ELECTROCHEMICAL INVESTIGATION OF OCTAETHYL PORPHYRIN IRON(III) CHLORIDE IN THE PRESENCE OF PYRIDINE, IMIDAZOLE AND COLLIDINE: AN APPROACH TO THE ROLE OF PYRIDINE IN THE COUPLED OXIDATION

Cyclic voltammogram and differential pulse polarograph of octaethyl porphyrin iron(III) chloride in dichloromethane was investigated in the presence of pyridine, imidazole and collidine. Values of E1/2 for FeIII/FeII redox reaction were monitored as a function of axial group concentration, and on th...

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Format: Article
Language:English
Published: University of Tehran 2000-06-01
Series:Journal of Sciences, Islamic Republic of Iran
Online Access:https://jsciences.ut.ac.ir/article_31852_828416030a1cc4cc630c596bfbf73f3f.pdf
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description Cyclic voltammogram and differential pulse polarograph of octaethyl porphyrin iron(III) chloride in dichloromethane was investigated in the presence of pyridine, imidazole and collidine. Values of E1/2 for FeIII/FeII redox reaction were monitored as a function of axial group concentration, and on the basis of these data, an overall oxidation-reduction and ligand addition scheme was formulated. Addition of pyridine resulted in anodic shift for oxidation wave from –0.16 V to –0.06 V while for imidazole and collidine we observed a cathodic shift.
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publishDate 2000-06-01
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series Journal of Sciences, Islamic Republic of Iran
spelling doaj-art-a2cea9f5402e4128a6d247380c764bb92025-08-20T02:25:51ZengUniversity of TehranJournal of Sciences, Islamic Republic of Iran1016-11042345-69142000-06-0111231852ELECTROCHEMICAL INVESTIGATION OF OCTAETHYL PORPHYRIN IRON(III) CHLORIDE IN THE PRESENCE OF PYRIDINE, IMIDAZOLE AND COLLIDINE: AN APPROACH TO THE ROLE OF PYRIDINE IN THE COUPLED OXIDATIONCyclic voltammogram and differential pulse polarograph of octaethyl porphyrin iron(III) chloride in dichloromethane was investigated in the presence of pyridine, imidazole and collidine. Values of E1/2 for FeIII/FeII redox reaction were monitored as a function of axial group concentration, and on the basis of these data, an overall oxidation-reduction and ligand addition scheme was formulated. Addition of pyridine resulted in anodic shift for oxidation wave from –0.16 V to –0.06 V while for imidazole and collidine we observed a cathodic shift.https://jsciences.ut.ac.ir/article_31852_828416030a1cc4cc630c596bfbf73f3f.pdf
spellingShingle ELECTROCHEMICAL INVESTIGATION OF OCTAETHYL PORPHYRIN IRON(III) CHLORIDE IN THE PRESENCE OF PYRIDINE, IMIDAZOLE AND COLLIDINE: AN APPROACH TO THE ROLE OF PYRIDINE IN THE COUPLED OXIDATION
Journal of Sciences, Islamic Republic of Iran
title ELECTROCHEMICAL INVESTIGATION OF OCTAETHYL PORPHYRIN IRON(III) CHLORIDE IN THE PRESENCE OF PYRIDINE, IMIDAZOLE AND COLLIDINE: AN APPROACH TO THE ROLE OF PYRIDINE IN THE COUPLED OXIDATION
title_full ELECTROCHEMICAL INVESTIGATION OF OCTAETHYL PORPHYRIN IRON(III) CHLORIDE IN THE PRESENCE OF PYRIDINE, IMIDAZOLE AND COLLIDINE: AN APPROACH TO THE ROLE OF PYRIDINE IN THE COUPLED OXIDATION
title_fullStr ELECTROCHEMICAL INVESTIGATION OF OCTAETHYL PORPHYRIN IRON(III) CHLORIDE IN THE PRESENCE OF PYRIDINE, IMIDAZOLE AND COLLIDINE: AN APPROACH TO THE ROLE OF PYRIDINE IN THE COUPLED OXIDATION
title_full_unstemmed ELECTROCHEMICAL INVESTIGATION OF OCTAETHYL PORPHYRIN IRON(III) CHLORIDE IN THE PRESENCE OF PYRIDINE, IMIDAZOLE AND COLLIDINE: AN APPROACH TO THE ROLE OF PYRIDINE IN THE COUPLED OXIDATION
title_short ELECTROCHEMICAL INVESTIGATION OF OCTAETHYL PORPHYRIN IRON(III) CHLORIDE IN THE PRESENCE OF PYRIDINE, IMIDAZOLE AND COLLIDINE: AN APPROACH TO THE ROLE OF PYRIDINE IN THE COUPLED OXIDATION
title_sort electrochemical investigation of octaethyl porphyrin iron iii chloride in the presence of pyridine imidazole and collidine an approach to the role of pyridine in the coupled oxidation
url https://jsciences.ut.ac.ir/article_31852_828416030a1cc4cc630c596bfbf73f3f.pdf