An Analytical Evaluation of the Synergistic Effect on Biodiesel Oxidation Stability Promoted by Binary and Ternary Blends Containing Multifunctional Additives

The antioxidant potential of a novel additive, named maleimide p-CH3, and the synergistic effect on biodiesel stabilization when combined with a traditional synthetic antioxidant (e.g., propyl gallate (PG)) as well as alternative additives (e.g., alizarin (ALZ) and citric acid (CA)) were investigate...

Full description

Saved in:
Bibliographic Details
Main Authors: Silvia S. Yahagi, Ana C. Roveda, Adrielli T. Sobral, Ivan P. Oliveira, Anderson R. L. Caires, Roberto S. Gomes, Magno A. G. Trindade
Format: Article
Language:English
Published: Wiley 2019-01-01
Series:International Journal of Analytical Chemistry
Online Access:http://dx.doi.org/10.1155/2019/6467183
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1850210205980164096
author Silvia S. Yahagi
Ana C. Roveda
Adrielli T. Sobral
Ivan P. Oliveira
Anderson R. L. Caires
Roberto S. Gomes
Magno A. G. Trindade
author_facet Silvia S. Yahagi
Ana C. Roveda
Adrielli T. Sobral
Ivan P. Oliveira
Anderson R. L. Caires
Roberto S. Gomes
Magno A. G. Trindade
author_sort Silvia S. Yahagi
collection DOAJ
description The antioxidant potential of a novel additive, named maleimide p-CH3, and the synergistic effect on biodiesel stabilization when combined with a traditional synthetic antioxidant (e.g., propyl gallate (PG)) as well as alternative additives (e.g., alizarin (ALZ) and citric acid (CA)) were investigated. The additives were combined in binary and/or ternary blends at low concentrations and their effectiveness against soybean biodiesel oxidation in the absence and presence of metal was tested. The effectiveness of binary and ternary blends was also evaluated by the Rancimat® method and compared with total acid number (TAN). The results showed that the combinations presented synergetic effects and were effective in stabilizing biodiesel in accordance with the minimum requirements of EN 14214 and also revealed that the mixture containing PG and p-CH3, even at low concentrations, can be successfully applied for biodiesel preservation. In summary, we report that the biodiesel stability can be obtained by using a reduced amount of additives, suggesting that biodiesel shelf life can be improved in association with a cost reduction when compared to the use of conventional antioxidants.
format Article
id doaj-art-96d0ca1a31334e4f9977e9d859054349
institution OA Journals
issn 1687-8760
1687-8779
language English
publishDate 2019-01-01
publisher Wiley
record_format Article
series International Journal of Analytical Chemistry
spelling doaj-art-96d0ca1a31334e4f9977e9d8590543492025-08-20T02:09:49ZengWileyInternational Journal of Analytical Chemistry1687-87601687-87792019-01-01201910.1155/2019/64671836467183An Analytical Evaluation of the Synergistic Effect on Biodiesel Oxidation Stability Promoted by Binary and Ternary Blends Containing Multifunctional AdditivesSilvia S. Yahagi0Ana C. Roveda1Adrielli T. Sobral2Ivan P. Oliveira3Anderson R. L. Caires4Roberto S. Gomes5Magno A. G. Trindade6Faculty of Exact Sciences and Technology, Federal University of Grande Dourados, Highway Dourados-Itahum, Km 12, P.O. Box 364, 79804-970 Dourados, MS, BrazilFaculty of Exact Sciences and Technology, Federal University of Grande Dourados, Highway Dourados-Itahum, Km 12, P.O. Box 364, 79804-970 Dourados, MS, BrazilFaculty of Exact Sciences and Technology, Federal University of Grande Dourados, Highway Dourados-Itahum, Km 12, P.O. Box 364, 79804-970 Dourados, MS, BrazilInstitute of Biomedical Sciences, University of São Paulo, Av. Prof. Lineu Prestes, 1524, 05508-900 São Paulo, SP, BrazilOptics and Photonics Group, Institute of Physics, Federal University of Mato Grosso do Sul, P.O. Box 549, 79070900 Campo Grande, MS, BrazilSynthesis and Molecular Modification Laboratory, Faculty of Exact Sciences and Technology, Federal University of Grande Dourados, Rodovia Dourados-Itahum, Km 12, 79804-970 Dourados, MS, BrazilFaculty of Exact Sciences and Technology, Federal University of Grande Dourados, Highway Dourados-Itahum, Km 12, P.O. Box 364, 79804-970 Dourados, MS, BrazilThe antioxidant potential of a novel additive, named maleimide p-CH3, and the synergistic effect on biodiesel stabilization when combined with a traditional synthetic antioxidant (e.g., propyl gallate (PG)) as well as alternative additives (e.g., alizarin (ALZ) and citric acid (CA)) were investigated. The additives were