Eu isotope fractionation and hydrothermal alteration

Abstract Europium (Eu) has two naturally stable isotopes (151Eu and 153Eu). The Eu anomalies produced by feldspar crystallization during magma differentiation have provided valuable geochemical information for understanding the evolutionary history of magma in the crust-mantle system. Recently, the...

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Main Authors: Seung-Gu Lee, ShuangShuang Chen, Tae Jong Lee, Hyeoncheol Kim, Seung Ryeol Lee, Sung Hi Choi, Ung San Ahn, Youn Soo Lee
Format: Article
Language:English
Published: Nature Portfolio 2025-08-01
Series:Scientific Reports
Online Access:https://doi.org/10.1038/s41598-025-14613-9
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author Seung-Gu Lee
ShuangShuang Chen
Tae Jong Lee
Hyeoncheol Kim
Seung Ryeol Lee
Sung Hi Choi
Ung San Ahn
Youn Soo Lee
author_facet Seung-Gu Lee
ShuangShuang Chen
Tae Jong Lee
Hyeoncheol Kim
Seung Ryeol Lee
Sung Hi Choi
Ung San Ahn
Youn Soo Lee
author_sort Seung-Gu Lee
collection DOAJ
description Abstract Europium (Eu) has two naturally stable isotopes (151Eu and 153Eu). The Eu anomalies produced by feldspar crystallization during magma differentiation have provided valuable geochemical information for understanding the evolutionary history of magma in the crust-mantle system. Recently, the correlation between the degree of Eu isotope fractionation (δ153Eu) and the magnitude of the Eu anomaly produced by magma differentiation has received much attention as a new research field for understanding the evolution of the Earth system1–4. Here, we report large variation of Eu isotope ratio for geochemically mafic volcanic rocks from the Korean Peninsula and Ocean Drilling Program (ODP) site 801 C, western Pacific Ocean. The Eu isotope ratio in this work was determined precisely via multicollector inductively coupled plasma mass spectrometry using a Sm internal standard5–7. We find that the δ153Eu values of hydrothermally altered alkaline mafic volcanic rocks vary from − 0.65‰ to -0.1‰, in contrast to the narrow range that characterizes the primary fresh subalkaline mafic volcanic rocks (from − 0.1‰ to 0.1‰). Our findings indicate that Eu isotope fractionation can occur through not only magmatic differentiation but also hydrothermal reactions in the Earth system.
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spelling doaj-art-a05cdcd20df9408891b1a9fa57b3da552025-08-20T04:01:51ZengNature PortfolioScientific Reports2045-23222025-08-011511910.1038/s41598-025-14613-9Eu isotope fractionation and hydrothermal alterationSeung-Gu Lee0ShuangShuang Chen1Tae Jong Lee2Hyeoncheol Kim3Seung Ryeol Lee4Sung Hi Choi5Ung San Ahn6Youn Soo Lee7Geological Survey Division, Korea Institute of Geoscience and Mineral ResourcesSchool of Earth Sciences and Engineering, Sun Yat-sen UniversityGeological Safety Division, Korea Institute of Geoscience and Mineral ResourcesGeological Survey Division, Korea Institute of Geoscience and Mineral ResourcesGeological Survey Division, Korea Institute of Geoscience and Mineral ResourcesDepartment of Geological Sciences, Chungnam National UniversityJeju Special Self-Governing Province, World Heritage OfficeDivision of Environmental Science and Engineering, Pohang University of Science and TechnologyAbstract Europium (Eu) has two naturally stable isotopes (151Eu and 153Eu). The Eu anomalies produced by feldspar crystallization during magma differentiation have provided valuable geochemical information for understanding the evolutionary history of magma in the crust-mantle system. Recently, the correlation between the degree of Eu isotope fractionation (δ153Eu) and the magnitude of the Eu anomaly produced by magma differentiation has received much attention as a new research field for understanding the evolution of the Earth system1–4. Here, we report large variation of Eu isotope ratio for geochemically mafic volcanic rocks from the Korean Peninsula and Ocean Drilling Program (ODP) site 801 C, western Pacific Ocean. The Eu isotope ratio in this work was determined precisely via multicollector inductively coupled plasma mass spectrometry using a Sm internal standard5–7. We find that the δ153Eu values of hydrothermally altered alkaline mafic volcanic rocks vary from − 0.65‰ to -0.1‰, in contrast to the narrow range that characterizes the primary fresh subalkaline mafic volcanic rocks (from − 0.1‰ to 0.1‰). Our findings indicate that Eu isotope fractionation can occur through not only magmatic differentiation but also hydrothermal reactions in the Earth system.https://doi.org/10.1038/s41598-025-14613-9
spellingShingle Seung-Gu Lee
ShuangShuang Chen
Tae Jong Lee
Hyeoncheol Kim
Seung Ryeol Lee
Sung Hi Choi
Ung San Ahn
Youn Soo Lee
Eu isotope fractionation and hydrothermal alteration
Scientific Reports
title Eu isotope fractionation and hydrothermal alteration
title_full Eu isotope fractionation and hydrothermal alteration
title_fullStr Eu isotope fractionation and hydrothermal alteration
title_full_unstemmed Eu isotope fractionation and hydrothermal alteration
title_short Eu isotope fractionation and hydrothermal alteration
title_sort eu isotope fractionation and hydrothermal alteration
url https://doi.org/10.1038/s41598-025-14613-9
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