Enzyme-Based Solid-Phase Electrochemiluminescence Sensors with Stable, Anchored Emitters for Sensitive Glucose Detection

Glucose (Glu) detection, as a fundamental analytical technique, has applications in medical diagnostics, clinical testing, bioanalysis and environmental monitoring. In this work, a solid-phase electrochemiluminescence (ECL) enzyme sensor was developed by immobilizing the ECL emitter in a stable mann...

Full description

Saved in:
Bibliographic Details
Main Authors: Chunyin Wei, Yanyan Zheng, Fei Yan, Lifang Xu
Format: Article
Language:English
Published: MDPI AG 2025-05-01
Series:Biosensors
Subjects:
Online Access:https://www.mdpi.com/2079-6374/15/5/332
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1850127393888403456
author Chunyin Wei
Yanyan Zheng
Fei Yan
Lifang Xu
author_facet Chunyin Wei
Yanyan Zheng
Fei Yan
Lifang Xu
author_sort Chunyin Wei
collection DOAJ
description Glucose (Glu) detection, as a fundamental analytical technique, has applications in medical diagnostics, clinical testing, bioanalysis and environmental monitoring. In this work, a solid-phase electrochemiluminescence (ECL) enzyme sensor was developed by immobilizing the ECL emitter in a stable manner within bipolar silica nanochannel array film (bp-SNA), enabling sensitive glucose detection. The sensor was constructed using an electrochemical-assisted self-assembly (EASA) method with various siloxane precursors to quickly modify the surface of indium tin oxide (ITO) electrodes with a bilayer SNA of different charge properties. The inner layer, including negatively charged SNA (n-SNA), attracted the positively charged ECL emitter tris(2,2′-bipyridyl)ruthenium(II) (Ru(bpy)<sub>3</sub><sup>2+</sup>) via electrostatic interaction, while the outer layer, including positively charged SNA (p-SNA), repelled it, forming a barrier that efficiently concentrated the Ru(bpy)<sub>3</sub><sup>2+</sup> emitter in a stable manner. After modifying the amine groups on the p-SNA surface with aldehyde groups, glucose oxidase (GOx) was covalently immobilized, forming the enzyme electrode. In the presence of glucose, GOx catalyzed the conversion of glucose to hydrogen peroxide (H<sub>2</sub>O<sub>2</sub>), which acted as a quencher for the Ru(bpy)<sub>3</sub><sup>2+</sup>/triethanolamine (TPA) system, reducing the ECL signal and enabling quantitative glucose analysis. The sensor exhibited a wide linear range from 10 μM to 7.0 mM and a limit of detection (LOD) of 1 μM (S/N = 3). Glucose detection in fetal bovine serum was realized. By replacing the enzyme type on the electrode surface, this sensing strategy holds the potential to provide a universal platform for the detection of different metabolites.
format Article
id doaj-art-93bb91ada4f147a3a93bb83e81e6420f
institution OA Journals
issn 2079-6374
language English
publishDate 2025-05-01
publisher MDPI AG
record_format Article
series Biosensors
spelling doaj-art-93bb91ada4f147a3a93bb83e81e6420f2025-08-20T02:33:40ZengMDPI AGBiosensors2079-63742025-05-0115533210.3390/bios15050332Enzyme-Based Solid-Phase Electrochemiluminescence Sensors with Stable, Anchored Emitters for Sensitive Glucose DetectionChunyin Wei0Yanyan Zheng1Fei Yan2Lifang Xu3Guangxi Medical University Cancer Hospital, Guangxi Medical University, Nanning 530021, ChinaSchool of Chemistry and Chemical Engineering, Zhejiang Sci-Tech University, Hangzhou 310018, ChinaSchool of Chemistry and Chemical Engineering, Zhejiang Sci-Tech University, Hangzhou 310018, ChinaThe Second Affiliated Hospital of Guangxi Medical University, Nanning 530007, ChinaGlucose (Glu) detection, as