Space charge characteristics and dielectric properties of PANI/PP‐g‐MAH/PP ternary composite

Abstract Space charge accumulation in polypropylene materials for direct current capacitor will accelerate the ageing of the materials, resulting in the degradation of their insulation properties. Besides, it will also affect the dielectric properties of the capacitor in a long term. In this paper,...

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Main Authors: Guochang Li, Tianzhen Liu, Zhenlu Gu, Xiaolong Chen, Beibei Sun, Yuanwei Zhu, Shengtao Li, Yanhui Wei
Format: Article
Language:English
Published: Wiley 2025-02-01
Series:High Voltage
Online Access:https://doi.org/10.1049/hve2.12497
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author Guochang Li
Tianzhen Liu
Zhenlu Gu
Xiaolong Chen
Beibei Sun
Yuanwei Zhu
Shengtao Li
Yanhui Wei
author_facet Guochang Li
Tianzhen Liu
Zhenlu Gu
Xiaolong Chen
Beibei Sun
Yuanwei Zhu
Shengtao Li
Yanhui Wei
author_sort Guochang Li
collection DOAJ
description Abstract Space charge accumulation in polypropylene materials for direct current capacitor will accelerate the ageing of the materials, resulting in the degradation of their insulation properties. Besides, it will also affect the dielectric properties of the capacitor in a long term. In this paper, a ternary composite of polyaniline (PANI)/maleic anhydride functionalised PP (PP‐g‐MAH)/polypropylene (PP) based on the PANI@ dopamine (PDA) coating structure is constructed from two perspectives of PP matrix grafting and PANI nano particle. This method takes advantage of the high permittivity and good compatibility of PANI to improve the relative dielectric constant of the composite while introducing deep traps inside the composite to inhibit space charge accumulation coating. The experimental results show that with the increase in PANI content, the maximum relative permittivity can be increased by 62%. The addition of the appropriate amount of PANI can effectively inhibit the space charge accumulation. The relative dielectric constant of the composite decreases significantly due to the heteropolar space charge. The relative dielectric constant of the modified polyaniline composites decreased significantly. The reduction rate decreased from 38% before modification to 12% after modification. This work has certain guiding significance for solving space charge problem of direct current capacitor.
format Article
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institution DOAJ
issn 2397-7264
language English
publishDate 2025-02-01
publisher Wiley
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series High Voltage
spelling doaj-art-95df05bfa3fd4ec8aebb49ae816496702025-08-20T03:00:09ZengWileyHigh Voltage2397-72642025-02-0110117818510.1049/hve2.12497Space charge characteristics and dielectric properties of PANI/PP‐g‐MAH/PP ternary compositeGuochang Li0Tianzhen Liu1Zhenlu Gu2Xiaolong Chen3Beibei Sun4Yuanwei Zhu5Shengtao Li6Yanhui Wei7College of Materials Science and Engineering Qingdao University of Science and Technology Qingdao ChinaCollege of Materials Science and Engineering Qingdao University of Science and Technology Qingdao ChinaCollege of Materials Science and Engineering Qingdao University of Science and Technology Qingdao ChinaCollege of Materials Science and Engineering Qingdao University of Science and Technology Qingdao ChinaCollege of Materials Science and Engineering Qingdao University of Science and Technology Qingdao ChinaState Key Laboratory of Electrical Insulation and Power Equipment Xi'an Jiaotong University Xi'an ChinaState Key Laboratory of Electrical Insulation and Power Equipment Xi'an Jiaotong University Xi'an ChinaCollege of Materials Science and Engineering Qingdao University of Science and Technology Qingdao ChinaAbstract Space charge accumulation in polypropylene materials for direct current capacitor will accelerate the ageing of the materials, resulting in the degradation of their insulation properties. Besides, it will also affect the dielectric properties of the capacitor in a long term. In this paper, a ternary composite of polyaniline (PANI)/maleic anhydride functionalised PP (PP‐g‐MAH)/polypropylene (PP) based on the PANI@ dopamine (PDA) coating structure is constructed from two perspectives of PP matrix grafting and PANI nano particle. This method takes advantage of the high permittivity and good compatibility of PANI to improve the relative dielectric constant of the composite while introducing deep traps inside the composite to inhibit space charge accumulation coating. The experimental results show that with the increase in PANI content, the maximum relative permittivity can be increased by 62%. The addition of the appropriate amount of PANI can effectively inhibit the space charge accumulation. The relative dielectric constant of the composite decreases significantly due to the heteropolar space charge. The relative dielectric constant of the modified polyaniline composites decreased significantly. The reduction rate decreased from 38% before modification to 12% after modification. This work has certain guiding significance for solving space charge problem of direct current capacitor.https://doi.org/10.1049/hve2.12497
spellingShingle Guochang Li
Tianzhen Liu
Zhenlu Gu
Xiaolong Chen
Beibei Sun
Yuanwei Zhu
Shengtao Li
Yanhui Wei
Space charge characteristics and dielectric properties of PANI/PP‐g‐MAH/PP ternary composite
High Voltage
title Space charge characteristics and dielectric properties of PANI/PP‐g‐MAH/PP ternary composite
title_full Space charge characteristics and dielectric properties of PANI/PP‐g‐MAH/PP ternary composite
title_fullStr Space charge characteristics and dielectric properties of PANI/PP‐g‐MAH/PP ternary composite
title_full_unstemmed Space charge characteristics and dielectric properties of PANI/PP‐g‐MAH/PP ternary composite
title_short Space charge characteristics and dielectric properties of PANI/PP‐g‐MAH/PP ternary composite
title_sort space charge characteristics and dielectric properties of pani pp g mah pp ternary composite
url https://doi.org/10.1049/hve2.12497
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