Rhizon sampler alteration of deep ocean sediment interstitial water samples, as indicated by chloride concentration and oxygen and hydrogen isotopes

Abstract Despite their potential to inform past ocean salinity, δ18O, and temperature, high‐resolution depth profiles of interstitial water chloride concentration and hydrogen and oxygen isotopes exist in very few locations. One of the primary limitations to the recovery of these depth profiles is t...

Full description

Saved in:
Bibliographic Details
Main Authors: Madeline D. Miller, Jess F. Adkins, David A. Hodell
Format: Article
Language:English
Published: Wiley 2014-06-01
Series:Geochemistry, Geophysics, Geosystems
Subjects:
Online Access:https://doi.org/10.1002/2014GC005308
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1849419465420177408
author Madeline D. Miller
Jess F. Adkins
David A. Hodell
author_facet Madeline D. Miller
Jess F. Adkins
David A. Hodell
author_sort Madeline D. Miller
collection DOAJ
description Abstract Despite their potential to inform past ocean salinity, δ18O, and temperature, high‐resolution depth profiles of interstitial water chloride concentration and hydrogen and oxygen isotopes exist in very few locations. One of the primary limitations to the recovery of these depth profiles is that traditional interstitial water sampling requires 5–10 cm whole rounds of the sediment core, which has the potential to interfere with stratigraphic continuity. The Rhizon sampler, a nondestructive tool developed for terrestrial sediment interstitial water extraction, has been proposed for efficient and nondestructive sampling of ocean sediment pore waters. However, there exists little documentation on the reliability and performance of Rhizon samplers in deep ocean sediments, particularly in regard to their effect on chloride concentration and oxygen and hydrogen isotopic measurements. We perform an intercomparison of chloride concentration and oxygen and hydrogen isotopic composition in samples taken using traditional squeezing versus those taken with Rhizon samplers. We find that samples taken with Rhizons have positive biases in both chloride concentration and stable isotopic ratios relative to those taken by squeezing water from sediments in a hydraulic press. The measured offsets between Rhizon and squeeze samples are consistent with a combination of absorption by and diffusive fractionation through the hydrophilic membrane of the Rhizon sampler. These results suggest caution is needed when using Rhizons for sampling interstitial waters in any research of processes that leave a small signal‐to‐noise ratio in dissolved concentrations or isotope ratios.
format Article
id doaj-art-99d1e14b60e545a4b046e5baab0ef600
institution Kabale University
issn 1525-2027
language English
publishDate 2014-06-01
publisher Wiley
record_format Article
series Geochemistry, Geophysics, Geosystems
spelling doaj-art-99d1e14b60e545a4b046e5baab0ef6002025-08-20T03:32:04ZengWileyGeochemistry, Geophysics, Geosystems1525-20272014-06-011562401241310.1002/2014GC005308Rhizon sampler alteration of deep ocean sediment interstitial water samples, as indicated by chloride concentration and oxygen and hydrogen isotopesMadeline D. Miller0Jess F. Adkins1David A. Hodell2Department of Mechanical EngineeringCalifornia Institute of TechnologyPasadena California USADivision of Geological and Planetary SciencesCalifornia Institute of TechnologyPasadena California USAGodwin Laboratory for Palaeoclimate Research Department of Earth SciencesUniversity of Cambridge Cambridge UKAbstract Despite their potential to inform past ocean salinity, δ18O, and temperature, high‐resolution depth profiles of interstitial water chloride concentration and hydrogen and oxygen isotopes exist in very few locations. One of the primary limitations to the recovery of these depth profiles is that traditional interstitial water sampling requires 5–10 cm whole rounds of the sediment core, which has the potential to interfere with stratigraphic continuity. The Rhizon sampler, a nondestructive tool developed for terrestrial sediment interstitial water extraction, has been proposed for efficient and nondestructive sampling of ocean sediment pore waters. However, there exists little documentation on the reliability and performance of Rhizon samplers in deep ocean sediments, particularly in regard to their effect on chloride concentration and oxygen and hydrogen isotopic measurements. We perform an intercomparison of chloride concentration and oxygen and hydrogen isotopic composition in samples taken using traditional squeezing versus those taken with Rhizon samplers. We find that samples taken with Rhizons have positive biases in both chloride concentration and stable isotopic ratios relative to those taken by squeezing water from sediments in a hydraulic press. The measured offsets between Rhizon and squeeze samples are consistent with a combination of absorption by and diffusive fractionation through the hydrophilic membrane of the Rhizon sampler. These results suggest caution is needed when using Rhizons for sampling interstitial waters in any research of processes that leave a small signal‐to‐noise ratio in dissolved concentrations or isotope ratios.https://doi.org/10.1002/2014GC005308Rhizonpore waterdeep oceansedimentisotopeconcentration
spellingShingle Madeline D. Miller
Jess F. Adkins
David A. Hodell
Rhizon sampler alteration of deep ocean sediment interstitial water samples, as indicated by chloride concentration and oxygen and hydrogen isotopes
Geochemistry, Geophysics, Geosystems
Rhizon
pore water
deep ocean
sediment
isotope
concentration
title Rhizon sampler alteration of deep ocean sediment interstitial water samples, as indicated by chloride concentration and oxygen and hydrogen isotopes
title_full Rhizon sampler alteration of deep ocean sediment interstitial water samples, as indicated by chloride concentration and oxygen and hydrogen isotopes
title_fullStr Rhizon sampler alteration of deep ocean sediment interstitial water samples, as indicated by chloride concentration and oxygen and hydrogen isotopes
title_full_unstemmed Rhizon sampler alteration of deep ocean sediment interstitial water samples, as indicated by chloride concentration and oxygen and hydrogen isotopes
title_short Rhizon sampler alteration of deep ocean sediment interstitial water samples, as indicated by chloride concentration and oxygen and hydrogen isotopes
title_sort rhizon sampler alteration of deep ocean sediment interstitial water samples as indicated by chloride concentration and oxygen and hydrogen isotopes
topic Rhizon
pore water
deep ocean
sediment
isotope
concentration
url https://doi.org/10.1002/2014GC005308
work_keys_str_mv AT madelinedmiller rhizonsampleralterationofdeepoceansedimentinterstitialwatersamplesasindicatedbychlorideconcentrationandoxygenandhydrogenisotopes
AT jessfadkins rhizonsampleralterationofdeepoceansedimentinterstitialwatersamplesasindicatedbychlorideconcentrationandoxygenandhydrogenisotopes
AT davidahodell rhizonsampleralterationofdeepoceansedimentinterstitialwatersamplesasindicatedbychlorideconcentrationandoxygenandhydrogenisotopes