Environmentally tolerant high-adhesion conductive eutectogels

This study presents the development of environmentally tolerant, high-adhesion conductive eutectogels based on poly(N-hydroxyethyl acrylamide) (PHEAA) based eutectogels. The eutectogels were synthesized via a one-pot polymerization process, resulting in materials with exceptional mechanical properti...

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Main Authors: Jiating Liu, Ying Chen, Shuo Li, Pengcheng Zhao, Tao Li, Tian Zhao, Yi Chen
Format: Article
Language:English
Published: Elsevier 2025-04-01
Series:Polymer Testing
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Online Access:http://www.sciencedirect.com/science/article/pii/S0142941825000674
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author Jiating Liu
Ying Chen
Shuo Li
Pengcheng Zhao
Tao Li
Tian Zhao
Yi Chen
author_facet Jiating Liu
Ying Chen
Shuo Li
Pengcheng Zhao
Tao Li
Tian Zhao
Yi Chen
author_sort Jiating Liu
collection DOAJ
description This study presents the development of environmentally tolerant, high-adhesion conductive eutectogels based on poly(N-hydroxyethyl acrylamide) (PHEAA) based eutectogels. The eutectogels were synthesized via a one-pot polymerization process, resulting in materials with exceptional mechanical properties, including high stretchability, tear resistance, and self-recovery capabilities. The eutectogels exhibited strong adhesion to various substrates, making them suitable for flexible sensor applications. Their non-volatile nature and thermal stability provided outstanding environmental tolerance, maintaining flexibility across a wide temperature range. Additionally, the eutectogels demonstrated high ionic conductivity and precise responsiveness, enabling their use in strain sensors and real-time electrocardiogram (ECG) monitoring. The results highlight the potential of PHEAA/DESs eutectogels for applications in flexible electronics, healthcare monitoring, and smart materials.
format Article
id doaj-art-a3ba0818b4d247bc8243e0c5bd02762f
institution OA Journals
issn 1873-2348
language English
publishDate 2025-04-01
publisher Elsevier
record_format Article
series Polymer Testing
spelling doaj-art-a3ba0818b4d247bc8243e0c5bd02762f2025-08-20T02:26:09ZengElsevierPolymer Testing1873-23482025-04-0114510875310.1016/j.polymertesting.2025.108753Environmentally tolerant high-adhesion conductive eutectogelsJiating Liu0Ying Chen1Shuo Li2Pengcheng Zhao3Tao Li4Tian Zhao5Yi Chen6Hunan Provincial Key Laboratory of Biomass Fiber Functional Materials, School of Packaging Materials and Engineering, Hunan University of Technology, Zhuzhou, Hunan, 412007, China; College of Packing and Materials Engineering, Hunan University of Technology, Zhuzhou, Hunan, 412007, ChinaHunan Provincial Key Laboratory of Biomass Fiber Functional Materials, School of Packaging Materials and Engineering, Hunan University of Technology, Zhuzhou, Hunan, 412007, China; National & Local Joint Engineering Research Center for Advanced Packaging Material and Technology, Hunan University of Technology, Zhuzhou, Hunan, 412007, ChinaHunan Provincial Key Laboratory of Biomass Fiber Functional Materials, School of Packaging Materials and Engineering, Hunan University of Technology, Zhuzhou, Hunan, 412007, China; College of Packing and Materials Engineering, Hunan University of Technology, Zhuzhou, Hunan, 412007, ChinaHunan Provincial Key Laboratory of Biomass Fiber Functional Materials, School of Packaging Materials and Engineering, Hunan University of Technology, Zhuzhou, Hunan, 412007, China; College of Packing and Materials Engineering, Hunan University of Technology, Zhuzhou, Hunan, 412007, ChinaHunan Provincial Key Laboratory of Biomass Fiber Functional Materials, School of Packaging Materials and Engineering, Hunan University of Technology, Zhuzhou, Hunan, 412007, China; College of Packing and Materials Engineering, Hunan University of Technology, Zhuzhou, Hunan, 412007, ChinaHunan Provincial Key Laboratory of Biomass Fiber Functional Materials, School of Packaging Materials and Engineering, Hunan University of Technology, Zhuzhou, Hunan, 412007, China; College of Packing and Materials Engineering, Hunan University of Technology, Zhuzhou, Hunan, 412007, ChinaHunan Provincial Key Laboratory of Biomass Fiber Functional Materials, School of Packaging Materials and Engineering, Hunan University of Technology, Zhuzhou, Hunan, 412007, China; College of Packing and Materials Engineering, Hunan University of Technology, Zhuzhou, Hunan, 412007, China; National & Local Joint Engineering Research Center for Advanced Packaging Material and Technology, Hunan University of Technology, Zhuzhou, Hunan, 412007, China; Corresponding author. Hunan Provincial Key Laboratory of Biomass Fiber Functional Materials, School of Packaging Materials and Engineering, Hunan University of Technology, Zhuzhou, Hunan, 412007, China.This study presents the development of environmentally tolerant, high-adhesion conductive eutectogels based on poly(N-hydroxyethyl acrylamide) (PHEAA) based eutectogels. The eutectogels were synthesized via a one-pot polymerization process, resulting in materials with exceptional mechanical properties, including high stretchability, tear resistance, and self-recovery capabilities. The eutectogels exhibited strong adhesion to various substrates, making them suitable for flexible sensor applications. Their non-volatile nature and thermal stability provided outstanding environmental tolerance, maintaining flexibility across a wide temperature range. Additionally, the eutectogels demonstrated high ionic conductivity and precise responsiveness, enabling their use in strain sensors and real-time electrocardiogram (ECG) monitoring. The results highlight the potential of PHEAA/DESs eutectogels for applications in flexible electronics, healthcare monitoring, and smart materials.http://www.sciencedirect.com/science/article/pii/S0142941825000674EutectogelsRemoldabilityIonic conductivityFlexible sensorsHealthcare monitoring
spellingShingle Jiating Liu
Ying Chen
Shuo Li
Pengcheng Zhao
Tao Li
Tian Zhao
Yi Chen
Environmentally tolerant high-adhesion conductive eutectogels
Polymer Testing
Eutectogels
Remoldability
Ionic conductivity
Flexible sensors
Healthcare monitoring
title Environmentally tolerant high-adhesion conductive eutectogels
title_full Environmentally tolerant high-adhesion conductive eutectogels
title_fullStr Environmentally tolerant high-adhesion conductive eutectogels
title_full_unstemmed Environmentally tolerant high-adhesion conductive eutectogels
title_short Environmentally tolerant high-adhesion conductive eutectogels
title_sort environmentally tolerant high adhesion conductive eutectogels
topic Eutectogels
Remoldability
Ionic conductivity
Flexible sensors
Healthcare monitoring
url http://www.sciencedirect.com/science/article/pii/S0142941825000674
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AT shuoli environmentallytoleranthighadhesionconductiveeutectogels
AT pengchengzhao environmentallytoleranthighadhesionconductiveeutectogels
AT taoli environmentallytoleranthighadhesionconductiveeutectogels
AT tianzhao environmentallytoleranthighadhesionconductiveeutectogels
AT yichen environmentallytoleranthighadhesionconductiveeutectogels