Structure of bifunctional variediene synthase yields unique insight on biosynthetic diterpene assembly and cyclization

Abstract An unusual family of bifunctional terpene synthases has been identified in which a prenyltransferase assembles 5-carbon precursors to form C20 geranylgeranyl diphosphate (GGPP), which is then converted into a polycyclic product by a cyclase. Here, we report the cryo-EM structure of a massiv...

Full description

Saved in:
Bibliographic Details
Main Authors: Eliott S. Wenger, David W. Christianson
Format: Article
Language:English
Published: Nature Portfolio 2025-06-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-025-60537-3
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1849434289743069184
author Eliott S. Wenger
David W. Christianson
author_facet Eliott S. Wenger
David W. Christianson
author_sort Eliott S. Wenger
collection DOAJ
description Abstract An unusual family of bifunctional terpene synthases has been identified in which a prenyltransferase assembles 5-carbon precursors to form C20 geranylgeranyl diphosphate (GGPP), which is then converted into a polycyclic product by a cyclase. Here, we report the cryo-EM structure of a massive, 495-kD bifunctional terpene synthase, variediene synthase from Emericella variecolor (EvVS). The structure reveals a hexameric prenyltransferase core sandwiched between two triads of cyclases. Surprisingly, GGPP is not channeled intramolecularly from the prenyltransferase to the cyclase, but instead is channeled intermolecularly to a non-native cyclase as indicated by substrate competition experiments. These results inform our understanding of carbon management in the greater family of bifunctional terpene synthases, hundreds of which have been identified in fungi. Using sequence similarity networks, we also report the identification of bifunctional terpene synthases in an animal, Adineta steineri, a bdelloid rotifer indigenous to freshwater environments.
format Article
id doaj-art-93b98a8d69a741708533534fa65ffb69
institution Kabale University
issn 2041-1723
language English
publishDate 2025-06-01
publisher Nature Portfolio
record_format Article
series Nature Communications
spelling doaj-art-93b98a8d69a741708533534fa65ffb692025-08-20T03:26:43ZengNature PortfolioNature Communications2041-17232025-06-0116111210.1038/s41467-025-60537-3Structure of bifunctional variediene synthase yields unique insight on biosynthetic diterpene assembly and cyclizationEliott S. Wenger0David W. Christianson1Department of Chemistry, Roy and Diana Vagelos Laboratories, University of PennsylvaniaDepartment of Chemistry, Roy and Diana Vagelos Laboratories, University of PennsylvaniaAbstract An unusual family of bifunctional terpene synthases has been identified in which a prenyltransferase assembles 5-carbon precursors to form C20 geranylgeranyl diphosphate (GGPP), which is then converted into a polycyclic product by a cyclase. Here, we report the cryo-EM structure of a massive, 495-kD bifunctional terpene synthase, variediene synthase from Emericella variecolor (EvVS). The structure reveals a hexameric prenyltransferase core sandwiched between two triads of cyclases. Surprisingly, GGPP is not channeled intramolecularly from the prenyltransferase to the cyclase, but instead is channeled intermolecularly to a non-native cyclase as indicated by substrate competition experiments. These results inform our understanding of carbon management in the greater family of bifunctional terpene synthases, hundreds of which have been identified in fungi. Using sequence similarity networks, we also report the identification of bifunctional terpene synthases in an animal, Adineta steineri, a bdelloid rotifer indigenous to freshwater environments.https://doi.org/10.1038/s41467-025-60537-3
spellingShingle Eliott S. Wenger
David W. Christianson
Structure of bifunctional variediene synthase yields unique insight on biosynthetic diterpene assembly and cyclization
Nature Communications
title Structure of bifunctional variediene synthase yields unique insight on biosynthetic diterpene assembly and cyclization
title_full Structure of bifunctional variediene synthase yields unique insight on biosynthetic diterpene assembly and cyclization
title_fullStr Structure of bifunctional variediene synthase yields unique insight on biosynthetic diterpene assembly and cyclization
title_full_unstemmed Structure of bifunctional variediene synthase yields unique insight on biosynthetic diterpene assembly and cyclization
title_short Structure of bifunctional variediene synthase yields unique insight on biosynthetic diterpene assembly and cyclization
title_sort structure of bifunctional variediene synthase yields unique insight on biosynthetic diterpene assembly and cyclization
url https://doi.org/10.1038/s41467-025-60537-3
work_keys_str_mv AT eliottswenger structureofbifunctionalvariedienesynthaseyieldsuniqueinsightonbiosyntheticditerpeneassemblyandcyclization
AT davidwchristianson structureofbifunctionalvariedienesynthaseyieldsuniqueinsightonbiosyntheticditerpeneassemblyandcyclization