combined in binary and/or ternary blends at low concentrations and their effectiveness against soybean biodiesel oxidation in the absence and presence of metal was tested. The effectiveness of binary and ternary blends was also evaluated by the Rancimat® method and compared with total acid number (TAN). The results showed that the combinations presented synergetic effects and were effective in stabilizing biodiesel in accordance with the minimum requirements of EN 14214 and also revealed that the mixture containing PG and p-CH3, even at low concentrations, can be successfully applied for biodiesel preservation. In summary, we report that the biodiesel stability can be obtained by using a reduced amount of additives, suggesting that biodiesel shelf life can be improved in association with a cost reduction when compared to the use of conventional antioxidants.http://dx.doi.org/10.1155/2019/6467183
spellingShingle Silvia S. Yahagi
Ana C. Roveda
Adrielli T. Sobral
Ivan P. Oliveira
Anderson R. L. Caires
Roberto S. Gomes
Magno A. G. Trindade
An Analytical Evaluation of the Synergistic Effect on Biodiesel Oxidation Stability Promoted by Binary and Ternary Blends Containing Multifunctional Additives
International Journal of Analytical Chemistry
title An Analytical Evaluation of the Synergistic Effect on Biodiesel Oxidation Stability Promoted by Binary and Ternary Blends Containing Multifunctional Additives
title_full An Analytical Evaluation of the Synergistic Effect on Biodiesel Oxidation Stability Promoted by Binary and Ternary Blends Containing Multifunctional Additives
title_fullStr An Analytical Evaluation of the Synergistic Effect on Biodiesel Oxidation Stability Promoted by Binary and Ternary Blends Containing Multifunctional Additives
title_full_unstemmed An Analytical Evaluation of the Synergistic Effect on Biodiesel Oxidation Stability Promoted by Binary and Ternary Blends Containing Multifunctional Additives
title_short An Analytical Evaluation of the Synergistic Effect on Biodiesel Oxidation Stability Promoted by Binary and Ternary Blends Containing Multifunctional Additives
title_sort analytical evaluation of the synergistic effect on biodiesel oxidation stability promoted by binary and ternary blends containing multifunctional additives
url http://dx.doi.org/10.1155/2019/6467183
work_keys_str_mv AT silviasyahagi ananalyticalevaluationofthesynergisticeffectonbiodieseloxidationstabilitypromotedbybinaryandternaryblendscontainingmultifunctionaladditives
AT anacroveda ananalyticalevaluationofthesynergisticeffectonbiodieseloxidationstabilitypromotedbybinaryandternaryblendscontainingmultifunctionaladditives
AT adriellitsobral ananalyticalevaluationofthesynergisticeffectonbiodieseloxidationstabilitypromotedbybinaryandternaryblendscontainingmultifunctionaladditives
AT ivanpoliveira ananalyticalevaluationofthesynergisticeffectonbiodieseloxidationstabilitypromotedbybinaryandternaryblendscontainingmultifunctionaladditives
AT andersonrlcaires ananalyticalevaluationofthesynergisticeffectonbiodieseloxidationstabilitypromotedbybinaryandternaryblendscontainingmultifunctionaladditives
AT robertosgomes ananalyticalevaluationofthesynergisticeffectonbiodieseloxidationstabilitypromotedbybinaryandternaryblendscontainingmultifunctionaladditives
AT magnoagtrindade ananalyticalevaluationofthesynergisticeffectonbiodieseloxidationstabilitypromotedbybinaryandternaryblendscontainingmultifunctionaladditives
AT silviasyahagi analyticalevaluationofthesynergisticeffectonbiodieseloxidationstabilitypromotedbybinaryandternaryblendscontainingmultifunctionaladditives
AT anacroveda analyticalevaluationofthesynergisticeffectonbiodieseloxidationstabilitypromotedbybinaryandternaryblendscontainingmultifunctionaladditives
AT adriellitsobral analyticalevaluationofthesynergisticeffectonbiodieseloxidationstabilitypromotedbybinaryandternaryblendscontainingmultifunctionaladditives
AT ivanpoliveira analyticalevaluationofthesynergisticeffectonbiodieseloxidationstabilitypromotedbybinaryandternaryblendscontainingmultifunctionaladditives
AT andersonrlcaires analyticalevaluationofthesynergisticeffectonbiodieseloxidationstabilitypromotedbybinaryandternaryblendscontainingmultifunctionaladditives
AT robertosgomes analyticalevaluationofthesynergisticeffectonbiodieseloxidationstabilitypromotedbybinaryandternaryblendscontainingmultifunctionaladditives
AT magnoagtrindade analyticalevaluationofthesynergisticeffectonbiodieseloxidationstabilitypromotedbybinaryandternaryblendscontainingmultifunctionaladditives