The glass transition in molecules, colloids and grains: universality and specificity

We highlight certain key achievements in experimental work on molecular, colloidal and granular glassformers. This short review considers these three classes of experimental systems and focusses largely on the work of the authors and their coworkers and thus is far from exhaustive. Our goal is rathe...

Full description

Saved in:
Bibliographic Details
Main Authors: Dauchot, Olivier, Ladieu, François, Royall, C. Patrick
Format: Article
Language:English
Published: Académie des sciences 2023-08-01
Series:Comptes Rendus. Physique
Subjects:
Online Access:https://comptes-rendus.academie-sciences.fr/physique/articles/10.5802/crphys.155/
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1825205790372265984
author Dauchot, Olivier
Ladieu, François
Royall, C. Patrick
author_facet Dauchot, Olivier
Ladieu, François
Royall, C. Patrick
author_sort Dauchot, Olivier
collection DOAJ
description We highlight certain key achievements in experimental work on molecular, colloidal and granular glassformers. This short review considers these three classes of experimental systems and focusses largely on the work of the authors and their coworkers and thus is far from exhaustive. Our goal is rather to discuss particular experimental results from these classes and to explore universality and specificity across the broad range of length– and time–scales they span. We emphasize that a variety of phenomena, not least dynamical heterogeneity, growing lengthscales and a change in structure, albeit subtle, are now well established in these three classes of glassformer. We then review some experimental measurements which depend more specifically on the class of glassformer, such as the Gardner transition and some which have been investigated more in one or two classes than in all, such as configurational entropy and evidence for a dynamical phase transition. We finally put forward some open questions and consider what could be done to fill some of the gaps between theoretical approaches and experiments.
format Article
id doaj-art-9a9912f955b44c2188488f8912066c67
institution Kabale University
issn 1878-1535
language English
publishDate 2023-08-01
publisher Académie des sciences
record_format Article
series Comptes Rendus. Physique
spelling doaj-art-9a9912f955b44c2188488f8912066c672025-02-07T13:52:26ZengAcadémie des sciencesComptes Rendus. Physique1878-15352023-08-0124S1255610.5802/crphys.15510.5802/crphys.155The glass transition in molecules, colloids and grains: universality and specificityDauchot, Olivier0Ladieu, François1Royall, C. Patrick2Gulliver UMR CNRS 7083, ESPCI Paris, PSL Research University, 10 rue Vauquelin, 75005 Paris, FranceSPEC, CEA, CNRS, Universit’e Paris-Saclay, CEA Saclay Bat 772, F-91191 Gif-sur-Yvette Cedex, FranceGulliver UMR CNRS 7083, ESPCI Paris, PSL Research University, 10 rue Vauquelin, 75005 Paris, FranceWe highlight certain key achievements in experimental work on molecular, colloidal and granular glassformers. This short review considers these three classes of experimental systems and focusses largely on the work of the authors and their coworkers and thus is far from exhaustive. Our goal is rather to discuss particular experimental results from these classes and to explore universality and specificity across the broad range of length– and time–scales they span. We emphasize that a variety of phenomena, not least dynamical heterogeneity, growing lengthscales and a change in structure, albeit subtle, are now well established in these three classes of glassformer. We then review some experimental measurements which depend more specifically on the class of glassformer, such as the Gardner transition and some which have been investigated more in one or two classes than in all, such as configurational entropy and evidence for a dynamical phase transition. We finally put forward some open questions and consider what could be done to fill some of the gaps between theoretical approaches and experiments.https://comptes-rendus.academie-sciences.fr/physique/articles/10.5802/crphys.155/GlassesCorrelationsColloidal Glass TransitionGranular Glass TransitionStructural Glass TransitionDynamical Heterogeneities
spellingShingle Dauchot, Olivier
Ladieu, François
Royall, C. Patrick
The glass transition in molecules, colloids and grains: universality and specificity
Comptes Rendus. Physique
Glasses
Correlations
Colloidal Glass Transition
Granular Glass Transition
Structural Glass Transition
Dynamical Heterogeneities
title The glass transition in molecules, colloids and grains: universality and specificity
title_full The glass transition in molecules, colloids and grains: universality and specificity
title_fullStr The glass transition in molecules, colloids and grains: universality and specificity
title_full_unstemmed The glass transition in molecules, colloids and grains: universality and specificity
title_short The glass transition in molecules, colloids and grains: universality and specificity
title_sort glass transition in molecules colloids and grains universality and specificity
topic Glasses
Correlations
Colloidal Glass Transition
Granular Glass Transition
Structural Glass Transition
Dynamical Heterogeneities
url https://comptes-rendus.academie-sciences.fr/physique/articles/10.5802/crphys.155/
work_keys_str_mv AT dauchotolivier theglasstransitioninmoleculescolloidsandgrainsuniversalityandspecificity
AT ladieufrancois theglasstransitioninmoleculescolloidsandgrainsuniversalityandspecificity
AT royallcpatrick theglasstransitioninmoleculescolloidsandgrainsuniversalityandspecificity
AT dauchotolivier glasstransitioninmoleculescolloidsandgrainsuniversalityandspecificity
AT ladieufrancois glasstransitioninmoleculescolloidsandgrainsuniversalityandspecificity
AT royallcpatrick glasstransitioninmoleculescolloidsandgrainsuniversalityandspecificity