234Th–238U pair technique is widely used in estimating particulate organic carbon (POC) flux, typically with a steady-state (SS) assumption. There is often a temporal bias between the SS-derived and actual POC fluxes caused by neglecting the temporal change in 234Th. However, this temporal bias...

Full description

Saved in:
Bibliographic Details
Main Authors: Mingxian Guo, Peng Xiu, Kuanbo Zhou
Format: Article
Language:English
Published: Frontiers Media S.A. 2025-04-01
Series:Frontiers in Marine Science
Subjects:
Online Access:https://www.frontiersin.org/articles/10.3389/fmars.2025.1554932/full
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1849736096571719680
author Mingxian Guo
Mingxian Guo
Peng Xiu
Peng Xiu
Kuanbo Zhou
Kuanbo Zhou
author_facet Mingxian Guo
Mingxian Guo
Peng Xiu
Peng Xiu
Kuanbo Zhou
Kuanbo Zhou
author_sort Mingxian Guo
collection DOAJ
description The 234Th–238U pair technique is widely used in estimating particulate organic carbon (POC) flux, typically with a steady-state (SS) assumption. There is often a temporal bias between the SS-derived and actual POC fluxes caused by neglecting the temporal change in 234Th. However, this temporal bias has not been fully investigated due to the lack of continuous sampling of 234Th profiles and sediment traps. Here, we develop a radioactive trace model of 234Th built on a physical–biogeochemical model to simulate the scavenging of 234Th in the water column by POC sinking processes at the South East Asia time series (SEATS) site. The seasonal patterns of the 234Th profiles simulated by the model generally compared well with in situ observations. Analysis based on the model simulation suggests that the temporal bias can be depicted and reproduced in a simplified 234Th continuity equation. By obtaining an analytical solution for the SS-derived POC flux from the simplified 234Th equation, we found that the temporal bias results from the phase difference in time between the SS-derived and direct sinking POC fluxes. To provide a method that does not need repeated samplings to reduce this temporal bias for in situ observations, a modification term was constructed for the SS-derived POC flux from the analytical solution. Applying this term to the data obtained at the Bermuda Atlantic time series and SEATS reduced the bias by up to 67% and 34%, respectively. This study provides a feasible way to improve 234Th-derived POC flux under the SS assumption.
format Article
id doaj-art-a6c60f44ce3a42638d7710454b4e5651
institution DOAJ
issn 2296-7745
language English
publishDate 2025-04-01
publisher Frontiers Media S.A.
record_format Article
series Frontiers in Marine Science
spelling doaj-art-a6c60f44ce3a42638d7710454b4e56512025-08-20T03:07:21ZengFrontiers Media S.A.Frontiers in Marine Science2296-77452025-04-011210.3389/fmars.2025.15549321554932Studying the temporal bias of the steady-state approximation of 234Th-derived carbon export during phytoplankton bloomsMingxian Guo0Mingxian Guo1Peng Xiu2Peng Xiu3Kuanbo Zhou4Kuanbo Zhou5State Key Laboratory of Tropical Oceanography, South China Sea Institute of Oceanology, Chinese Academy of Sciences, Guangzhou, ChinaGuangdong Key Laboratory of Ocean Remote Sensing, South China Sea Institute of Oceanology, Chinese Academy of Sciences, Guangzhou, ChinaState Key Laboratory of Marine Environmental Science, Xiamen University, Xiamen, ChinaCollege of Ocean and Earth, Sciences, Xiamen University, Xiamen, ChinaState Key Laboratory of Marine Environmental Science, Xiamen University, Xiamen, ChinaCollege of Ocean and Earth, Sciences, Xiamen University, Xiamen, ChinaThe 234Th–238U pair technique is widely used in estimating particulate organic carbon (POC) flux, typically with a steady-state (SS) assumption. There is often a temporal bias between the SS-derived and actual POC fluxes caused by neglecting the temporal change in 234Th. However, this temporal bias has not been fully investigated due to the lack of continuous sampling of 234Th profiles and sediment traps. Here, we develop a radioactive trace model of 234Th built on a physical–biogeochemical model to simulate the scavenging of 234Th in the water column by POC sinking processes at the South East Asia time series (SEATS) site. The seasonal patterns of the 234Th profiles simulated by the model generally compared well with in situ observations. Analysis based on the model simulation suggests that the temporal bias can be depicted and reproduced in a simplified 234Th continuity equation. By obtaining an analytical solution for the SS-derived POC flux from the simplified 234Th equation, we found that the temporal bias results from the phase difference in time between the SS-derived and direct sinking POC fluxes. To provide a method that does not need repeated samplings to reduce this temporal bias for in situ observations, a modification term was constructed for the SS-derived POC flux from the analytical solution. Applying this term to the data obtained at the Bermuda Atlantic time series and SEATS reduced the bias by up to 67% and 34%, respectively. This study provides a feasible way to improve 234Th-derived POC flux under the SS assumption.https://www.frontiersin.org/articles/10.3389/fmars.2025.1554932/fullbiological carbon pumpparticulate organic carbon fluxthe 234Th–238U pair techniquea radioactive trace model of 234Therror correction
spellingShingle Mingxian Guo
Mingxian Guo
Peng Xiu
Peng Xiu
Kuanbo Zhou
Kuanbo Zhou
Studying the temporal bias of the steady-state approximation of 234Th-derived carbon export during phytoplankton blooms
Frontiers in Marine Science
biological carbon pump
particulate organic carbon flux
the 234Th–238U pair technique
a radioactive trace model of 234Th
error correction
title Studying the temporal bias of the steady-state approximation of 234Th-derived carbon export during phytoplankton blooms
title_full Studying the temporal bias of the steady-state approximation of 234Th-derived carbon export during phytoplankton blooms
title_fullStr Studying the temporal bias of the steady-state approximation of 234Th-derived carbon export during phytoplankton blooms
title_full_unstemmed Studying the temporal bias of the steady-state approximation of 234Th-derived carbon export during phytoplankton blooms
title_short Studying the temporal bias of the steady-state approximation of 234Th-derived carbon export during phytoplankton blooms
title_sort studying the temporal bias of the steady state approximation of 234th derived carbon export during phytoplankton blooms
topic biological carbon pump
particulate organic carbon flux
the 234Th–238U pair technique
a radioactive trace model of 234Th
error correction
url https://www.frontiersin.org/articles/10.3389/fmars.2025.1554932/full
work_keys_str_mv AT mingxianguo studyingthetemporalbiasofthesteadystateapproximationof234thderivedcarbonexportduringphytoplanktonblooms
AT mingxianguo studyingthetemporalbiasofthesteadystateapproximationof234thderivedcarbonexportduringphytoplanktonblooms
AT pengxiu studyingthetemporalbiasofthesteadystateapproximationof234thderivedcarbonexportduringphytoplanktonblooms
AT pengxiu studyingthetemporalbiasofthesteadystateapproximationof234thderivedcarbonexportduringphytoplanktonblooms
AT kuanbozhou studyingthetemporalbiasofthesteadystateapproximationof234thderivedcarbonexportduringphytoplanktonblooms
AT kuanbozhou studyingthetemporalbiasofthesteadystateapproximationof234thderivedcarbonexportduringphytoplanktonblooms