Thermoelectric Modulation of Neat Ti3C2Tx MXenes by Finely Regulating the Stacking of Nanosheets

Highlights Investigation of dispersing solvents on processing Ti3C2Tx thin films revealed that deionized water is superior to realize tight stacking and high orientation of MXene nanosheets. A simultaneous elevation of Seebeck coefficient and electrical conductivity of neat Ti3C2Tx films is achieved...

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Main Authors: Junhui Tang, Renyang Zhu, Ya-Hsin Pai, Yan Zhao, Chen Xu, Ziqi Liang
Format: Article
Language:English
Published: SpringerOpen 2024-12-01
Series:Nano-Micro Letters
Subjects:
Online Access:https://doi.org/10.1007/s40820-024-01594-z
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author Junhui Tang
Renyang Zhu
Ya-Hsin Pai
Yan Zhao
Chen Xu
Ziqi Liang
author_facet Junhui Tang
Renyang Zhu
Ya-Hsin Pai
Yan Zhao
Chen Xu
Ziqi Liang
author_sort Junhui Tang
collection DOAJ
description Highlights Investigation of dispersing solvents on processing Ti3C2Tx thin films revealed that deionized water is superior to realize tight stacking and high orientation of MXene nanosheets. A simultaneous elevation of Seebeck coefficient and electrical conductivity of neat Ti3C2Tx films is achieved by increasing the centrifugal speed of MXene aqueous suspensions due to the energy filtering effect. Further construction of Ti3C2Tx nanocomposites significantly strengthens Seebeck coefficient yet disrupts the stacking of MXene nanosheets.
format Article
id doaj-art-973ce3a5e91942e5a1ad5409f02b58e6
institution Kabale University
issn 2311-6706
2150-5551
language English
publishDate 2024-12-01
publisher SpringerOpen
record_format Article
series Nano-Micro Letters
spelling doaj-art-973ce3a5e91942e5a1ad5409f02b58e62025-08-20T04:03:01ZengSpringerOpenNano-Micro Letters2311-67062150-55512024-12-0117111610.1007/s40820-024-01594-zThermoelectric Modulation of Neat Ti3C2Tx MXenes by Finely Regulating the Stacking of NanosheetsJunhui Tang0Renyang Zhu1Ya-Hsin Pai2Yan Zhao3Chen Xu4Ziqi Liang5Department of Materials Science, Fudan UniversityDepartment of Materials Science, Fudan UniversityDepartment of Materials Science, Fudan UniversityDepartment of Materials Science, Fudan UniversitySpine Center, Department of Orthopedics, Shanghai Changzheng Hospital, Naval Medical UniversityDepartment of Materials Science, Fudan UniversityHighlights Investigation of dispersing solvents on processing Ti3C2Tx thin films revealed that deionized water is superior to realize tight stacking and high orientation of MXene nanosheets. A simultaneous elevation of Seebeck coefficient and electrical conductivity of neat Ti3C2Tx films is achieved by increasing the centrifugal speed of MXene aqueous suspensions due to the energy filtering effect. Further construction of Ti3C2Tx nanocomposites significantly strengthens Seebeck coefficient yet disrupts the stacking of MXene nanosheets.https://doi.org/10.1007/s40820-024-01594-zMXeneNanosheet stackingElectrical conductivitySeebeck coefficientThermoelectrics
spellingShingle Junhui Tang
Renyang Zhu
Ya-Hsin Pai
Yan Zhao
Chen Xu
Ziqi Liang
Thermoelectric Modulation of Neat Ti3C2Tx MXenes by Finely Regulating the Stacking of Nanosheets
Nano-Micro Letters
MXene
Nanosheet stacking
Electrical conductivity
Seebeck coefficient
Thermoelectrics
title Thermoelectric Modulation of Neat Ti3C2Tx MXenes by Finely Regulating the Stacking of Nanosheets
title_full Thermoelectric Modulation of Neat Ti3C2Tx MXenes by Finely Regulating the Stacking of Nanosheets
title_fullStr Thermoelectric Modulation of Neat Ti3C2Tx MXenes by Finely Regulating the Stacking of Nanosheets
title_full_unstemmed Thermoelectric Modulation of Neat Ti3C2Tx MXenes by Finely Regulating the Stacking of Nanosheets
title_short Thermoelectric Modulation of Neat Ti3C2Tx MXenes by Finely Regulating the Stacking of Nanosheets
title_sort thermoelectric modulation of neat ti3c2tx mxenes by finely regulating the stacking of nanosheets
topic MXene
Nanosheet stacking
Electrical conductivity
Seebeck coefficient
Thermoelectrics
url https://doi.org/10.1007/s40820-024-01594-z
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