Construction and Application of Au NRs/4-MBA/PAM Ratiometric Surface-Enhanced Raman Scattering Substrate for Fish Veterinary Drug Residue Detection

Surface-enhanced Raman scattering (SERS) is widely used for trace detection of substances, and the key to this technology lies in the preparation of the substrate material. In this study, a composite SERS material of Au NRs/4-MBA/PAM was constructed and characterized to better immobilize the referen...

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Main Authors: Jianxing Yu, Huiping Fu, Qing Gu
Format: Article
Language:English
Published: MDPI AG 2024-11-01
Series:Nanomaterials
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Online Access:https://www.mdpi.com/2079-4991/14/22/1774
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author Jianxing Yu
Huiping Fu
Qing Gu
author_facet Jianxing Yu
Huiping Fu
Qing Gu
author_sort Jianxing Yu
collection DOAJ
description Surface-enhanced Raman scattering (SERS) is widely used for trace detection of substances, and the key to this technology lies in the preparation of the substrate material. In this study, a composite SERS material of Au NRs/4-MBA/PAM was constructed and characterized to better immobilize the reference molecule 4-mercaptobenzoic acid (4-MBA). Electron transmission microscopy results demonstrated that the PAM film helps Au NRs to pack closely, enhancing the stability of the material structure and reducing the interference of external environmental factors on the response of 4-MBA, thus improving the accuracy of quantitative determination. Comparative experimental results with the Au NRs/4-MBA substrate showed that the relative standard deviations (RSDs) of the detection results for MG on different batches of Au NRs/4-MBA/PAM were less than 8.0%, and the RSDs of different points on the same material were less than 10.0%, indicating that the Au NRs/4-MBA/PAM has higher uniformity, better reproducibility, and higher sensitivity in detecting malachite green (MG). Applying this material in the recovery determination of fish extract showed that the recovery rates of MG were between 75.60% and 83.24%. Therefore, the Au NRs/4-MBA/PAM substrate can accurately detect and quantify veterinary drug residue in complex matrices such as food tissue.
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spelling doaj-art-98d69c7f6d3345d1ab401f8f174d7ff62025-08-20T02:48:06ZengMDPI AGNanomaterials2079-49912024-11-011422177410.3390/nano14221774Construction and Application of Au NRs/4-MBA/PAM Ratiometric Surface-Enhanced Raman Scattering Substrate for Fish Veterinary Drug Residue DetectionJianxing Yu0Huiping Fu1Qing Gu2Zhejiang Key Laboratory of Food Microbiology and Nutritional Health, School of Food Science and Biotechnology, Zhejiang Gongshang University, Hangzhou 310018, ChinaCollege of Chemistry, Fuzhou University, Fuzhou 350116, ChinaZhejiang Key Laboratory of Food Microbiology and Nutritional Health, School of Food Science and Biotechnology, Zhejiang Gongshang University, Hangzhou 310018, ChinaSurface-enhanced Raman scattering (SERS) is widely used for trace detection of substances, and the key to this technology lies in the preparation of the substrate material. In this study, a composite SERS material of Au NRs/4-MBA/PAM was constructed and characterized to better immobilize the reference molecule 4-mercaptobenzoic acid (4-MBA). Electron transmission microscopy results demonstrated that the PAM film helps Au NRs to pack closely, enhancing the stability of the material structure and reducing the interference of external environmental factors on the response of 4-MBA, thus improving the accuracy of quantitative determination. Comparative experimental results with the Au NRs/4-MBA substrate showed that the relative standard deviations (RSDs) of the detection results for MG on different batches of Au NRs/4-MBA/PAM were less than 8.0%, and the RSDs of different points on the same material were less than 10.0%, indicating that the Au NRs/4-MBA/PAM has higher uniformity, better reproducibility, and higher sensitivity in detecting malachite green (MG). Applying this material in the recovery determination of fish extract showed that the recovery rates of MG were between 75.60% and 83.24%. Therefore, the Au NRs/4-MBA/PAM substrate can accurately detect and quantify veterinary drug residue in complex matrices such as food tissue.https://www.mdpi.com/2079-4991/14/22/1774Au nanorodssurface-enhanced Raman scatteringpolyacrylamide4-mercaptobenzoic acidveterinary drug residues
spellingShingle Jianxing Yu
Huiping Fu
Qing Gu
Construction and Application of Au NRs/4-MBA/PAM Ratiometric Surface-Enhanced Raman Scattering Substrate for Fish Veterinary Drug Residue Detection
Nanomaterials
Au nanorods
surface-enhanced Raman scattering
polyacrylamide
4-mercaptobenzoic acid
veterinary drug residues
title Construction and Application of Au NRs/4-MBA/PAM Ratiometric Surface-Enhanced Raman Scattering Substrate for Fish Veterinary Drug Residue Detection
title_full Construction and Application of Au NRs/4-MBA/PAM Ratiometric Surface-Enhanced Raman Scattering Substrate for Fish Veterinary Drug Residue Detection
title_fullStr Construction and Application of Au NRs/4-MBA/PAM Ratiometric Surface-Enhanced Raman Scattering Substrate for Fish Veterinary Drug Residue Detection
title_full_unstemmed Construction and Application of Au NRs/4-MBA/PAM Ratiometric Surface-Enhanced Raman Scattering Substrate for Fish Veterinary Drug Residue Detection
title_short Construction and Application of Au NRs/4-MBA/PAM Ratiometric Surface-Enhanced Raman Scattering Substrate for Fish Veterinary Drug Residue Detection
title_sort construction and application of au nrs 4 mba pam ratiometric surface enhanced raman scattering substrate for fish veterinary drug residue detection
topic Au nanorods
surface-enhanced Raman scattering
polyacrylamide
4-mercaptobenzoic acid
veterinary drug residues
url https://www.mdpi.com/2079-4991/14/22/1774
work_keys_str_mv AT jianxingyu constructionandapplicationofaunrs4mbapamratiometricsurfaceenhancedramanscatteringsubstrateforfishveterinarydrugresiduedetection
AT huipingfu constructionandapplicationofaunrs4mbapamratiometricsurfaceenhancedramanscatteringsubstrateforfishveterinarydrugresiduedetection
AT qinggu constructionandapplicationofaunrs4mbapamratiometricsurfaceenhancedramanscatteringsubstrateforfishveterinarydrugresiduedetection