Dynamic changes in aroma of large-leaf yellow tea during the whole processing at an industrial scale: From fresh leaf to finished tea

Large-leaf yellow tea (LYT) is a yellow tea product with a specific aroma characteristic and the flavor code has recently been revealed. To elucidate the transformation of odorants from fresh leaves to finished LYT, this study tracked dynamic changes in aroma compounds throughout an industrial-scale...

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Main Authors: Jing Wang, Yuemeng Hu, Zhenyu Guan, Ronggang Zhai, Jieyao Yu, Marina Rigling, Yanyan Zhang, Xiaochun Wan, Xiaoting Zhai
Format: Article
Language:English
Published: Elsevier 2025-05-01
Series:Food Chemistry: X
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Online Access:http://www.sciencedirect.com/science/article/pii/S2590157525004754
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author Jing Wang
Yuemeng Hu
Zhenyu Guan
Ronggang Zhai
Jieyao Yu
Marina Rigling
Yanyan Zhang
Xiaochun Wan
Xiaoting Zhai
author_facet Jing Wang
Yuemeng Hu
Zhenyu Guan
Ronggang Zhai
Jieyao Yu
Marina Rigling
Yanyan Zhang
Xiaochun Wan
Xiaoting Zhai
author_sort Jing Wang
collection DOAJ
description Large-leaf yellow tea (LYT) is a yellow tea product with a specific aroma characteristic and the flavor code has recently been revealed. To elucidate the transformation of odorants from fresh leaves to finished LYT, this study tracked dynamic changes in aroma compounds throughout an industrial-scale experiment. The odorants' contributions of each step were evaluated by stable isotope dilution assays, internal standard method, and odor activity values. Among 39 quantitated odorants, the loss of top-note compounds such as dimethyl sulfide, 2-/3-methylbutanal, and 2-methylpropanal during yellowing was compensated during roasting. In contrast, floral compounds like geraniol and linalool declined progressively, while pyrazines were mainly generated during the final roasting and increased with roasting intensity. Therefore, yellowing and roasting steps were identified as key processes influencing LYT aroma formation, and the roasting degree significantly influenced the final aroma profile. These findings provide a mechanistic understanding of aroma development in LYT and offer practical guidance for optimizing processing parameters to tailor flavor profiles.
format Article
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institution Kabale University
issn 2590-1575
language English
publishDate 2025-05-01
publisher Elsevier
record_format Article
series Food Chemistry: X
spelling doaj-art-96790d8f00534b9ab5479b0581dca7fa2025-08-20T03:26:39ZengElsevierFood Chemistry: X2590-15752025-05-012810262810.1016/j.fochx.2025.102628Dynamic changes in aroma of large-leaf yellow tea during the whole processing at an industrial scale: From fresh leaf to finished teaJing Wang0Yuemeng Hu1Zhenyu Guan2Ronggang Zhai3Jieyao Yu4Marina Rigling5Yanyan Zhang6Xiaochun Wan7Xiaoting Zhai8National Key Laboratory for Tea Plant Germplasm Innovation and Resource Utilization, Anhui Agricultural University, Hefei 230036, China; International Joint Laboratory on Tea Chemistry and Health Effects of Ministry of Education, Anhui Agricultural University, Hefei 230036, China; Key Laboratory of Tea Science of Ministry of Education, Hunan Agricultural University, Changsha 410128, ChinaNational Key Laboratory for Tea Plant Germplasm Innovation and Resource Utilization, Anhui Agricultural University, Hefei 230036, China; International Joint Laboratory on Tea Chemistry and Health Effects of Ministry of Education, Anhui Agricultural University, Hefei 230036, ChinaNational Key Laboratory for Tea Plant Germplasm Innovation and Resource Utilization, Anhui Agricultural University, Hefei 230036, China; International Joint Laboratory on Tea Chemistry and Health Effects of Ministry of Education, Anhui Agricultural University, Hefei 230036, ChinaCollege of Electronics and Information Engineering, Anhui Institute of Post and Telecommunications Vocational and Technical College, Anhui Hefei, 230031, ChinaNational Key Laboratory for Tea Plant Germplasm Innovation and Resource