a fundamental analytical technique, has applications in medical diagnostics, clinical testing, bioanalysis and environmental monitoring. In this work, a solid-phase electrochemiluminescence (ECL) enzyme sensor was developed by immobilizing the ECL emitter in a stable manner within bipolar silica nanochannel array film (bp-SNA), enabling sensitive glucose detection. The sensor was constructed using an electrochemical-assisted self-assembly (EASA) method with various siloxane precursors to quickly modify the surface of indium tin oxide (ITO) electrodes with a bilayer SNA of different charge properties. The inner layer, including negatively charged SNA (n-SNA), attracted the positively charged ECL emitter tris(2,2′-bipyridyl)ruthenium(II) (Ru(bpy)<sub>3</sub><sup>2+</sup>) via electrostatic interaction, while the outer layer, including positively charged SNA (p-SNA), repelled it, forming a barrier that efficiently concentrated the Ru(bpy)<sub>3</sub><sup>2+</sup> emitter in a stable manner. After modifying the amine groups on the p-SNA surface with aldehyde groups, glucose oxidase (GOx) was covalently immobilized, forming the enzyme electrode. In the presence of glucose, GOx catalyzed the conversion of glucose to hydrogen peroxide (H<sub>2</sub>O<sub>2</sub>), which acted as a quencher for the Ru(bpy)<sub>3</sub><sup>2+</sup>/triethanolamine (TPA) system, reducing the ECL signal and enabling quantitative glucose analysis. The sensor exhibited a wide linear range from 10 μM to 7.0 mM and a limit of detection (LOD) of 1 μM (S/N = 3). Glucose detection in fetal bovine serum was realized. By replacing the enzyme type on the electrode surface, this sensing strategy holds the potential to provide a universal platform for the detection of different metabolites.https://www.mdpi.com/2079-6374/15/5/332enzyme sensorelectrochemiluminescenceimmobilized emitternanochannel arrayglucose
spellingShingle Chunyin Wei
Yanyan Zheng
Fei Yan
Lifang Xu
Enzyme-Based Solid-Phase Electrochemiluminescence Sensors with Stable, Anchored Emitters for Sensitive Glucose Detection
Biosensors
enzyme sensor
electrochemiluminescence
immobilized emitter
nanochannel array
glucose
title Enzyme-Based Solid-Phase Electrochemiluminescence Sensors with Stable, Anchored Emitters for Sensitive Glucose Detection
title_full Enzyme-Based Solid-Phase Electrochemiluminescence Sensors with Stable, Anchored Emitters for Sensitive Glucose Detection
title_fullStr Enzyme-Based Solid-Phase Electrochemiluminescence Sensors with Stable, Anchored Emitters for Sensitive Glucose Detection
title_full_unstemmed Enzyme-Based Solid-Phase Electrochemiluminescence Sensors with Stable, Anchored Emitters for Sensitive Glucose Detection
title_short Enzyme-Based Solid-Phase Electrochemiluminescence Sensors with Stable, Anchored Emitters for Sensitive Glucose Detection
title_sort enzyme based solid phase electrochemiluminescence sensors with stable anchored emitters for sensitive glucose detection
topic enzyme sensor
electrochemiluminescence
immobilized emitter
nanochannel array
glucose
url https://www.mdpi.com/2079-6374/15/5/332
work_keys_str_mv AT chunyinwei enzymebasedsolidphaseelectrochemiluminescencesensorswithstableanchoredemittersforsensitiveglucosedetection
AT yanyanzheng enzymebasedsolidphaseelectrochemiluminescencesensorswithstableanchoredemittersforsensitiveglucosedetection
AT feiyan enzymebasedsolidphaseelectrochemiluminescencesensorswithstableanchoredemittersforsensitiveglucosedetection
AT lifangxu enzymebasedsolidphaseelectrochemiluminescencesensorswithstableanchoredemittersforsensitiveglucosedetection