Plant volatiles-loaded core-shell micro-nano fibers to achieve efficient and sustained bisexual attraction to pests

Abstract Background Chemical pesticides face significant challenges regarding their efficacy and environmental impact. Plant-based food attractants have emerged as a promising green alternative for pest control. However, their field application is limited by the short duration of effectiveness, nece...

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Main Authors: Chenglong Cui, Wenjie Shangguan, Kebin Li, Xingfu Jiang, Zhimin Wang, Jiao Yin, Lidong Cao
Format: Article
Language:English
Published: BMC 2025-04-01
Series:Journal of Nanobiotechnology
Subjects:
Online Access:https://doi.org/10.1186/s12951-025-03269-2
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author Chenglong Cui
Wenjie Shangguan
Kebin Li
Xingfu Jiang
Zhimin Wang
Jiao Yin
Lidong Cao
author_facet Chenglong Cui
Wenjie Shangguan
Kebin Li
Xingfu Jiang
Zhimin Wang
Jiao Yin
Lidong Cao
author_sort Chenglong Cui
collection DOAJ
description Abstract Background Chemical pesticides face significant challenges regarding their efficacy and environmental impact. Plant-based food attractants have emerged as a promising green alternative for pest control. However, their field application is limited by the short duration of effectiveness, necessitating improved carrier systems for sustained release. Electrospinning is a promising technology in this field, with core-shell fibers offering superior performance in efficient loading and sustained release compared to uniaxial fibers, highlighting their potential for further development. Results In this study, core-shell micro-nano fiber mats were prepared via coaxial electrospinning using multiple environmentally friendly polymers. These mats were firstly and successfully loaded with food attractants bisexually attractive to Loxostege sticticalis adults, including 1-octen-3-ol, trans-2-hexenal, linalool, and anethole, enabling sustained release and effective trapping. The components in the core-shell spinning solution were chemically compatible, and after spinning, the poly(3-hydroxybutyrate-co-4-hydroxybutyrate)/polycaprolactone (PHB/PCL) in the shell layer and polyethylene oxide (PEO) in the core layer formed core-shell fibers with clear boundaries. The mats achieved an average encapsulation efficiency of 78% for active ingredients, with a sustained release profile that delivered over 60% of the attractants within 80 days while mitigating early burst release. Electroantennogram and behavioral studies revealed that the mats retained electrophysiological activity for at least 90 days, effectively attracting male and female adult insects even after 75 days. Field trials demonstrated that the mats significantly outperformed commercial slow-release carriers, attracting a higher number of L. sticticalis adults. Additionally, the mats exhibited strong stress resistance, biodegradability, and environmental compatibility, effectively protecting active molecules while minimizing ecological impact. Conclusions The developed fiber mats provide a highly efficient, eco-friendly carrier for plant-based food attractants, offering prolonged efficacy and improved insect trapping performance. This study highlights their potential for sustainable agriculture and pest management, paving the way for greener alternatives to chemical pesticides. Graphical abstract
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spelling doaj-art-98828cf4b2cd4b6fb48760e58aa589092025-08-20T02:25:41ZengBMCJournal of Nanobiotechnology1477-31552025-04-0123111710.1186/s12951-025-03269-2Plant volatiles-loaded core-shell micro-nano fibers to achieve efficient and sustained bisexual attraction to pestsChenglong Cui0Wenjie Shangguan1Kebin Li2Xingfu Jiang3Zhimin Wang4Jiao Yin5Lidong Cao6State Key Laboratory for Biology of Plant Diseases and Insect Pests, Institute of Plant Protection of Chinese Academy of Agricultural SciencesState Key Laboratory for Biology of Plant Diseases and Insect Pests, Institute of Plant Protection of Chinese Academy of Agricultural SciencesState Key Laboratory for Biology of Plant Diseases and Insect Pests, Institute of Plant Protection of Chinese Academy of Agricultural SciencesState Key Laboratory for Biology of Plant Diseases and Insect