Controllable Synthesis of Three-Dimensional Chiral Au Nanoflowers Induced by Cysteine with Excellent Biocompatible Properties

Chiral molecules are ubiquitous in nature and biological systems, where the unique optical and physical properties of chiral nanoparticles are closely linked to their shapes. Synthesizing chiral plasmonic nanomaterials with precise structures and tunable sizes is essential for exploring their applic...

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Main Authors: Shengmiao Liu, Jianhao Zhang, Wenjing Yan
Format: Article
Language:English
Published: MDPI AG 2024-12-01
Series:Nanomaterials
Subjects:
Online Access:https://www.mdpi.com/2079-4991/14/24/2040
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author Shengmiao Liu
Jianhao Zhang
Wenjing Yan
author_facet Shengmiao Liu
Jianhao Zhang
Wenjing Yan
author_sort Shengmiao Liu
collection DOAJ
description Chiral molecules are ubiquitous in nature and biological systems, where the unique optical and physical properties of chiral nanoparticles are closely linked to their shapes. Synthesizing chiral plasmonic nanomaterials with precise structures and tunable sizes is essential for exploring their applications. This study presents a method for growing three-dimensional chiral gold nanoflowers (Au NFs) derived from trisoctahedral (TOH) nanocrystals using D-cysteine and L-cysteine as chiral inducers. By employing a two-step seed-mediated growth approach, stable chiral Au nanoparticles with customizable sizes, shapes, and optical properties were produced by adjusting the Au nanosphere (Au NP) seed concentration and cysteine dosage. These nanoparticles exhibited optical activity in both the visible and near-infrared regions, with a maximum anisotropy factor (<i>g</i>-factor) of 0.024. Furthermore, the PEG-modified chiral Au NFs demonstrated excellent biocompatibility. This approach provides a precise method for geometrically controlling the design of three-dimensional chiral nanomaterials, holding great potential for biomedical applications.
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institution Kabale University
issn 2079-4991
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publishDate 2024-12-01
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series Nanomaterials
spelling doaj-art-9bc7469ca3cb470482d87ca93405b99a2024-12-27T14:43:34ZengMDPI AGNanomaterials2079-49912024-12-011424204010.3390/nano14242040Controllable Synthesis of Three-Dimensional Chiral Au Nanoflowers Induced by Cysteine with Excellent Biocompatible PropertiesShengmiao Liu0Jianhao Zhang1Wenjing Yan2College of Food Science and Technology, Nanjing Agricultural University, Nanjing 210095, ChinaCollege of Food Science and Technology, Nanjing Agricultural University, Nanjing 210095, ChinaCollege of Food Science and Technology, Nanjing Agricultural University, Nanjing 210095, ChinaChiral molecules are ubiquitous in nature and biological systems, where the unique optical and physical properties of chiral nanoparticles are closely linked to their shapes. Synthesizing chiral plasmonic nanomaterials with precise structures and tunable sizes is essential for exploring their applications. This study presents a method for growing three-dimensional chiral gold nanoflowers (Au NFs) derived from trisoctahedral (TOH) nanocrystals using D-cysteine and L-cysteine as chiral inducers. By employing a two-step seed-mediated growth approach, stable chiral Au nanoparticles with customizable sizes, shapes, and optical properties were produced by adjusting the Au nanosphere (Au NP) seed concentration and cysteine dosage. These nanoparticles exhibited optical activity in both the visible and near-infrared regions, with a maximum anisotropy factor (<i>g</i>-factor) of 0.024. Furthermore, the PEG-modified chiral Au NFs demonstrated excellent biocompatibility. This approach provides a precise method for geometrically controlling the design of three-dimensional chiral nanomaterials, holding great potential for biomedical applications.https://www.mdpi.com/2079-4991/14/24/2040chiral nanomaterialscysteine<i>g</i>-factoroptical propertiesbiocompatibility
spellingShingle Shengmiao Liu
Jianhao Zhang
Wenjing Yan
Controllable Synthesis of Three-Dimensional Chiral Au Nanoflowers Induced by Cysteine with Excellent Biocompatible Properties
Nanomaterials
chiral nanomaterials
cysteine
<i>g</i>-factor
optical properties
biocompatibility
title Controllable Synthesis of Three-Dimensional Chiral Au Nanoflowers Induced by Cysteine with Excellent Biocompatible Properties
title_full Controllable Synthesis of Three-Dimensional Chiral Au Nanoflowers Induced by Cysteine with Excellent Biocompatible Properties
title_fullStr Controllable Synthesis of Three-Dimensional Chiral Au Nanoflowers Induced by Cysteine with Excellent Biocompatible Properties
title_full_unstemmed Controllable Synthesis of Three-Dimensional Chiral Au Nanoflowers Induced by Cysteine with Excellent Biocompatible Properties
title_short Controllable Synthesis of Three-Dimensional Chiral Au Nanoflowers Induced by Cysteine with Excellent Biocompatible Properties
title_sort controllable synthesis of three dimensional chiral au nanoflowers induced by cysteine with excellent biocompatible properties
topic chiral nanomaterials
cysteine
<i>g</i>-factor
optical properties
biocompatibility
url https://www.mdpi.com/2079-4991/14/24/2040
work_keys_str_mv AT shengmiaoliu controllablesynthesisofthreedimensionalchiralaunanoflowersinducedbycysteinewithexcellentbiocompatibleproperties
AT jianhaozhang controllablesynthesisofthreedimensionalchiralaunanoflowersinducedbycysteinewithexcellentbiocompatibleproperties
AT wenjingyan controllablesynthesisofthreedimensionalchiralaunanoflowersinducedbycysteinewithexcellentbiocompatibleproperties