Modelling key reactive processes relevant to bisulfide transport through highly compacted bentonite

The Canadian deep geological repository (DGR) design consists of copper coated used fuel containers (UFCs) placed within a highly compacted bentonite (HCB) buffer surrounded by a suitable host rock. Although the copper is thermodynamically stable in oxygen-free environments, it is potentially suscep...

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Main Authors: Md Abdullah Asad, Tarek L. Rashwan, Ian L. Molnar, Mehran Behazin, Peter G. Keech, Magdalena M. Krol
Format: Article
Language:English
Published: Elsevier 2024-12-01
Series:Results in Engineering
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Online Access:http://www.sciencedirect.com/science/article/pii/S2590123024017389
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author Md Abdullah Asad
Tarek L. Rashwan
Ian L. Molnar
Mehran Behazin
Peter G. Keech
Magdalena M. Krol
author_facet Md Abdullah Asad
Tarek L. Rashwan
Ian L. Molnar
Mehran Behazin
Peter G. Keech
Magdalena M. Krol
author_sort Md Abdullah Asad
collection DOAJ
description The Canadian deep geological repository (DGR) design consists of copper coated used fuel containers (UFCs) placed within a highly compacted bentonite (HCB) buffer surrounded by a suitable host rock. Although the copper is thermodynamically stable in oxygen-free environments, it is potentially susceptible to microbiologically influenced corrosion from bisulfide (HS-). Therefore, understanding HS- corrosion is important to ensure long-term performance of UFCs. Various reactions in the bentonite barrier of the DGR can affect HS- transport through the HCB and therefore the extent of copper corrosion caused by HS-. Since HS- transport and reactive processes are interconnected, numerical models are required to assess the complex HS- reactive transport dynamics and quantify the influence of reactive processes on HS- transport and corrosion. In this paper, various HS- transport models were coupled with (i) a key geochemical reaction between HS- and iron (i.e., simulating HS- retardation due to iron sulfide formation) or (ii) HS- adsorption. Since HS- is an anion, anion exclusion was also explored. Valuable insight was obtained through validation, comparison, and sensitivity analyses of these models. A comparison between experimental and modelled HS- transport dynamics showed that HS- is being retained by the bentonite due to reactive processes and anion exclusion is occurring. Lastly, HS- transport was simulated for the entire DGR lifespan and was found to be delayed (≈50–800 years) due to FeS formation or HS- adsorption. However, these predicted HS- diffusion delays are relatively short in a DGR lifespan (i.e., 1 million years) and do not impact long-term HS- corrosion.
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spelling doaj-art-a2a55e8fa31e4a2aa43f0e1212659af72025-08-20T02:52:27ZengElsevierResults in Engineering2590-12302024-12-012410348610.1016/j.rineng.2024.103486Modelling key reactive processes relevant to bisulfide transport through highly compacted bentoniteMd Abdullah Asad0Tarek L. Rashwan1Ian L. Molnar2Mehran Behazin3Peter G. Keech4Magdalena M. Krol5Department of Civil Engineering, Lassonde School of Engineering, York University, Toronto, Ontario, M3J 1P3, CanadaDepartment of Engineering and Innovation, The Open University, Milton Keynes, MK76AA, United KingdomSchool of Geosciences, University of Edinburgh, Edinburgh, Scotland, EH8 8AQ, United KingdomNuclear Waste Management Organization, Toronto, Ontario, M4T 2S3, CanadaNuclear Waste Management Organization, Toronto, Ontario, M4T 2S3, CanadaDepartment of Civil Engineering, Lassonde School of Engineering, York University, Toronto, Ontario, M3J 1P3, Canada; Corresponding author.The Canadian deep geological repository (DGR) design consists of copper coated used fuel containers (UFCs) placed within a highly compacted bentonite (HCB) buffer surrounded by a suitable host rock. Although the copper is thermodynamically stable in oxygen-free environments, it is potentially susceptible to microbiologically influenced corrosion from bisulfide (HS-). Therefore, understanding HS- corrosion is important to ensure long-term performance of UFCs. Various reactions in the bentonite barrier of the DGR can affect HS- transport through the HCB and therefore the extent of copper corrosion caused by HS-. Since HS- transport and reactive processes are interconnected, numerical models are required to assess the complex HS- reactive transport dynamics and quantify the influence of reactive processes on HS- transport and corrosion. In this paper, various HS- transport models were coupled with (i) a key geochemical reaction between HS- and iron (i.e., simulating HS- retardation due to iron sulfide formation) or (ii) HS- adsorption. Since HS- is an anion, anion exclusion was also explored. Valuable insight was obtained through validation, comparison, and sensitivity analyses of these models. A comparison between experimental and modelled HS- transport dynamics showed that HS- is being retained by the bentonite due to reactive processes and anion exclusion is occurring. Lastly, HS- transport was simulated for the entire DGR lifespan and was found to be delayed (≈50–800 years) due to FeS formation or HS- adsorption. However, these predicted HS- diffusion delays are relatively short in a DGR lifespan (i.e., 1 million years) and do not impact long-term HS- corrosion.http://www.sciencedirect.com/science/article/pii/S2590123024017389Deep geological repositoryUsed nuclear fuelsNumerical modelsReactive processesBisulfide transportSorption
spellingShingle Md Abdullah Asad
Tarek L. Rashwan
Ian L. Molnar
Mehran Behazin
Peter G. Keech
Magdalena M. Krol
Modelling key reactive processes relevant to bisulfide transport through highly compacted bentonite
Results in Engineering
Deep geological repository
Used nuclear fuels
Numerical models
Reactive processes
Bisulfide transport
Sorption
title Modelling key reactive processes relevant to bisulfide transport through highly compacted bentonite
title_full Modelling key reactive processes relevant to bisulfide transport through highly compacted bentonite
title_fullStr Modelling key reactive processes relevant to bisulfide transport through highly compacted bentonite
title_full_unstemmed Modelling key reactive processes relevant to bisulfide transport through highly compacted bentonite
title_short Modelling key reactive processes relevant to bisulfide transport through highly compacted bentonite
title_sort modelling key reactive processes relevant to bisulfide transport through highly compacted bentonite
topic Deep geological repository
Used nuclear fuels
Numerical models
Reactive processes
Bisulfide transport
Sorption
url http://www.sciencedirect.com/science/article/pii/S2590123024017389
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