Deformation and fracture of lithosphere-inspired polymeric multi-layer composites

Inspired by the diversity of structures and patterns inherent in the earth's lithosphere, this study endeavors to enhance the interplay between stiffness and toughness through the introduction of a new class of polymeric multi-layer composite materials termed by the authors as ''litho...

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Main Authors: Christoph Waly, Rita Höller, Thomas Griesser, Florian Arbeiter
Format: Article
Language:English
Published: Elsevier 2024-12-01
Series:Results in Engineering
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Online Access:http://www.sciencedirect.com/science/article/pii/S2590123024017717
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author Christoph Waly
Rita Höller
Thomas Griesser
Florian Arbeiter
author_facet Christoph Waly
Rita Höller
Thomas Griesser
Florian Arbeiter
author_sort Christoph Waly
collection DOAJ
description Inspired by the diversity of structures and patterns inherent in the earth's lithosphere, this study endeavors to enhance the interplay between stiffness and toughness through the introduction of a new class of polymeric multi-layer composite materials termed by the authors as ''lithomers''. Structured single-edge notched bending specimens were fabricated using a combination of additive manufacturing and casting, employing two different methacrylate-thiol resins. The outer layers exhibit a stiff and brittle characteristic, while the layer in between is compliant in nature. Three types of lithomers with wave-like structures and one with a rectilinear structure were investigated regarding their stiffness and toughness in a 3-point bending setup. The results were compared with those of a pure stiff matrix material. The findings revealed that fracture toughness increased regardless of the interlayer's shape compared to the pure matrix material. Correspondingly, this enhancement in fracture toughness correlated with a reduction in stiffness. The most balanced results in terms of stiffness and fracture toughness were achieved, with the lithomer having a wave-like structure in its initial stage. It exhibited a roughly 27 times improvement in fracture toughness with a moderate decrease in stiffness of approx. 1/5 compared to the pure matrix material.
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spelling doaj-art-990d86ba09104c5f80c3ffeb7dbd19a92025-08-20T02:34:36ZengElsevierResults in Engineering2590-12302024-12-012410351910.1016/j.rineng.2024.103519Deformation and fracture of lithosphere-inspired polymeric multi-layer compositesChristoph Waly0Rita Höller1Thomas Griesser2Florian Arbeiter3Materials Science and Testing of Polymers, Montanuniversitaet Leoben, Otto Gloeckel-Strasse 2 8700, Leoben, AustriaInstitute of Chemistry of Polymeric Materials, Montanuniversitaet Leoben, Otto Gloeckel-Strasse 2 8700, Leoben, AustriaInstitute of Chemistry of Polymeric Materials, Montanuniversitaet Leoben, Otto Gloeckel-Strasse 2 8700, Leoben, AustriaMaterials Science and Testing of Polymers, Montanuniversitaet Leoben, Otto Gloeckel-Strasse 2 8700, Leoben, Austria; Corresponding author.Inspired by the diversity of structures and patterns inherent in the earth's lithosphere, this study endeavors to enhance the interplay between stiffness and toughness through the introduction of a new class of polymeric multi-layer composite materials termed by the authors as ''lithomers''. Structured single-edge notched bending specimens were fabricated using a combination of additive manufacturing and casting, employing two different methacrylate-thiol resins. The outer layers exhibit a stiff and brittle characteristic, while the layer in between is compliant in nature. Three types of lithomers with wave-like structures and one with a rectilinear structure were investigated regarding their stiffness and toughness in a 3-point bending setup. The results were compared with those of a pure stiff matrix material. The findings revealed that fracture toughness increased regardless of the interlayer's shape compared to the pure matrix material. Correspondingly, this enhancement in fracture toughness correlated with a reduction in stiffness. The most balanced results in terms of stiffness and fracture toughness were achieved, with the lithomer having a wave-like structure in its initial stage. It exhibited a roughly 27 times improvement in fracture toughness with a moderate decrease in stiffness of approx. 1/5 compared to the pure matrix material.http://www.sciencedirect.com/science/article/pii/S2590123024017717LithomersLithomimeticsBiomimeticsFracture toughnessMulti-layered structure
spellingShingle Christoph Waly
Rita Höller
Thomas Griesser
Florian Arbeiter
Deformation and fracture of lithosphere-inspired polymeric multi-layer composites
Results in Engineering
Lithomers
Lithomimetics
Biomimetics
Fracture toughness
Multi-layered structure
title Deformation and fracture of lithosphere-inspired polymeric multi-layer composites
title_full Deformation and fracture of lithosphere-inspired polymeric multi-layer composites
title_fullStr Deformation and fracture of lithosphere-inspired polymeric multi-layer composites
title_full_unstemmed Deformation and fracture of lithosphere-inspired polymeric multi-layer composites
title_short Deformation and fracture of lithosphere-inspired polymeric multi-layer composites
title_sort deformation and fracture of lithosphere inspired polymeric multi layer composites
topic Lithomers
Lithomimetics
Biomimetics
Fracture toughness
Multi-layered structure
url http://www.sciencedirect.com/science/article/pii/S2590123024017717
work_keys_str_mv AT christophwaly deformationandfractureoflithosphereinspiredpolymericmultilayercomposites
AT ritaholler deformationandfractureoflithosphereinspiredpolymericmultilayercomposites
AT thomasgriesser deformationandfractureoflithosphereinspiredpolymericmultilayercomposites
AT florianarbeiter deformationandfractureoflithosphereinspiredpolymericmultilayercomposites