Application of the Cellular Thermal Shift Assay (CETSA) to validate drug target engagement in platelets

Small molecule drugs play a major role in the study of human platelets. Effective action of a drug requires it to bind to one or more targets within the platelet (target engagement). However, although in vitro assays with isolated proteins can be used to determine drug affinity to these targets, add...

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Main Authors: Joanna-Marie Howes, Matthew T. Harper
Format: Article
Language:English
Published: Taylor & Francis Group 2024-12-01
Series:Platelets
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Online Access:https://www.tandfonline.com/doi/10.1080/09537104.2024.2354833
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author Joanna-Marie Howes
Matthew T. Harper
author_facet Joanna-Marie Howes
Matthew T. Harper
author_sort Joanna-Marie Howes
collection DOAJ
description Small molecule drugs play a major role in the study of human platelets. Effective action of a drug requires it to bind to one or more targets within the platelet (target engagement). However, although in vitro assays with isolated proteins can be used to determine drug affinity to these targets, additional factors affect target engagement and its consequences in an intact platelet, including plasma membrane permeability, intracellular metabolism or compartmentalization, and level of target expression. Mechanistic interpretation of the effect of drugs on platelet activity requires comprehensive investigation of drug binding in the proper cellular context, i.e. in intact platelets. The Cellular Thermal Shift Assay (CETSA) is a valuable method to investigate target engagement within complex cellular environments. The assay is based on the principle that drug binding to a target protein increases that protein’s thermal stability. In this technical report, we describe the application of CETSA to platelets. We highlight CETSA as a quick and informative technique for confirming the direct binding of drugs to platelet protein targets, providing a platform for understanding the mechanism of action of drugs in platelets, and which will be a valuable tool for investigating platelet signaling and function.
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spelling doaj-art-9aade0f0cb9a4384bad97a096502b8f72025-08-20T02:12:19ZengTaylor & Francis GroupPlatelets0953-71041369-16352024-12-0135110.1080/09537104.2024.2354833Application of the Cellular Thermal Shift Assay (CETSA) to validate drug target engagement in plateletsJoanna-Marie Howes0Matthew T. Harper1Department of Pharmacology, University of Cambridge, Cambridge, UKDepartment of Pharmacology, University of Cambridge, Cambridge, UKSmall molecule drugs play a major role in the study of human platelets. Effective action of a drug requires it to bind to one or more targets within the platelet (target engagement). However, although in vitro assays with isolated proteins can be used to determine drug affinity to these targets, additional factors affect target engagement and its consequences in an intact platelet, including plasma membrane permeability, intracellular metabolism or compartmentalization, and level of target expression. Mechanistic interpretation of the effect of drugs on platelet activity requires comprehensive investigation of drug binding in the proper cellular context, i.e. in intact platelets. The Cellular Thermal Shift Assay (CETSA) is a valuable method to investigate target engagement within complex cellular environments. The assay is based on the principle that drug binding to a target protein increases that protein’s thermal stability. In this technical report, we describe the application of CETSA to platelets. We highlight CETSA as a quick and informative technique for confirming the direct binding of drugs to platelet protein targets, providing a platform for understanding the mechanism of action of drugs in platelets, and which will be a valuable tool for investigating platelet signaling and function.https://www.tandfonline.com/doi/10.1080/09537104.2024.2354833CETSAdrug bindingplateletsthermal stability
spellingShingle Joanna-Marie Howes
Matthew T. Harper
Application of the Cellular Thermal Shift Assay (CETSA) to validate drug target engagement in platelets
Platelets
CETSA
drug binding
platelets
thermal stability
title Application of the Cellular Thermal Shift Assay (CETSA) to validate drug target engagement in platelets
title_full Application of the Cellular Thermal Shift Assay (CETSA) to validate drug target engagement in platelets
title_fullStr Application of the Cellular Thermal Shift Assay (CETSA) to validate drug target engagement in platelets
title_full_unstemmed Application of the Cellular Thermal Shift Assay (CETSA) to validate drug target engagement in platelets
title_short Application of the Cellular Thermal Shift Assay (CETSA) to validate drug target engagement in platelets
title_sort application of the cellular thermal shift assay cetsa to validate drug target engagement in platelets
topic CETSA
drug binding
platelets
thermal stability
url https://www.tandfonline.com/doi/10.1080/09537104.2024.2354833
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