Simulated Experiment Study of Factors Influencing the Hydration Activity of f-CaO in Basic Oxygen Furnace Slag

The compositions and formation process of f-CaO in BOF slag were revealed and simulated to understand its expansion rules and why its hydration activity is low. BSE showed the compositions of f-CaO, which included calcium iron phase and calcium iron manganese phase, were diverse. The hydration activ...

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Main Authors: Ruiquan Jia, Jiaxiang Liu
Format: Article
Language:English
Published: Wiley 2016-01-01
Series:Advances in Materials Science and Engineering
Online Access:http://dx.doi.org/10.1155/2016/7529382
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author Ruiquan Jia
Jiaxiang Liu
author_facet Ruiquan Jia
Jiaxiang Liu
author_sort Ruiquan Jia
collection DOAJ
description The compositions and formation process of f-CaO in BOF slag were revealed and simulated to understand its expansion rules and why its hydration activity is low. BSE showed the compositions of f-CaO, which included calcium iron phase and calcium iron manganese phase, were diverse. The hydration activity sequence was Ca2Fe2O5 and Ca3Fe1.5Mn1.5O8 in tricomponent f-CaO < CaO in tricomponent f-CaO < monocomponent f-CaO; only Ca2Fe2O5 and Ca3Fe1.5Mn1.5O8 were hard to hydrate, and the volume expansion rates of the tricomponent f-CaO varied with different compositions. Inductively, in BOF slag, the hydration activity sequence was solid solutions CaO-FeOx and CaO-FeOx-MnOy in tricomponent f-CaO < CaO in tricomponent f-CaO < monocomponent f-CaO; the volume expansion rates of tricomponent f-CaO changed with different compositions, and CaO-FeOx and CaO-FeOx-MnOy were difficult to hydrate. The reason why solid solutions CaO-FeOx and CaO-FeOx-MnOy were hard to hydrate was that their hydration reaction driving force, which is the absolute value of standard molar reaction Gibbs functions, decreased.
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spelling doaj-art-9c9e52ece2b146e0a191bdeaa48ec6b52025-08-20T02:18:28ZengWileyAdvances in Materials Science and Engineering1687-84341687-84422016-01-01201610.1155/2016/75293827529382Simulated Experiment Study of Factors Influencing the Hydration Activity of f-CaO in Basic Oxygen Furnace SlagRuiquan Jia0Jiaxiang Liu1Beijing Key Laboratory of Electrochemical Process and Technology for Materials, Beijing University of Chemical Technology, Beijing 100029, ChinaBeijing Key Laboratory of Electrochemical Process and Technology for Materials, Beijing University of Chemical Technology, Beijing 100029, ChinaThe compositions and formation process of f-CaO in BOF slag were revealed and simulated to understand its expansion rules and why its hydration activity is low. BSE showed the compositions of f-CaO, which included calcium iron phase and calcium iron manganese phase, were diverse. The hydration activity sequence was Ca2Fe2O5 and Ca3Fe1.5Mn1.5O8 in tricomponent f-CaO < CaO in tricomponent f-CaO < monocomponent f-CaO; only Ca2Fe2O5 and Ca3Fe1.5Mn1.5O8 were hard to hydrate, and the volume expansion rates of the tricomponent f-CaO varied with different compositions. Inductively, in BOF slag, the hydration activity sequence was solid solutions CaO-FeOx and CaO-FeOx-MnOy in tricomponent f-CaO < CaO in tricomponent f-CaO < monocomponent f-CaO; the volume expansion rates of tricomponent f-CaO changed with different compositions, and CaO-FeOx and CaO-FeOx-MnOy were difficult to hydrate. The reason why solid solutions CaO-FeOx and CaO-FeOx-MnOy were hard to hydrate was that their hydration reaction driving force, which is the absolute value of standard molar reaction Gibbs functions, decreased.http://dx.doi.org/10.1155/2016/7529382
spellingShingle Ruiquan Jia
Jiaxiang Liu
Simulated Experiment Study of Factors Influencing the Hydration Activity of f-CaO in Basic Oxygen Furnace Slag
Advances in Materials Science and Engineering
title Simulated Experiment Study of Factors Influencing the Hydration Activity of f-CaO in Basic Oxygen Furnace Slag
title_full Simulated Experiment Study of Factors Influencing the Hydration Activity of f-CaO in Basic Oxygen Furnace Slag
title_fullStr Simulated Experiment Study of Factors Influencing the Hydration Activity of f-CaO in Basic Oxygen Furnace Slag
title_full_unstemmed Simulated Experiment Study of Factors Influencing the Hydration Activity of f-CaO in Basic Oxygen Furnace Slag
title_short Simulated Experiment Study of Factors Influencing the Hydration Activity of f-CaO in Basic Oxygen Furnace Slag
title_sort simulated experiment study of factors influencing the hydration activity of f cao in basic oxygen furnace slag
url http://dx.doi.org/10.1155/2016/7529382
work_keys_str_mv AT ruiquanjia simulatedexperimentstudyoffactorsinfluencingthehydrationactivityoffcaoinbasicoxygenfurnaceslag
AT jiaxiangliu simulatedexperimentstudyoffactorsinfluencingthehydrationactivityoffcaoinbasicoxygenfurnaceslag