Effect of anionic polyelectrolytes on formation of hydroxyapatite particles in simulated body fluids

Recently, fabrication of organic-inorganic hybrid biomedical materials using biomimetic mineralization processes has received attention because it proceeds under mild conditions and biocompatible inorganic components are incorporated in the resulting hybrids. In the present study, the preparation of...

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Main Authors: Takuya Sagawa, Noritaka Kako, Masatoshi Nakaya, Takaaki Izumi, Kosuke Takeda, Kazutoshi Iijima, Mineo Hashizume
Format: Article
Language:English
Published: Taylor & Francis Group 2024-12-01
Series:Journal of Asian Ceramic Societies
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Online Access:https://www.tandfonline.com/doi/10.1080/21870764.2024.2445444
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author Takuya Sagawa
Noritaka Kako
Masatoshi Nakaya
Takaaki Izumi
Kosuke Takeda
Kazutoshi Iijima
Mineo Hashizume
author_facet Takuya Sagawa
Noritaka Kako
Masatoshi Nakaya
Takaaki Izumi
Kosuke Takeda
Kazutoshi Iijima
Mineo Hashizume
author_sort Takuya Sagawa
collection DOAJ
description Recently, fabrication of organic-inorganic hybrid biomedical materials using biomimetic mineralization processes has received attention because it proceeds under mild conditions and biocompatible inorganic components are incorporated in the resulting hybrids. In the present study, the preparation of anionic polyelectrolyte-apatite hybrids, having potential as a biomedical material, in simulated body fluids (SBFs) was performed. Anionic polyelectrolytes such as heparin, poly(4-styrene sulfonate) (PSS), or poly(vinyl sulfate) (PVS) were added to SBFs and incubated to induce nucleation of hydroxyapatite, which resulted in the formation of anionic polyelectrolyte-apatite hybrids. Physical characterization of the resulting deposits in SBFs using scanning electron microscopy (SEM), energy-dispersive X-ray spectroscopy (EDX), FT-IR spectroscopy, and X-ray diffraction (XRD) revealed that the polyelectrolyte concentration affected the yield of the resulting deposits. It seemed that the reaction condition affected the apatite nucleation process in SBFs. Effect of chemical structures and concentrations of anionic polyelectrolytes on hybrid formation is discussed.
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institution OA Journals
issn 2187-0764
language English
publishDate 2024-12-01
publisher Taylor & Francis Group
record_format Article
series Journal of Asian Ceramic Societies
spelling doaj-art-958ab9ad0ac44e1cad075abe0f116cd62025-08-20T02:32:00ZengTaylor & Francis GroupJournal of Asian Ceramic Societies2187-07642024-12-011910.1080/21870764.2024.2445444Effect of anionic polyelectrolytes on formation of hydroxyapatite particles in simulated body fluidsTakuya Sagawa0Noritaka Kako1Masatoshi Nakaya2Takaaki Izumi3Kosuke Takeda4Kazutoshi Iijima5Mineo Hashizume6Department of Industrial Chemistry, Faculty of Engineering, Tokyo University of Science, Katsushika-ku, Tokyo, JapanDepartment of Industrial Chemistry, Faculty of Engineering, Tokyo University of Science, Katsushika-ku, Tokyo, JapanDepartment of Industrial Chemistry, Faculty of Engineering, Tokyo University of Science, Katsushika-ku, Tokyo, JapanDepartment of Industrial Chemistry, Faculty of Engineering, Tokyo University of Science, Katsushika-ku, Tokyo, JapanDepartment of Industrial Chemistry, Faculty of Engineering, Tokyo University of Science, Katsushika-ku, Tokyo, JapanDepartment of Industrial Chemistry, Faculty of Engineering, Tokyo University of Science, Katsushika-ku, Tokyo, JapanDepartment of Industrial Chemistry, Faculty of Engineering, Tokyo University of Science, Katsushika-ku, Tokyo, JapanRecently, fabrication of organic-inorganic hybrid biomedical materials using biomimetic mineralization processes has received attention because it proceeds under mild conditions and biocompatible inorganic components are incorporated in the resulting hybrids. In the present study, the preparation of anionic polyelectrolyte-apatite hybrids, having potential as a biomedical material, in simulated body fluids (SBFs) was performed. Anionic polyelectrolytes such as heparin, poly(4-styrene sulfonate) (PSS), or poly(vinyl sulfate) (PVS) were added to SBFs and incubated to induce nucleation of hydroxyapatite, which resulted in the formation of anionic polyelectrolyte-apatite hybrids. Physical characterization of the resulting deposits in SBFs using scanning electron microscopy (SEM), energy-dispersive X-ray spectroscopy (EDX), FT-IR spectroscopy, and X-ray diffraction (XRD) revealed that the polyelectrolyte concentration affected the yield of the resulting deposits. It seemed that the reaction condition affected the apatite nucleation process in SBFs. Effect of chemical structures and concentrations of anionic polyelectrolytes on hybrid formation is discussed.https://www.tandfonline.com/doi/10.1080/21870764.2024.2445444HydroxyapatiteAnionic polyelectrolyteSimulated body fluidOrganic-inorganic hybrid
spellingShingle Takuya Sagawa
Noritaka Kako
Masatoshi Nakaya
Takaaki Izumi
Kosuke Takeda
Kazutoshi Iijima
Mineo Hashizume
Effect of anionic polyelectrolytes on formation of hydroxyapatite particles in simulated body fluids
Journal of Asian Ceramic Societies
Hydroxyapatite
Anionic polyelectrolyte
Simulated body fluid
Organic-inorganic hybrid
title Effect of anionic polyelectrolytes on formation of hydroxyapatite particles in simulated body fluids
title_full Effect of anionic polyelectrolytes on formation of hydroxyapatite particles in simulated body fluids
title_fullStr Effect of anionic polyelectrolytes on formation of hydroxyapatite particles in simulated body fluids
title_full_unstemmed Effect of anionic polyelectrolytes on formation of hydroxyapatite particles in simulated body fluids
title_short Effect of anionic polyelectrolytes on formation of hydroxyapatite particles in simulated body fluids
title_sort effect of anionic polyelectrolytes on formation of hydroxyapatite particles in simulated body fluids
topic Hydroxyapatite
Anionic polyelectrolyte
Simulated body fluid
Organic-inorganic hybrid
url https://www.tandfonline.com/doi/10.1080/21870764.2024.2445444
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