Pests, Institute of Plant Protection of Chinese Academy of Agricultural SciencesState Key Laboratory for Biology of Plant Diseases and Insect Pests, Institute of Plant Protection of Chinese Academy of Agricultural SciencesState Key Laboratory for Biology of Plant Diseases and Insect Pests, Institute of Plant Protection of Chinese Academy of Agricultural SciencesState Key Laboratory for Biology of Plant Diseases and Insect Pests, Institute of Plant Protection of Chinese Academy of Agricultural SciencesAbstract Background Chemical pesticides face significant challenges regarding their efficacy and environmental impact. Plant-based food attractants have emerged as a promising green alternative for pest control. However, their field application is limited by the short duration of effectiveness, necessitating improved carrier systems for sustained release. Electrospinning is a promising technology in this field, with core-shell fibers offering superior performance in efficient loading and sustained release compared to uniaxial fibers, highlighting their potential for further development. Results In this study, core-shell micro-nano fiber mats were prepared via coaxial electrospinning using multiple environmentally friendly polymers. These mats were firstly and successfully loaded with food attractants bisexually attractive to Loxostege sticticalis adults, including 1-octen-3-ol, trans-2-hexenal, linalool, and anethole, enabling sustained release and effective trapping. The components in the core-shell spinning solution were chemically compatible, and after spinning, the poly(3-hydroxybutyrate-co-4-hydroxybutyrate)/polycaprolactone (PHB/PCL) in the shell layer and polyethylene oxide (PEO) in the core layer formed core-shell fibers with clear boundaries. The mats achieved an average encapsulation efficiency of 78% for active ingredients, with a sustained release profile that delivered over 60% of the attractants within 80 days while mitigating early burst release. Electroantennogram and behavioral studies revealed that the mats retained electrophysiological activity for at least 90 days, effectively attracting male and female adult insects even after 75 days. Field trials demonstrated that the mats significantly outperformed commercial slow-release carriers, attracting a higher number of L. sticticalis adults. Additionally, the mats exhibited strong stress resistance, biodegradability, and environmental compatibility, effectively protecting active molecules while minimizing ecological impact. Conclusions The developed fiber mats provide a highly efficient, eco-friendly carrier for plant-based food attractants, offering prolonged efficacy and improved insect trapping performance. This study highlights their potential for sustainable agriculture and pest management, paving the way for greener alternatives to chemical pesticides. Graphical abstracthttps://doi.org/10.1186/s12951-025-03269-2Food attractantsMicro-nano fiberSustained releaseCoaxial electrospinningGreen pesticide
spellingShingle Chenglong Cui
Wenjie Shangguan
Kebin Li
Xingfu Jiang
Zhimin Wang
Jiao Yin
Lidong Cao
Plant volatiles-loaded core-shell micro-nano fibers to achieve efficient and sustained bisexual attraction to pests
Journal of Nanobiotechnology
Food attractants
Micro-nano fiber
Sustained release
Coaxial electrospinning
Green pesticide
title Plant volatiles-loaded core-shell micro-nano fibers to achieve efficient and sustained bisexual attraction to pests
title_full Plant volatiles-loaded core-shell micro-nano fibers to achieve efficient and sustained bisexual attraction to pests
title_fullStr Plant volatiles-loaded core-shell micro-nano fibers to achieve efficient and sustained bisexual attraction to pests
title_full_unstemmed Plant volatiles-loaded core-shell micro-nano fibers to achieve efficient and sustained bisexual attraction to pests
title_short Plant volatiles-loaded core-shell micro-nano fibers to achieve efficient and sustained bisexual attraction to pests
title_sort plant volatiles loaded core shell micro nano fibers to achieve efficient and sustained bisexual attraction to pests
topic Food attractants
Micro-nano fiber
Sustained release
Coaxial electrospinning
Green pesticide
url https://doi.org/10.1186/s12951-025-03269-2
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