Influence of babassu fiber content on the chemical, physical and mechanical properties of polyhydroxybutyrate/babassu biocomposites

Polyhydroxybutyrate (PHB)/Babassu fiber biocomposites were developed via compression molding and subjected to extensive characterization. ATR-FTIR analysis indicated physical interactions between the components due to their chemical similarities. XRD patterns revealed minor structural disorganizatio...

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Main Authors: Camila Ferreira Gerardo, Laysa Silva Barboza, Ana Carolina Bastos Rodrigues, Beatriz Cruz Bastos, Pedro Henrique Poubel Mendonça da Silveira, Sergio Neves Monteiro, Shirleny Fontes Santos, Neyda de La Caridad Om Tapanes, Daniele Cruz Bastos
Format: Article
Language:English
Published: Elsevier 2025-05-01
Series:Journal of Materials Research and Technology
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Online Access:http://www.sciencedirect.com/science/article/pii/S223878542501141X
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Summary:Polyhydroxybutyrate (PHB)/Babassu fiber biocomposites were developed via compression molding and subjected to extensive characterization. ATR-FTIR analysis indicated physical interactions between the components due to their chemical similarities. XRD patterns revealed minor structural disorganization in the PHB/Babassu 85/15 and 80/20 formulations, with a slight decrease in crystallinity. SEM analysis demonstrated weak polymer-matrix adhesion in these samples, which may affect mechanical performance. The incorporation of babassu increased the water contact angle, enhancing hydrophobicity, particularly in the 90/10 and 80/20 formulations. Tensile tests showed that the PHB/Babassu 90/10 composite maintained mechanical properties comparable to pure PHB, while higher babassu content (20 %) led to decreased performance due to poor interfacial adhesion. Impact resistance was slightly improved in the 90/10 formulation, aligning with hardness results. Thermogravimetric analysis indicated that PHB primarily degrades between 250 and 310 °C, while PHB/Babassu composites exhibited an initial weight loss due to moisture release. Babassu had minimal influence on thermal stability; however, a 10 % filler content increased Tonset by approximately 10 °C, whereas higher concentrations showed negligible variation. The PHB/Babassu 90/10 composition stands out for its balance between mechanical strength and environmental sustainability, making it a promising candidate for biodegradable applications, such as packaging and agricultural films. Further studies should explore improved filler dispersion to enhance mechanical properties and broaden potential applications.
ISSN:2238-7854