Nonequilibrium Brownian motion beyond the effective temperature.

The condition of thermal equilibrium simplifies the theoretical treatment of fluctuations as found in the celebrated Einstein's relation between mobility and diffusivity for Brownian motion. Several recent theories relax the hypothesis of thermal equilibrium resulting in at least two main scena...

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Main Authors: Andrea Gnoli, Andrea Puglisi, Alessandro Sarracino, Angelo Vulpiani
Format: Article
Language:English
Published: Public Library of Science (PLoS) 2014-01-01
Series:PLoS ONE
Online Access:https://journals.plos.org/plosone/article/file?id=10.1371/journal.pone.0093720&type=printable
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author Andrea Gnoli
Andrea Puglisi
Alessandro Sarracino
Angelo Vulpiani
author_facet Andrea Gnoli
Andrea Puglisi
Alessandro Sarracino
Angelo Vulpiani
author_sort Andrea Gnoli
collection DOAJ
description The condition of thermal equilibrium simplifies the theoretical treatment of fluctuations as found in the celebrated Einstein's relation between mobility and diffusivity for Brownian motion. Several recent theories relax the hypothesis of thermal equilibrium resulting in at least two main scenarios. With well separated timescales, as in aging glassy systems, equilibrium Fluctuation-Dissipation Theorem applies at each scale with its own "effective" temperature. With mixed timescales, as for example in active or granular fluids or in turbulence, temperature is no more well-defined, the dynamical nature of fluctuations fully emerges and a Generalized Fluctuation-Dissipation Theorem (GFDT) applies. Here, we study experimentally the mixed timescale regime by studying fluctuations and linear response in the Brownian motion of a rotating intruder immersed in a vibro-fluidized granular medium. Increasing the packing fraction, the system is moved from a dilute single-timescale regime toward a denser multiple-timescale stage. Einstein's relation holds in the former and is violated in the latter. The violation cannot be explained in terms of effective temperatures, while the GFDT is able to impute it to the emergence of a strong coupling between the intruder and the surrounding fluid. Direct experimental measurements confirm the development of spatial correlations in the system when the density is increased.
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spelling doaj-art-a01f3aa6d28c4867a7eb18d8c2212a4c2025-08-20T02:14:42ZengPublic Library of Science (PLoS)PLoS ONE1932-62032014-01-0194e9372010.1371/journal.pone.0093720Nonequilibrium Brownian motion beyond the effective temperature.Andrea GnoliAndrea PuglisiAlessandro SarracinoAngelo VulpianiThe condition of thermal equilibrium simplifies the theoretical treatment of fluctuations as found in the celebrated Einstein's relation between mobility and diffusivity for Brownian motion. Several recent theories relax the hypothesis of thermal equilibrium resulting in at least two main scenarios. With well separated timescales, as in aging glassy systems, equilibrium Fluctuation-Dissipation Theorem applies at each scale with its own "effective" temperature. With mixed timescales, as for example in active or granular fluids or in turbulence, temperature is no more well-defined, the dynamical nature of fluctuations fully emerges and a Generalized Fluctuation-Dissipation Theorem (GFDT) applies. Here, we study experimentally the mixed timescale regime by studying fluctuations and linear response in the Brownian motion of a rotating intruder immersed in a vibro-fluidized granular medium. Increasing the packing fraction, the system is moved from a dilute single-timescale regime toward a denser multiple-timescale stage. Einstein's relation holds in the former and is violated in the latter. The violation cannot be explained in terms of effective temperatures, while the GFDT is able to impute it to the emergence of a strong coupling between the intruder and the surrounding fluid. Direct experimental measurements confirm the development of spatial correlations in the system when the density is increased.https://journals.plos.org/plosone/article/file?id=10.1371/journal.pone.0093720&type=printable
spellingShingle Andrea Gnoli
Andrea Puglisi
Alessandro Sarracino
Angelo Vulpiani
Nonequilibrium Brownian motion beyond the effective temperature.
PLoS ONE
title Nonequilibrium Brownian motion beyond the effective temperature.
title_full Nonequilibrium Brownian motion beyond the effective temperature.
title_fullStr Nonequilibrium Brownian motion beyond the effective temperature.
title_full_unstemmed Nonequilibrium Brownian motion beyond the effective temperature.
title_short Nonequilibrium Brownian motion beyond the effective temperature.
title_sort nonequilibrium brownian motion beyond the effective temperature
url https://journals.plos.org/plosone/article/file?id=10.1371/journal.pone.0093720&type=printable
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