Modulating Ru-Co bond lengths in Ru1Co single-atom alloys through crystal phase engineering for electrocatalytic nitrate-to-ammonia conversion

Abstract Single atom alloys (SAAs) with maximum atomic efficiency and uniform active sites show great promise for heterogeneous catalytic applications. Meanwhile, crystal phase engineering has granered significant interest due to tailored atomic arrangements and coordination environments. However, t...

Full description

Saved in:
Bibliographic Details
Main Authors: Xiaojuan Zhu, Yi-Chi Wang, Kaiyu Qu, Leyang Song, Jing Wang, Yushuang Gong, Xiang Liu, Cheng-Fei Li, Shiling Yuan, Qipeng Lu, An-Liang Wang
Format: Article
Language:English
Published: Nature Portfolio 2025-07-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-025-61232-z
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1849238473881419776
author Xiaojuan Zhu
Yi-Chi Wang
Kaiyu Qu
Leyang Song
Jing Wang
Yushuang Gong
Xiang Liu
Cheng-Fei Li
Shiling Yuan
Qipeng Lu
An-Liang Wang
author_facet Xiaojuan Zhu
Yi-Chi Wang
Kaiyu Qu
Leyang Song
Jing Wang
Yushuang Gong
Xiang Liu
Cheng-Fei Li
Shiling Yuan
Qipeng Lu
An-Liang Wang
author_sort Xiaojuan Zhu
collection DOAJ
description Abstract Single atom alloys (SAAs) with maximum atomic efficiency and uniform active sites show great promise for heterogeneous catalytic applications. Meanwhile, crystal phase engineering has granered significant interest due to tailored atomic arrangements and coordination environments. However, the crystal phase engineering of SAAs remains challenging owing to high surface energy and complex phase transition dynamics. Herein, Ru1Co SAAs with tunable crystal phases (hexagonal-close-packed (hcp), face-centered-cubic (fcc), and hcp/fcc structure) are successfully synthesized via controlled phase transitions. These SAAs exhibit distinct crystal phase-dependent performance towards nitrate reduction reaction (NO3RR), where hcp-Ru1Co outperforms its counterparts with a NH3 Faradaic efficiency of 96.78% at 0 V vs. reversible hydrogen electrode and long-term stability exceeding 1200 h. Mechanistic investigations reveal that the hcp configurations enables shorter Ru-Co distances, stronger interatomic interactions, and more positive surface potential compared to hcp/fcc-Ru1Co and fcc-Ru1Co, which enhances the NO3 − adsorption, reduces the free energy barrier, and suppresses competitive hydrogen evolution.
format Article
id doaj-art-9deb4ea8968846c8a01164caf39bc2ff
institution Kabale University
issn 2041-1723
language English
publishDate 2025-07-01
publisher Nature Portfolio
record_format Article
series Nature Communications
spelling doaj-art-9deb4ea8968846c8a01164caf39bc2ff2025-08-20T04:01:35ZengNature PortfolioNature Communications2041-17232025-07-0116111410.1038/s41467-025-61232-zModulating Ru-Co bond lengths in Ru1Co single-atom alloys through crystal phase engineering for electrocatalytic nitrate-to-ammonia conversionXiaojuan Zhu0Yi-Chi Wang1Kaiyu Qu2Leyang Song3Jing Wang4Yushuang Gong5Xiang Liu6Cheng-Fei Li7Shiling Yuan8Qipeng Lu9An-Liang Wang10Key Laboratory for Colloid and Interface Chemistry, Ministry of Education, School of Chemistry and Chemical Engineering, Shandong UniversityBeijing National Center for Electron Microscopy and Laboratory of Advanced Materials, School of Materials Science and Engineering, Tsinghua UniversityKey Laboratory for Colloid and Interface Chemistry, Ministry of Education, School of Chemistry and Chemical Engineering, Shandong UniversityKey Laboratory for Colloid and Interface Chemistry, Ministry of Education, School of Chemistry and Chemical Engineering, Shandong UniversityKey Laboratory for Colloid and Interface Chemistry, Ministry of Education, School of Chemistry and Chemical Engineering, Shandong UniversityKey Laboratory for Colloid and Interface Chemistry, Ministry of Education, School of Chemistry and Chemical Engineering, Shandong UniversityKey Laboratory for Colloid and Interface Chemistry, Ministry of Education, School of Chemistry and Chemical Engineering, Shandong UniversityNational Energy Key Laboratory for New Hydrogen-Ammonia Energy Technologies, Foshan Xianhu LaboratoryKey Laboratory for Colloid and Interface Chemistry, Ministry of Education, School of Chemistry and Chemical Engineering, Shandong UniversitySchool