Crystallization and melting behavior of nanoclay-containing polypropylene/poly(trimethylene terephthalate) blends

This contribution concerns preparation and characterization of polypropylene (PP)/poly(trimethylene terephthalate) (PTT) melt-mixed blends in the presence of organically-modified montmorillonite nanoclays and functional compatibilizers. Immiscibility and nanocomposite formation were confirmed via tr...

Full description

Saved in:
Bibliographic Details
Main Authors: S. H. Jafari, A. Kalati-vahid, H. A. Khonakdar, A. Asadinezhad, U. Wagenknecht, D. Jehnichen
Format: Article
Language:English
Published: Budapest University of Technology and Economics 2012-02-01
Series:eXPRESS Polymer Letters
Subjects:
Online Access:http://www.expresspolymlett.com/letolt.php?file=EPL-0002637&mi=cd
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1849404422416760832
author S. H. Jafari
A. Kalati-vahid
H. A. Khonakdar
A. Asadinezhad
U. Wagenknecht
D. Jehnichen
author_facet S. H. Jafari
A. Kalati-vahid
H. A. Khonakdar
A. Asadinezhad
U. Wagenknecht
D. Jehnichen
author_sort S. H. Jafari
collection DOAJ
description This contribution concerns preparation and characterization of polypropylene (PP)/poly(trimethylene terephthalate) (PTT) melt-mixed blends in the presence of organically-modified montmorillonite nanoclays and functional compatibilizers. Immiscibility and nanocomposite formation were confirmed via transmission electron microscopy. An intercalated structure was observed by wide angle X-ray diffraction technique. Crystallization, and melting characteristics were studied by differential scanning calorimetry in both isothermal and non-isothermal modes, supplemented by temperature modulated DSC (TMDSC). A concurrent crystallization was found for both polymeric components in the blends. Whereas blending favored PP crystallizability, it interrupted that of PTT. The addition compatibilizers interfered with rate, temperature, and degree of crystallization of PP and PTT. On the contrary, nanoclays incorporation increased crystallizability of each individual component. However, as for blend nanocomposite samples, the way the crystallization behavior changed was established to depend on the type of nanoclay. Based on kinetic analysis, isothermal crystallization nucleation followed athermal mechanism, while that of non-isothermal obeyed thermal mode. Addition of nanoclays shifted nucleation mechanism from athermal to thermal mode.
format Article
id doaj-art-a59294573fd44decaccbe082ebdbd538
institution Kabale University
issn 1788-618X
language English
publishDate 2012-02-01
publisher Budapest University of Technology and Economics
record_format Article
series eXPRESS Polymer Letters
spelling doaj-art-a59294573fd44decaccbe082ebdbd5382025-08-20T03:36:58ZengBudapest University of Technology and EconomicseXPRESS Polymer Letters1788-618X2012-02-016214815810.3144/expresspolymlett.2012.16Crystallization and melting behavior of nanoclay-containing polypropylene/poly(trimethylene terephthalate) blendsS. H. JafariA. Kalati-vahidH. A. KhonakdarA. AsadinezhadU. WagenknechtD. JehnichenThis contribution concerns preparation and characterization of polypropylene (PP)/poly(trimethylene terephthalate) (PTT) melt-mixed blends in the presence of organically-modified montmorillonite nanoclays and functional compatibilizers. Immiscibility and nanocomposite formation were confirmed via transmission electron microscopy. An intercalated structure was observed by wide angle X-ray diffraction technique. Crystallization, and melting characteristics were studied by differential scanning calorimetry in both isothermal and non-isothermal modes, supplemented by temperature modulated DSC (TMDSC). A concurrent crystallization was found for both polymeric components in the blends. Whereas blending favored PP crystallizability, it interrupted that of PTT. The addition compatibilizers interfered with rate, temperature, and degree of crystallization of PP and PTT. On the contrary, nanoclays incorporation increased crystallizability of each individual component. However, as for blend nanocomposite samples, the way the crystallization behavior changed was established to depend on the type of nanoclay. Based on kinetic analysis, isothermal crystallization nucleation followed athermal mechanism, while that of non-isothermal obeyed thermal mode. Addition of nanoclays shifted nucleation mechanism from athermal to thermal mode.http://www.expresspolymlett.com/letolt.php?file=EPL-0002637&mi=cdNanocompositespolymer blendscrystallizationpolypropylenePoly(trimethylene terephthalat
spellingShingle S. H. Jafari
A. Kalati-vahid
H. A. Khonakdar
A. Asadinezhad
U. Wagenknecht
D. Jehnichen
Crystallization and melting behavior of nanoclay-containing polypropylene/poly(trimethylene terephthalate) blends
eXPRESS Polymer Letters
Nanocomposites
polymer blends
crystallization
polypropylene
Poly(trimethylene terephthalat
title Crystallization and melting behavior of nanoclay-containing polypropylene/poly(trimethylene terephthalate) blends
title_full Crystallization and melting behavior of nanoclay-containing polypropylene/poly(trimethylene terephthalate) blends
title_fullStr Crystallization and melting behavior of nanoclay-containing polypropylene/poly(trimethylene terephthalate) blends
title_full_unstemmed Crystallization and melting behavior of nanoclay-containing polypropylene/poly(trimethylene terephthalate) blends
title_short Crystallization and melting behavior of nanoclay-containing polypropylene/poly(trimethylene terephthalate) blends
title_sort crystallization and melting behavior of nanoclay containing polypropylene poly trimethylene terephthalate blends
topic Nanocomposites
polymer blends
crystallization
polypropylene
Poly(trimethylene terephthalat
url http://www.expresspolymlett.com/letolt.php?file=EPL-0002637&mi=cd
work_keys_str_mv AT shjafari crystallizationandmeltingbehaviorofnanoclaycontainingpolypropylenepolytrimethyleneterephthalateblends
AT akalativahid crystallizationandmeltingbehaviorofnanoclaycontainingpolypropylenepolytrimethyleneterephthalateblends
AT hakhonakdar crystallizationandmeltingbehaviorofnanoclaycontainingpolypropylenepolytrimethyleneterephthalateblends
AT aasadinezhad crystallizationandmeltingbehaviorofnanoclaycontainingpolypropylenepolytrimethyleneterephthalateblends
AT uwagenknecht crystallizationandmeltingbehaviorofnanoclaycontainingpolypropylenepolytrimethyleneterephthalateblends
AT djehnichen crystallizationandmeltingbehaviorofnanoclaycontainingpolypropylenepolytrimethyleneterephthalateblends