Soil Mercury Pollution in Nature-Based Solutions Across Various Land Uses: A Review of Trends, Treatment Outcomes, and Future Directions

Mercury (Hg) contamination in soils poses significant environmental risks. In response, various nature-based solutions (NbSs) have been developed and studied in the past to treat mercury along with other heavy metals from both point and nonpoint sources. However, various land uses present uncertaint...

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Main Authors: Miguel Enrico Robles, Yugyeong Oh, Md Tashdedul Haque, Minsu Jeon, Lee-Hyung Kim
Format: Article
Language:English
Published: MDPI AG 2025-06-01
Series:Applied Sciences
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Online Access:https://www.mdpi.com/2076-3417/15/12/6502
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author Miguel Enrico Robles
Yugyeong Oh
Md Tashdedul Haque
Minsu Jeon
Lee-Hyung Kim
author_facet Miguel Enrico Robles
Yugyeong Oh
Md Tashdedul Haque
Minsu Jeon
Lee-Hyung Kim
author_sort Miguel Enrico Robles
collection DOAJ
description Mercury (Hg) contamination in soils poses significant environmental risks. In response, various nature-based solutions (NbSs) have been developed and studied in the past to treat mercury along with other heavy metals from both point and nonpoint sources. However, various land uses present uncertainties in mercury mobility and treatment efficiency, affecting the scalability of NbS systems. In this study, a systematic review of peer-reviewed articles addressing mercury pollution in NbS soils was conducted. Results revealed that lakeside environments and mining areas are key Hg accumulation zones due to hydrological connectivity and anthropogenic pressures. Constructed wetlands were the most studied NbSs, where those with <i>Acorus calamus</i> and <i>Aquarius palifolius</i> as the main vegetation achieved >90% Hg removal efficiencies. Although NbSs achieved high Hg removal, anaerobic conditions were found to promote MeHg formation, a critical drawback. Moreover, biochar demonstrated potential for immobilizing Hg and reducing bioavailability, though certain types increased MeHg formation under specific redox conditions. Overall, the study highlighted the need for site-specific design, long-term field evaluation, and multidisciplinary strategies to optimize NbS performance for mercury removal. Furthermore, future research on the scalability of mercury-treating NbSs across diverse land uses is recommended to address mercury risks and improve effectiveness.
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spelling doaj-art-9a0ac73e0e694dcfb2fa3b406956412a2025-08-20T03:32:28ZengMDPI AGApplied Sciences2076-34172025-06-011512650210.3390/app15126502Soil Mercury Pollution in Nature-Based Solutions Across Various Land Uses: A Review of Trends, Treatment Outcomes, and Future DirectionsMiguel Enrico Robles0Yugyeong Oh1Md Tashdedul Haque2Minsu Jeon3Lee-Hyung Kim4Department of Civil and Environmental Engineering, Kongju National University, Cheonan 31080, Republic of KoreaDepartment of Civil and Environmental Engineering, Kongju National University, Cheonan 31080, Republic of KoreaDepartment of Civil and Environmental Engineering, Kongju National University, Cheonan 31080, Republic of KoreaDepartment of Civil and Environmental Engineering, Kongju National University, Cheonan 31080, Republic of KoreaDepartment of Civil and Environmental Engineering, Kongju National University, Cheonan 31080, Republic of KoreaMercury (Hg) contamination in soils poses significant environmental risks. In response, various nature-based solutions (NbSs) have been developed and studied in the past to treat mercury along with other heavy metals from both point and nonpoint sources. However, various land uses present uncertainties in mercury mobility and treatment efficiency, affecting the scalability of NbS systems. In this study, a systematic review of peer-reviewed articles addressing mercury pollution in NbS soils was conducted. Results revealed that lakeside environments and mining areas are key Hg accumulation zones due to hydrological connectivity and anthropogenic pressures. Constructed wetlands were the most studied NbSs, where those with <i>Acorus calamus</i> and <i>Aquarius palifolius</i> as the main vegetation achieved >90% Hg removal efficiencies. Although NbSs achieved high Hg removal, anaerobic conditions were found to promote MeHg formation, a critical drawback. Moreover, biochar demonstrated potential for immobilizing Hg and reducing bioavailability, though certain types increased MeHg formation under specific redox conditions. Overall, the study highlighted the need for site-specific design, long-term field evaluation, and multidisciplinary strategies to optimize NbS performance for mercury removal. Furthermore, future research on the scalability of mercury-treating NbSs across diverse land uses is recommended to address mercury risks and improve effectiveness.https://www.mdpi.com/2076-3417/15/12/6502mercury contaminationmethylmercurynature-based solutionsheavy metalssystematic review
spellingShingle Miguel Enrico Robles
Yugyeong Oh
Md Tashdedul Haque
Minsu Jeon
Lee-Hyung Kim
Soil Mercury Pollution in Nature-Based Solutions Across Various Land Uses: A Review of Trends, Treatment Outcomes, and Future Directions
Applied Sciences
mercury contamination
methylmercury
nature-based solutions
heavy metals
systematic review
title Soil Mercury Pollution in Nature-Based Solutions Across Various Land Uses: A Review of Trends, Treatment Outcomes, and Future Directions
title_full Soil Mercury Pollution in Nature-Based Solutions Across Various Land Uses: A Review of Trends, Treatment Outcomes, and Future Directions
title_fullStr Soil Mercury Pollution in Nature-Based Solutions Across Various Land Uses: A Review of Trends, Treatment Outcomes, and Future Directions
title_full_unstemmed Soil Mercury Pollution in Nature-Based Solutions Across Various Land Uses: A Review of Trends, Treatment Outcomes, and Future Directions
title_short Soil Mercury Pollution in Nature-Based Solutions Across Various Land Uses: A Review of Trends, Treatment Outcomes, and Future Directions
title_sort soil mercury pollution in nature based solutions across various land uses a review of trends treatment outcomes and future directions
topic mercury contamination
methylmercury
nature-based solutions
heavy metals
systematic review
url https://www.mdpi.com/2076-3417/15/12/6502
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