of Materials Science and Engineering, University of Science and Technology BeijingKey Laboratory for Colloid and Interface Chemistry, Ministry of Education, School of Chemistry and Chemical Engineering, Shandong UniversityAbstract Single atom alloys (SAAs) with maximum atomic efficiency and uniform active sites show great promise for heterogeneous catalytic applications. Meanwhile, crystal phase engineering has granered significant interest due to tailored atomic arrangements and coordination environments. However, the crystal phase engineering of SAAs remains challenging owing to high surface energy and complex phase transition dynamics. Herein, Ru1Co SAAs with tunable crystal phases (hexagonal-close-packed (hcp), face-centered-cubic (fcc), and hcp/fcc structure) are successfully synthesized via controlled phase transitions. These SAAs exhibit distinct crystal phase-dependent performance towards nitrate reduction reaction (NO3RR), where hcp-Ru1Co outperforms its counterparts with a NH3 Faradaic efficiency of 96.78% at 0 V vs. reversible hydrogen electrode and long-term stability exceeding 1200 h. Mechanistic investigations reveal that the hcp configurations enables shorter Ru-Co distances, stronger interatomic interactions, and more positive surface potential compared to hcp/fcc-Ru1Co and fcc-Ru1Co, which enhances the NO3 − adsorption, reduces the free energy barrier, and suppresses competitive hydrogen evolution.https://doi.org/10.1038/s41467-025-61232-z
spellingShingle Xiaojuan Zhu
Yi-Chi Wang
Kaiyu Qu
Leyang Song
Jing Wang
Yushuang Gong
Xiang Liu
Cheng-Fei Li
Shiling Yuan
Qipeng Lu
An-Liang Wang
Modulating Ru-Co bond lengths in Ru1Co single-atom alloys through crystal phase engineering for electrocatalytic nitrate-to-ammonia conversion
Nature Communications
title Modulating Ru-Co bond lengths in Ru1Co single-atom alloys through crystal phase engineering for electrocatalytic nitrate-to-ammonia conversion
title_full Modulating Ru-Co bond lengths in Ru1Co single-atom alloys through crystal phase engineering for electrocatalytic nitrate-to-ammonia conversion
title_fullStr Modulating Ru-Co bond lengths in Ru1Co single-atom alloys through crystal phase engineering for electrocatalytic nitrate-to-ammonia conversion
title_full_unstemmed Modulating Ru-Co bond lengths in Ru1Co single-atom alloys through crystal phase engineering for electrocatalytic nitrate-to-ammonia conversion
title_short Modulating Ru-Co bond lengths in Ru1Co single-atom alloys through crystal phase engineering for electrocatalytic nitrate-to-ammonia conversion
title_sort modulating ru co bond lengths in ru1co single atom alloys through crystal phase engineering for electrocatalytic nitrate to ammonia conversion
url https://doi.org/10.1038/s41467-025-61232-z
work_keys_str_mv AT xiaojuanzhu modulatingrucobondlengthsinru1cosingleatomalloysthroughcrystalphaseengineeringforelectrocatalyticnitratetoammoniaconversion
AT yichiwang modulatingrucobondlengthsinru1cosingleatomalloysthroughcrystalphaseengineeringforelectrocatalyticnitratetoammoniaconversion
AT kaiyuqu modulatingrucobondlengthsinru1cosingleatomalloysthroughcrystalphaseengineeringforelectrocatalyticnitratetoammoniaconversion
AT leyangsong modulatingrucobondlengthsinru1cosingleatomalloysthroughcrystalphaseengineeringforelectrocatalyticnitratetoammoniaconversion
AT jingwang modulatingrucobondlengthsinru1cosingleatomalloysthroughcrystalphaseengineeringforelectrocatalyticnitratetoammoniaconversion
AT yushuanggong modulatingrucobondlengthsinru1cosingleatomalloysthroughcrystalphaseengineeringforelectrocatalyticnitratetoammoniaconversion
AT xiangliu modulatingrucobondlengthsinru1cosingleatomalloysthroughcrystalphaseengineeringforelectrocatalyticnitratetoammoniaconversion
AT chengfeili modulatingrucobondlengthsinru1cosingleatomalloysthroughcrystalphaseengineeringforelectrocatalyticnitratetoammoniaconversion
AT shilingyuan modulatingrucobondlengthsinru1cosingleatomalloysthroughcrystalphaseengineeringforelectrocatalyticnitratetoammoniaconversion
AT qipenglu modulatingrucobondlengthsinru1cosingleatomalloysthroughcrystalphaseengineeringforelectrocatalyticnitratetoammoniaconversion
AT anliangwang modulatingrucobondlengthsinru1cosingleatomalloysthroughcrystalphaseengineeringforelectrocatalyticnitratetoammoniaconversion