Parametric Study of Time-Dependent Corrosion Product Activity due to 56Mn, 58Co, and 60Co in the Primary Coolant Circuit of a Typical Pressurized Water Reactor

Results of a detailed study, based on the parametric analysis of activated corrosion products, in primary coolant of a typical pressurized water reactor (PWR) are presented. The parameters influencing time dependent buildup of corrosion product activity (CPA) in primary coolant loop of PWR were iden...

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Main Authors: Muhammad Rafique, Nasir M. Mirza, Sikander M. Mirza, Kimberlee J. Kearfott, Shahab A. Abbasi, Syed F. Naeem
Format: Article
Language:English
Published: Wiley 2015-01-01
Series:Journal of Chemistry
Online Access:http://dx.doi.org/10.1155/2015/809672
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author Muhammad Rafique
Nasir M. Mirza
Sikander M. Mirza
Kimberlee J. Kearfott
Shahab A. Abbasi
Syed F. Naeem
author_facet Muhammad Rafique
Nasir M. Mirza
Sikander M. Mirza
Kimberlee J. Kearfott
Shahab A. Abbasi
Syed F. Naeem
author_sort Muhammad Rafique
collection DOAJ
description Results of a detailed study, based on the parametric analysis of activated corrosion products, in primary coolant of a typical pressurized water reactor (PWR) are presented. The parameters influencing time dependent buildup of corrosion product activity (CPA) in primary coolant loop of PWR were identified. The computer program CPAIR was used to accommodate for time dependent corrosion rates. The behaviors of 56Mn, 58Co, and 60Co were studied over the reactor operational time. During the course of normal operation of reactor, the CPA is dominated by 56Mn, while 58Co and 60Co are the predominant radionuclides after reactor shutdown. Parametric study suggests that the total CPA is most sensitive to ion-exchanger removal rates. For a removal rate of 300 cm3-s−1, the specific activity due to 56Mn has the maximum value of 3.552 × 104 Bq-m−3 after 1,000 hours of reactor operation. This value decreases drastically to 8.325 × 103 Bq-m−3 at removal rate of 900 cm3-s−1. Additionally, CPA due to 56Mn, 58Co, and 60Co shows strong dependence on removal rates from the core material surfaces. Variations in the values of radionuclide removal rates from piping surface and radionuclide removal rate from deposition on pipes showed only very small effects on CPA buildup.
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spelling doaj-art-9858f4cef8434f8c92fcc13fd95bf4642025-02-03T06:11:21ZengWileyJournal of Chemistry2090-90632090-90712015-01-01201510.1155/2015/809672809672Parametric Study of Time-Dependent Corrosion Product Activity due to 56Mn, 58Co, and 60Co in the Primary Coolant Circuit of a Typical Pressurized Water ReactorMuhammad Rafique0Nasir M. Mirza1Sikander M. Mirza2Kimberlee J. Kearfott3Shahab A. Abbasi4Syed F. Naeem5Department of Physics, University of Azad Jammu and Kashmir, Muzaffarabad, Azad Kashmir 13100, PakistanDepartment of Physics and Applied Mathematics, Pakistan Institute of Engineering and Applied Sciences, Nilore, Islamabad 45650, PakistanDepartment of Physics and Applied Mathematics, Pakistan Institute of Engineering and Applied Sciences, Nilore, Islamabad 45650, PakistanDepartment of Nuclear Engineering and Radiological Sciences, University of Michigan, 2355 Bonisteel Boulevard, Ann Arbor, MI 48109-2104, USADepartment of Physics, University of Azad Jammu and Kashmir, Muzaffarabad, Azad Kashmir 13100, PakistanDepartment of Nuclear Engineering and Radiological Sciences, University of Michigan, 2355 Bonisteel Boulevard, Ann Arbor, MI 48109-2104, USAResults of a detailed study, based on the parametric analysis of activated corrosion products, in primary coolant of a typical pressurized water reactor (PWR) are presented. The parameters influencing time dependent buildup of corrosion product activity (CPA) in primary coolant loop of PWR were identified. The computer program CPAIR was used to accommodate for time dependent corrosion rates. The behaviors of 56Mn, 58Co, and 60Co were studied over the reactor operational time. During the course of normal operation of reactor, the CPA is dominated by 56Mn, while 58Co and 60Co are the predominant radionuclides after reactor shutdown. Parametric study suggests that the total CPA is most sensitive to ion-exchanger removal rates. For a removal rate of 300 cm3-s−1, the specific activity due to 56Mn has the maximum value of 3.552 × 104 Bq-m−3 after 1,000 hours of reactor operation. This value decreases drastically to 8.325 × 103 Bq-m−3 at removal rate of 900 cm3-s−1. Additionally, CPA due to 56Mn, 58Co, and 60Co shows strong dependence on removal rates from the core material surfaces. Variations in the values of radionuclide removal rates from piping surface and radionuclide removal rate from deposition on pipes showed only very small effects on CPA buildup.http://dx.doi.org/10.1155/2015/809672
spellingShingle Muhammad Rafique
Nasir M. Mirza
Sikander M. Mirza
Kimberlee J. Kearfott
Shahab A. Abbasi
Syed F. Naeem
Parametric Study of Time-Dependent Corrosion Product Activity due to 56Mn, 58Co, and 60Co in the Primary Coolant Circuit of a Typical Pressurized Water Reactor
Journal of Chemistry
title Parametric Study of Time-Dependent Corrosion Product Activity due to 56Mn, 58Co, and 60Co in the Primary Coolant Circuit of a Typical Pressurized Water Reactor
title_full Parametric Study of Time-Dependent Corrosion Product Activity due to 56Mn, 58Co, and 60Co in the Primary Coolant Circuit of a Typical Pressurized Water Reactor
title_fullStr Parametric Study of Time-Dependent Corrosion Product Activity due to 56Mn, 58Co, and 60Co in the Primary Coolant Circuit of a Typical Pressurized Water Reactor
title_full_unstemmed Parametric Study of Time-Dependent Corrosion Product Activity due to 56Mn, 58Co, and 60Co in the Primary Coolant Circuit of a Typical Pressurized Water Reactor
title_short Parametric Study of Time-Dependent Corrosion Product Activity due to 56Mn, 58Co, and 60Co in the Primary Coolant Circuit of a Typical Pressurized Water Reactor
title_sort parametric study of time dependent corrosion product activity due to 56mn 58co and 60co in the primary coolant circuit of a typical pressurized water reactor
url http://dx.doi.org/10.1155/2015/809672
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