Metal adsorption behavior of 2,4-dinitrophenyl hydrazine modified polyacrylonitrile nanofibers

Electrospun polyacrylonitrile nanofiber mats (es-PAN nanofiber mats) were surface modified by 2,4-dinitrophenyl-hydrazine (2,4-DNPH) to yield the metal ion adsorption material (es-PAN-DNPH nanofiber mats) and were investigated their adsorption behaviors. Functional modification of the es-PAN nanofib...

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Main Authors: S. Jitjaicham, P. Supaphol, P. Kampalanonwat
Format: Article
Language:English
Published: Budapest University of Technology and Economics 2013-10-01
Series:eXPRESS Polymer Letters
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Online Access:http://www.expresspolymlett.com/letolt.php?file=EPL-0004471&mi=cd
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author S. Jitjaicham
P. Supaphol
P. Kampalanonwat
author_facet S. Jitjaicham
P. Supaphol
P. Kampalanonwat
author_sort S. Jitjaicham
collection DOAJ
description Electrospun polyacrylonitrile nanofiber mats (es-PAN nanofiber mats) were surface modified by 2,4-dinitrophenyl-hydrazine (2,4-DNPH) to yield the metal ion adsorption material (es-PAN-DNPH nanofiber mats) and were investigated their adsorption behaviors. Functional modification of the es-PAN nanofiber mats and conventional polyacrylonitrile fibers (c-PAN fibers) were prepared by using 4% (w/v) of 2,4-DNPH in 1,2-ethandiol at 110°C for 6 h to obtained c-PAN-DNPH fibers. The average diameter of the es-PAN-DNPH nanofiber mats was 0.25 µm, which was comparatively smaller than the es-PAN precursor. Their functional groups were confirmed by Fourier transform infrared spectroscopy (FT-IR) and their adsorption behaviors to trace Ag(I), Bi(III), Ga(III), and In(III) from aqueous solutions and were investigated by the induced couple plasma technique. The FT-IR spectra showed the existence of NN=C–NHNH–, O=C–NHNH–, and –NO2 functional groups for metal complexes. The adsorption capacities of the obtained es-PAN-DNPH were 7.14 to 36.36% higher than those of c-PAN-DNPH fibers. All adsorption plots onto es-PAN-DNPH nanofiber mats and c-PANDNPH fibers followed the Langmuir isotherm and indicated monolayer adsorption characteristics.
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spelling doaj-art-a14d8a3364e3455fbe8d8b66f935e93d2025-08-20T03:35:51ZengBudapest University of Technology and EconomicseXPRESS Polymer Letters1788-618X2013-10-0171083284110.3144/expresspolymlett.2013.80Metal adsorption behavior of 2,4-dinitrophenyl hydrazine modified polyacrylonitrile nanofibersS. JitjaichamP. SupapholP. KampalanonwatElectrospun polyacrylonitrile nanofiber mats (es-PAN nanofiber mats) were surface modified by 2,4-dinitrophenyl-hydrazine (2,4-DNPH) to yield the metal ion adsorption material (es-PAN-DNPH nanofiber mats) and were investigated their adsorption behaviors. Functional modification of the es-PAN nanofiber mats and conventional polyacrylonitrile fibers (c-PAN fibers) were prepared by using 4% (w/v) of 2,4-DNPH in 1,2-ethandiol at 110°C for 6 h to obtained c-PAN-DNPH fibers. The average diameter of the es-PAN-DNPH nanofiber mats was 0.25 µm, which was comparatively smaller than the es-PAN precursor. Their functional groups were confirmed by Fourier transform infrared spectroscopy (FT-IR) and their adsorption behaviors to trace Ag(I), Bi(III), Ga(III), and In(III) from aqueous solutions and were investigated by the induced couple plasma technique. The FT-IR spectra showed the existence of NN=C–NHNH–, O=C–NHNH–, and –NO2 functional groups for metal complexes. The adsorption capacities of the obtained es-PAN-DNPH were 7.14 to 36.36% higher than those of c-PAN-DNPH fibers. All adsorption plots onto es-PAN-DNPH nanofiber mats and c-PANDNPH fibers followed the Langmuir isotherm and indicated monolayer adsorption characteristics.http://www.expresspolymlett.com/letolt.php?file=EPL-0004471&mi=cdNanomaterialselectrospinningpolyacrylonitrile
spellingShingle S. Jitjaicham
P. Supaphol
P. Kampalanonwat
Metal adsorption behavior of 2,4-dinitrophenyl hydrazine modified polyacrylonitrile nanofibers
eXPRESS Polymer Letters
Nanomaterials
electrospinning
polyacrylonitrile
title Metal adsorption behavior of 2,4-dinitrophenyl hydrazine modified polyacrylonitrile nanofibers
title_full Metal adsorption behavior of 2,4-dinitrophenyl hydrazine modified polyacrylonitrile nanofibers
title_fullStr Metal adsorption behavior of 2,4-dinitrophenyl hydrazine modified polyacrylonitrile nanofibers
title_full_unstemmed Metal adsorption behavior of 2,4-dinitrophenyl hydrazine modified polyacrylonitrile nanofibers
title_short Metal adsorption behavior of 2,4-dinitrophenyl hydrazine modified polyacrylonitrile nanofibers
title_sort metal adsorption behavior of 2 4 dinitrophenyl hydrazine modified polyacrylonitrile nanofibers
topic Nanomaterials
electrospinning
polyacrylonitrile
url http://www.expresspolymlett.com/letolt.php?file=EPL-0004471&mi=cd
work_keys_str_mv AT sjitjaicham metaladsorptionbehaviorof24dinitrophenylhydrazinemodifiedpolyacrylonitrilenanofibers
AT psupaphol metaladsorptionbehaviorof24dinitrophenylhydrazinemodifiedpolyacrylonitrilenanofibers
AT pkampalanonwat metaladsorptionbehaviorof24dinitrophenylhydrazinemodifiedpolyacrylonitrilenanofibers