Research on the Hierarchical Separation of Rare Earths and Lithium from Rare Earth Molten Salt Slag

Lithium is an important non-renewable resource, and the study of the tiered separation of rare earths and lithium from rare earth molten salt slag is an important approach to solving the current global resource shortage. This article adopts a sulfuric acid leaching process and a lithium-containing s...

Full description

Saved in:
Bibliographic Details
Main Authors: Hao Tang, Chunfa Liao, Fupeng Liu, Jiahui Mao, Zecheng Zhou, Yijian Zheng
Format: Article
Language:English
Published: MDPI AG 2024-11-01
Series:Metals
Subjects:
Online Access:https://www.mdpi.com/2075-4701/14/11/1247
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1850227060571635712
author Hao Tang
Chunfa Liao
Fupeng Liu
Jiahui Mao
Zecheng Zhou
Yijian Zheng
author_facet Hao Tang
Chunfa Liao
Fupeng Liu
Jiahui Mao
Zecheng Zhou
Yijian Zheng
author_sort Hao Tang
collection DOAJ
description Lithium is an important non-renewable resource, and the study of the tiered separation of rare earths and lithium from rare earth molten salt slag is an important approach to solving the current global resource shortage. This article adopts a sulfuric acid leaching process and a lithium-containing solution iron lithium extraction separation process to recover lithium from rare earth molten salt slag. The method systematically investigates the impact of sulfuric acid concentration, liquid-to-solid ratio, leaching temperature, leaching time, pH, P507 concentration, phase ratio, extraction temperature, and extraction time on the lithium extraction effect and iron lithium separation effect in rare earth molten salt slag. The results show that under the conditions of a sulfuric acid concentration of 0.9 mol/L, a liquid-to-solid ratio of 8:1 mL/g, a leaching temperature of 70 °C, a leaching time of 90 min, a pH of 0.9, a P507 concentration of 50%, a phase ratio of 5:3, an extraction temperature of 30 °C, and an extraction time of 20 min, the lithium leaching rate reaches 97.8%, and the separation of iron and lithium is fully achieved. This method can efficiently recover the valuable element lithium from rare earth molten salt slag, which is of great significance for the subsequent preparation of lithium products and the realization of a closed-loop production of rare earth alloys by molten salt electrolysis.
format Article
id doaj-art-a19d7d7ba0a0428e84df9458f49a4bd0
institution OA Journals
issn 2075-4701
language English
publishDate 2024-11-01
publisher MDPI AG
record_format Article
series Metals
spelling doaj-art-a19d7d7ba0a0428e84df9458f49a4bd02025-08-20T02:04:55ZengMDPI AGMetals2075-47012024-11-011411124710.3390/met14111247Research on the Hierarchical Separation of Rare Earths and Lithium from Rare Earth Molten Salt SlagHao Tang0Chunfa Liao1Fupeng Liu2Jiahui Mao3Zecheng Zhou4Yijian Zheng5School of Metallurgical Engineering, Jiangxi University of Science and Technology, Ganzhou 341000, ChinaSchool of Metallurgical Engineering, Jiangxi University of Science and Technology, Ganzhou 341000, ChinaSchool of Metallurgical Engineering, Jiangxi University of Science and Technology, Ganzhou 341000, ChinaSchool of Metallurgical Engineering, Jiangxi University of Science and Technology, Ganzhou 341000, ChinaSchool of Metallurgical Engineering, Jiangxi University of Science and Technology, Ganzhou 341000, ChinaSchool of Metallurgical Engineering, Jiangxi University of Science and Technology, Ganzhou 341000, ChinaLithium is an important non-renewable resource, and the study of the tiered separation of rare earths and lithium from rare earth molten salt slag is an important approach to solving the current global resource shortage. This article adopts a sulfuric acid leaching process and a lithium-containing solution iron lithium extraction separation process to recover lithium from rare earth molten salt slag. The method systematically investigates the impact of sulfuric acid concentration, liquid-to-solid ratio, leaching temperature, leaching time, pH, P507 concentration, phase ratio, extraction temperature, and extraction time on the lithium extraction effect and iron lithium separation effect in rare earth molten salt slag. The results show that under the conditions of a sulfuric acid concentration of 0.9 mol/L, a liquid-to-solid ratio of 8:1 mL/g, a leaching temperature of 70 °C, a leaching time of 90 min, a pH of 0.9, a P507 concentration of 50%, a phase ratio of 5:3, an extraction temperature of 30 °C, and an extraction time of 20 min, the lithium leaching rate reaches 97.8%, and the separation of iron and lithium is fully achieved. This method can efficiently recover the valuable element lithium from rare earth molten salt slag, which is of great significance for the subsequent preparation of lithium products and the realization of a closed-loop production of rare earth alloys by molten salt electrolysis.https://www.mdpi.com/2075-4701/14/11/1247rare earthmolten salt electrolysis slaghierarchical separationlithiumiron removal
spellingShingle Hao Tang
Chunfa Liao
Fupeng Liu
Jiahui Mao
Zecheng Zhou
Yijian Zheng
Research on the Hierarchical Separation of Rare Earths and Lithium from Rare Earth Molten Salt Slag
Metals
rare earth
molten salt electrolysis slag
hierarchical separation
lithium
iron removal
title Research on the Hierarchical Separation of Rare Earths and Lithium from Rare Earth Molten Salt Slag
title_full Research on the Hierarchical Separation of Rare Earths and Lithium from Rare Earth Molten Salt Slag
title_fullStr Research on the Hierarchical Separation of Rare Earths and Lithium from Rare Earth Molten Salt Slag
title_full_unstemmed Research on the Hierarchical Separation of Rare Earths and Lithium from Rare Earth Molten Salt Slag
title_short Research on the Hierarchical Separation of Rare Earths and Lithium from Rare Earth Molten Salt Slag
title_sort research on the hierarchical separation of rare earths and lithium from rare earth molten salt slag
topic rare earth
molten salt electrolysis slag
hierarchical separation
lithium
iron removal
url https://www.mdpi.com/2075-4701/14/11/1247
work_keys_str_mv AT haotang researchonthehierarchicalseparationofrareearthsandlithiumfromrareearthmoltensaltslag
AT chunfaliao researchonthehierarchicalseparationofrareearthsandlithiumfromrareearthmoltensaltslag
AT fupengliu researchonthehierarchicalseparationofrareearthsandlithiumfromrareearthmoltensaltslag
AT jiahuimao researchonthehierarchicalseparationofrareearthsandlithiumfromrareearthmoltensaltslag
AT zechengzhou researchonthehierarchicalseparationofrareearthsandlithiumfromrareearthmoltensaltslag
AT yijianzheng researchonthehierarchicalseparationofrareearthsandlithiumfromrareearthmoltensaltslag