Utilization, Anhui Agricultural University, Hefei 230036, China; International Joint Laboratory on Tea Chemistry and Health Effects of Ministry of Education, Anhui Agricultural University, Hefei 230036, China; School of Chemical Sciences, University of Auckland, Auckland 1010, New ZealandDepartment of Flavor Chemistry, University of Hohenheim, 70599 Stuttgart, GermanyDepartment of Flavor Chemistry, University of Hohenheim, 70599 Stuttgart, GermanyNational Key Laboratory for Tea Plant Germplasm Innovation and Resource Utilization, Anhui Agricultural University, Hefei 230036, China; International Joint Laboratory on Tea Chemistry and Health Effects of Ministry of Education, Anhui Agricultural University, Hefei 230036, China; Corresponding author at: National Key Laboratory for Tea Plant Germplasm Innovation and Resource Utilization, Anhui Agricultural University, 130 Changjiang West Road, Hefei, Anhui 230036, China.National Key Laboratory for Tea Plant Germplasm Innovation and Resource Utilization, Anhui Agricultural University, Hefei 230036, China; International Joint Laboratory on Tea Chemistry and Health Effects of Ministry of Education, Anhui Agricultural University, Hefei 230036, China; Corresponding author at: National Key Laboratory for Tea Plant Germplasm Innovation and Resource Utilization, Anhui Agricultural University, 130 Changjiang West Road, Hefei, Anhui 230036, China.Large-leaf yellow tea (LYT) is a yellow tea product with a specific aroma characteristic and the flavor code has recently been revealed. To elucidate the transformation of odorants from fresh leaves to finished LYT, this study tracked dynamic changes in aroma compounds throughout an industrial-scale experiment. The odorants' contributions of each step were evaluated by stable isotope dilution assays, internal standard method, and odor activity values. Among 39 quantitated odorants, the loss of top-note compounds such as dimethyl sulfide, 2-/3-methylbutanal, and 2-methylpropanal during yellowing was compensated during roasting. In contrast, floral compounds like geraniol and linalool declined progressively, while pyrazines were mainly generated during the final roasting and increased with roasting intensity. Therefore, yellowing and roasting steps were identified as key processes influencing LYT aroma formation, and the roasting degree significantly influenced the final aroma profile. These findings provide a mechanistic understanding of aroma development in LYT and offer practical guidance for optimizing processing parameters to tailor flavor profiles.http://www.sciencedirect.com/science/article/pii/S2590157525004754Large-leaf yellow teaCharacteristic aromaAroma dynamic changeYellowingRoasting
spellingShingle Jing Wang
Yuemeng Hu
Zhenyu Guan
Ronggang Zhai
Jieyao Yu
Marina Rigling
Yanyan Zhang
Xiaochun Wan
Xiaoting Zhai
Dynamic changes in aroma of large-leaf yellow tea during the whole processing at an industrial scale: From fresh leaf to finished tea
Food Chemistry: X
Large-leaf yellow tea
Characteristic aroma
Aroma dynamic change
Yellowing
Roasting
title Dynamic changes in aroma of large-leaf yellow tea during the whole processing at an industrial scale: From fresh leaf to finished tea
title_full Dynamic changes in aroma of large-leaf yellow tea during the whole processing at an industrial scale: From fresh leaf to finished tea
title_fullStr Dynamic changes in aroma of large-leaf yellow tea during the whole processing at an industrial scale: From fresh leaf to finished tea
title_full_unstemmed Dynamic changes in aroma of large-leaf yellow tea during the whole processing at an industrial scale: From fresh leaf to finished tea
title_short Dynamic changes in aroma of large-leaf yellow tea during the whole processing at an industrial scale: From fresh leaf to finished tea
title_sort dynamic changes in aroma of large leaf yellow tea during the whole processing at an industrial scale from fresh leaf to finished tea
topic Large-leaf yellow tea
Characteristic aroma
Aroma dynamic change
Yellowing
Roasting
url http://www.sciencedirect.com/science/article/pii/S2590157525004754
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