Current-driven nonequilibrium electrodynamics in graphene revealed by nano-infrared imaging
Abstract Electrons in low-dimensional materials driven out of equilibrium by a strong electric field exhibit intriguing effects that have direct analogues in high-energy physics. In this work we demonstrate that two of these effects can be observed in graphene, leading to relevant implications for l...
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| Language: | English |
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Nature Portfolio
2025-04-01
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| Series: | Nature Communications |
| Online Access: | https://doi.org/10.1038/s41467-025-58953-6 |
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| author | Y. Dong Z. Sun I. Y. Phinney D. Sun T. I. Andersen L. Xiong Y. Shao S. Zhang Andrey Rikhter S. Liu P. Jarillo-Herrero P. Kim C. R. Dean A. J. Millis M. M. Fogler D. A. Bandurin D. N. Basov |
| author_facet | Y. Dong Z. Sun I. Y. Phinney D. Sun T. I. Andersen L. Xiong Y. Shao S. Zhang Andrey Rikhter S. Liu P. Jarillo-Herrero P. Kim C. R. Dean A. J. Millis M. M. Fogler D. A. Bandurin D. N. Basov |
| author_sort | Y. Dong |
| collection | DOAJ |
| description | Abstract Electrons in low-dimensional materials driven out of equilibrium by a strong electric field exhibit intriguing effects that have direct analogues in high-energy physics. In this work we demonstrate that two of these effects can be observed in graphene, leading to relevant implications for light-matter interactions at the nanoscale. For doped graphene, the Cherenkov emission of phonons caused by the fast flow of out-of-equilibrium electrons was found to induce direction-dependent asymmetric plasmon damping and an unexpected generation of photocurrent. For graphene close to charge neutrality, incident infrared photons were found to disrupt the creation-recombination balance of electron-hole pairs enabled by the condensed matter version of the Schwinger effect, resulting in an excess photocurrent that we term Schwinger photocurrent. Both Schwinger and Cherenkov photocurrents are different from other known light-to-current down conversions scenarios and thus expand the family of photoelectric effects in solid state devices. Through nano-infrared imaging methodology, we provide a more comprehensive view of current-driven nonequilibrium electrodynamics in graphene. |
| format | Article |
| id | doaj-art-a6771ff1cc5b4909989d1ab23a37808c |
| institution | OA Journals |
| issn | 2041-1723 |
| language | English |
| publishDate | 2025-04-01 |
| publisher | Nature Portfolio |
| record_format | Article |
| series | Nature Communications |
| spelling | doaj-art-a6771ff1cc5b4909989d1ab23a37808c2025-08-20T02:28:41ZengNature PortfolioNature Communications2041-17232025-04-011611810.1038/s41467-025-58953-6Current-driven nonequilibrium electrodynamics in graphene revealed by nano-infrared imagingY. Dong0Z. Sun1I. Y. Phinney2D. Sun3T. I. Andersen4L. Xiong5Y. Shao6S. Zhang7Andrey Rikhter8S. Liu9P. Jarillo-Herrero10P. Kim11C. R. Dean12A. J. Millis13M. M. Fogler14D. A. Bandurin15D. N. Basov16Department of Applied Physics and Applied Mathematics, Columbia UniversityDepartment of Physics, Columbia UniversityDepartment of Physics, Massachusetts Institute of TechnologyDepartment of Physics, Columbia UniversityDepartment of Physics, Harvard UniversityDepartment of Physics, Columbia UniversityDepartment of Physics, Columbia UniversityDepartment of Physics, Columbia UniversityDepartment of Physics, University of California San DiegoDepartment of Mechanical Engineering, Columbia UniversityDepartment of Physics, Massachusetts Institute of TechnologyDepartment of Physics, Harvard UniversityDepartment of Physics, Columbia UniversityDepartment of Physics, Columbia UniversityDepartment of Physics, University of California San DiegoDepartment of Materials Science and Engineering, National University of SingaporeDepartment of Physics, Columbia UniversityAbstract Electrons in low-dimensional materials driven out of equilibrium by a strong electric field exhibit intriguing effects that have direct analogues in high-energy physics. In this work we demonstrate that two of these effects can be observed in graphene, leading to relevant implications for light-matter interactions at the nanoscale. For doped graphene, the Cherenkov emission of phonons caused by the fast flow of out-of-equilibrium electrons was found to induce direction-dependent asymmetric plasmon damping and an unexpected generation of photocurrent. For graphene close to charge neutrality, incident infrared photons were found to disrupt the creation-recombination balance of electron-hole pairs enabled by the condensed matter version of the Schwinger effect, resulting in an excess photocurrent that we term Schwinger photocurrent. Both Schwinger and Cherenkov photocurrents are different from other known light-to-current down conversions scenarios and thus expand the family of photoelectric effects in solid state devices. Through nano-infrared imaging methodology, we provide a more comprehensive view of current-driven nonequilibrium electrodynamics in graphene.https://doi.org/10.1038/s41467-025-58953-6 |
| spellingShingle | Y. Dong Z. Sun I. Y. Phinney D. Sun T. I. Andersen L. Xiong Y. Shao S. Zhang Andrey Rikhter S. Liu P. Jarillo-Herrero P. Kim C. R. Dean A. J. Millis M. M. Fogler D. A. Bandurin D. N. Basov Current-driven nonequilibrium electrodynamics in graphene revealed by nano-infrared imaging Nature Communications |
| title | Current-driven nonequilibrium electrodynamics in graphene revealed by nano-infrared imaging |
| title_full | Current-driven nonequilibrium electrodynamics in graphene revealed by nano-infrared imaging |
| title_fullStr | Current-driven nonequilibrium electrodynamics in graphene revealed by nano-infrared imaging |
| title_full_unstemmed | Current-driven nonequilibrium electrodynamics in graphene revealed by nano-infrared imaging |
| title_short | Current-driven nonequilibrium electrodynamics in graphene revealed by nano-infrared imaging |
| title_sort | current driven nonequilibrium electrodynamics in graphene revealed by nano infrared imaging |
| url | https://doi.org/10.1038/s41467-025-58953-6 |
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