Synergistic effect of proteins and tannic acid-yielding systems with improved mechanical performance for use in load-bearing tissues

Developing bioactive hydrogels with mechanical properties resembling those of load-bearing connective tissues remains a significant challenge in the biomedical field. In this study, we address this limitation by incorporating human platelet lysate (PL) proteins, tannic acid (TA), and chitosan methac...

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Main Authors: Maria Clara Gomes, Claudio Mortier, Håvard J Haugen, Jonny J Blaker, João F Mano
Format: Article
Language:English
Published: IOP Publishing 2025-01-01
Series:Materials Research Express
Subjects:
Online Access:https://doi.org/10.1088/2053-1591/adee7e
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author Maria Clara Gomes
Claudio Mortier
Håvard J Haugen
Jonny J Blaker
João F Mano
author_facet Maria Clara Gomes
Claudio Mortier
Håvard J Haugen
Jonny J Blaker
João F Mano
author_sort Maria Clara Gomes
collection DOAJ
description Developing bioactive hydrogels with mechanical properties resembling those of load-bearing connective tissues remains a significant challenge in the biomedical field. In this study, we address this limitation by incorporating human platelet lysate (PL) proteins, tannic acid (TA), and chitosan methacrylate (CHI-MA) to formulate reinforced hydrogel systems with markedly improved mechanical performance. The resulting PL/CHI-MA/TA hydrogels exhibit exceptional mechanical characteristics, attaining strengths of approximately 7 MPa and stiffness values of 5 MPa, comparable to those found in load-bearing tissues such as cartilage. This improvement can be attributed to the synergistic effect, which enhances the interaction between PL proteins and the polymeric network, thereby increasing strength, toughness, and efficient energy dissipation. Moreover, these hydrogels support the adhesion and proliferation of human-derived adipose stem cells, underscoring their potential utility in tissue engineering and regenerative medicine applications targeting load-bearing connective tissues, such as cartilage.
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spelling doaj-art-98ad817afdc246d69c4eaabd3b2576fe2025-08-20T03:51:24ZengIOP PublishingMaterials Research Express2053-15912025-01-0112707540410.1088/2053-1591/adee7eSynergistic effect of proteins and tannic acid-yielding systems with improved mechanical performance for use in load-bearing tissuesMaria Clara Gomes0Claudio Mortier1Håvard J Haugen2https://orcid.org/0000-0002-6690-7233Jonny J Blaker3João F Mano4https://orcid.org/0000-0002-2342-3765Department of Chemistry, CICECO-Aveiro Institute of Materials, University of Aveiro , PortugalDepartment of Chemistry, CICECO-Aveiro Institute of Materials, University of Aveiro , Portugal; Institute of Clinical Dentistry, University of Oslo , NorwayInstitute of Clinical Dentistry, University of Oslo , NorwayInstitute of Clinical Dentistry, University of Oslo , Norway; Department of Materials & Henry Royce Institute, The University of Manchester , Manchester, United KingdomDepartment of Chemistry, CICECO-Aveiro Institute of Materials, University of Aveiro , PortugalDeveloping bioactive hydrogels with mechanical properties resembling those of load-bearing connective tissues remains a significant challenge in the biomedical field. In this study, we address this limitation by incorporating human platelet lysate (PL) proteins, tannic acid (TA), and chitosan methacrylate (CHI-MA) to formulate reinforced hydrogel systems with markedly improved mechanical performance. The resulting PL/CHI-MA/TA hydrogels exhibit exceptional mechanical characteristics, attaining strengths of approximately 7 MPa and stiffness values of 5 MPa, comparable to those found in load-bearing tissues such as cartilage. This improvement can be attributed to the synergistic effect, which enhances the interaction between PL proteins and the polymeric network, thereby increasing strength, toughness, and efficient energy dissipation. Moreover, these hydrogels support the adhesion and proliferation of human-derived adipose stem cells, underscoring their potential utility in tissue engineering and regenerative medicine applications targeting load-bearing connective tissues, such as cartilage.https://doi.org/10.1088/2053-1591/adee7eplatelet lysatesproteinsimproved mechanical propertieshydrogels
spellingShingle Maria Clara Gomes
Claudio Mortier
Håvard J Haugen
Jonny J Blaker
João F Mano
Synergistic effect of proteins and tannic acid-yielding systems with improved mechanical performance for use in load-bearing tissues
Materials Research Express
platelet lysates
proteins
improved mechanical properties
hydrogels
title Synergistic effect of proteins and tannic acid-yielding systems with improved mechanical performance for use in load-bearing tissues
title_full Synergistic effect of proteins and tannic acid-yielding systems with improved mechanical performance for use in load-bearing tissues
title_fullStr Synergistic effect of proteins and tannic acid-yielding systems with improved mechanical performance for use in load-bearing tissues
title_full_unstemmed Synergistic effect of proteins and tannic acid-yielding systems with improved mechanical performance for use in load-bearing tissues
title_short Synergistic effect of proteins and tannic acid-yielding systems with improved mechanical performance for use in load-bearing tissues
title_sort synergistic effect of proteins and tannic acid yielding systems with improved mechanical performance for use in load bearing tissues
topic platelet lysates
proteins
improved mechanical properties
hydrogels
url https://doi.org/10.1088/2053-1591/adee7e
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AT havardjhaugen synergisticeffectofproteinsandtannicacidyieldingsystemswithimprovedmechanicalperformanceforuseinloadbearingtissues
AT jonnyjblaker synergisticeffectofproteinsandtannicacidyieldingsystemswithimprovedmechanicalperformanceforuseinloadbearingtissues
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