Plasmonic slot waveguides: a quantum leap in nonlinear nanophotonics

Interest and excitement in nanophotonics—the study and control of light-matter interactions at the nanoscale—are driven by the ability to confine light to volumes well below a cubic wavelength, and, thereby, achieve extremely high intensities. This leads to light-matter interactions of unprecedented...

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Main Authors: Libertad Rojas Yanez, Huatian Hu, Cristian Ciracì, Stefano Palomba
Format: Article
Language:English
Published: Frontiers Media S.A. 2025-02-01
Series:Frontiers in Nanotechnology
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Online Access:https://www.frontiersin.org/articles/10.3389/fnano.2025.1536462/full
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author Libertad Rojas Yanez
Huatian Hu
Cristian Ciracì
Stefano Palomba
author_facet Libertad Rojas Yanez
Huatian Hu
Cristian Ciracì
Stefano Palomba
author_sort Libertad Rojas Yanez
collection DOAJ
description Interest and excitement in nanophotonics—the study and control of light-matter interactions at the nanoscale—are driven by the ability to confine light to volumes well below a cubic wavelength, and, thereby, achieve extremely high intensities. This leads to light-matter interactions of unprecedented localization and strength. Such extreme behavior—both in terms of field enhancement and localization—can be achieved using plasmonic nanostructures, which concentrate light in regions much smaller than the wavelength of light, reducing the excitation power and, under certain conditions, removing phase-matching requirements in the nonlinear regime. In this study, we theoretically show that metal–dielectric–metal (MDM) slot waveguides (WGs), consisting of a thin dielectric layer sandwiched between metal films, provide the strongest confinement. We also demonstrate that integrating epsilon-near-zero (ENZ) materials within the MDM slot significantly improves the nonlinear conversion efficiency of these structures. The results show that the degenerate four-wave mixing conversion efficiency of these ENZ-MDM structures surpasses that of regular plasmonic structures and their dielectric counterparts, even under low pump power conditions, and remains robust despite higher losses in the ENZ material.
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publishDate 2025-02-01
publisher Frontiers Media S.A.
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series Frontiers in Nanotechnology
spelling doaj-art-a2b2b4e6a6b5466d9f2e98b8c37d6bcb2025-08-20T03:11:22ZengFrontiers Media S.A.Frontiers in Nanotechnology2673-30132025-02-01710.3389/fnano.2025.15364621536462Plasmonic slot waveguides: a quantum leap in nonlinear nanophotonicsLibertad Rojas Yanez0Huatian Hu1Cristian Ciracì2Stefano Palomba3Institute for Photonics and Optical Sciences, School of Physics, University of Sydney, Sydney, NSW, AustraliaIstituto Italiano di Tecnologia, Center for Biomolecular Nanotechnologies, Lecce, ItalyIstituto Italiano di Tecnologia, Center for Biomolecular Nanotechnologies, Lecce, ItalyInstitute for Photonics and Optical Sciences, School of Physics, University of Sydney, Sydney, NSW, AustraliaInterest and excitement in nanophotonics—the study and control of light-matter interactions at the nanoscale—are driven by the ability to confine light to volumes well below a cubic wavelength, and, thereby, achieve extremely high intensities. This leads to light-matter interactions of unprecedented localization and strength. Such extreme behavior—both in terms of field enhancement and localization—can be achieved using plasmonic nanostructures, which concentrate light in regions much smaller than the wavelength of light, reducing the excitation power and, under certain conditions, removing phase-matching requirements in the nonlinear regime. In this study, we theoretically show that metal–dielectric–metal (MDM) slot waveguides (WGs), consisting of a thin dielectric layer sandwiched between metal films, provide the strongest confinement. We also demonstrate that integrating epsilon-near-zero (ENZ) materials within the MDM slot significantly improves the nonlinear conversion efficiency of these structures. The results show that the degenerate four-wave mixing conversion efficiency of these ENZ-MDM structures surpasses that of regular plasmonic structures and their dielectric counterparts, even under low pump power conditions, and remains robust despite higher losses in the ENZ material.https://www.frontiersin.org/articles/10.3389/fnano.2025.1536462/fullmetal–dielectric–metal slot waveguidenonlinear plasmonicsepsilon-near-zero materialsnanophotonicsfour-wave mixing
spellingShingle Libertad Rojas Yanez
Huatian Hu
Cristian Ciracì
Stefano Palomba
Plasmonic slot waveguides: a quantum leap in nonlinear nanophotonics
Frontiers in Nanotechnology
metal–dielectric–metal slot waveguide
nonlinear plasmonics
epsilon-near-zero materials
nanophotonics
four-wave mixing
title Plasmonic slot waveguides: a quantum leap in nonlinear nanophotonics
title_full Plasmonic slot waveguides: a quantum leap in nonlinear nanophotonics
title_fullStr Plasmonic slot waveguides: a quantum leap in nonlinear nanophotonics
title_full_unstemmed Plasmonic slot waveguides: a quantum leap in nonlinear nanophotonics
title_short Plasmonic slot waveguides: a quantum leap in nonlinear nanophotonics
title_sort plasmonic slot waveguides a quantum leap in nonlinear nanophotonics
topic metal–dielectric–metal slot waveguide
nonlinear plasmonics
epsilon-near-zero materials
nanophotonics
four-wave mixing
url https://www.frontiersin.org/articles/10.3389/fnano.2025.1536462/full
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AT cristianciraci plasmonicslotwaveguidesaquantumleapinnonlinearnanophotonics
AT stefanopalomba plasmonicslotwaveguidesaquantumleapinnonlinearnanophotonics