Review on migration and entrapment of light nonaqueous phase liquids ‎in the subsurface environment

Groundwater contamination by Light Non-aqueous Phase liquids‎ (LNAPLs) has attracted ‎massive research attention over the past decades to ensure a safe environment for living beings. The knowledge of LNAPL distribution and entrapment in the subsurface environment is still scattered, preventing a cle...

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Main Authors: Doaa F. Almaliki, Harris Ramli, Ali Zaiter, Ishmail Sheriff
Format: Article
Language:English
Published: Elsevier 2025-04-01
Series:Desalination and Water Treatment
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Online Access:http://www.sciencedirect.com/science/article/pii/S1944398625001110
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author Doaa F. Almaliki
Harris Ramli
Ali Zaiter
Ishmail Sheriff
author_facet Doaa F. Almaliki
Harris Ramli
Ali Zaiter
Ishmail Sheriff
author_sort Doaa F. Almaliki
collection DOAJ
description Groundwater contamination by Light Non-aqueous Phase liquids‎ (LNAPLs) has attracted ‎massive research attention over the past decades to ensure a safe environment for living beings. The knowledge of LNAPL distribution and entrapment in the subsurface environment is still scattered, preventing a clear view of the occurring processes. This review discusses ‎the effect of (1) groundwater table fluctuation, (2) sand arrangement and particle size, and (3) spilled LNAPL volume on LNAPL behavior and entrapment in ‎the subsurface. From the available literature, changes in the groundwater table increase LNAPL entrapment in the initial wet soil conditions by ‎over 130 % and reduce trapped LNAPL in saturated soil by 101.65 % promoting the ‎contaminant loss through enhanced dissolution and degradation in the unsaturated zone. ‎Researchers have investigated LNAPL movement in layered heterogeneous sand to ‎understand the effects of local low permeability on the contaminant ‎velocities. It showed that LNAPL displacement was 20.78 %, 20.5 %, and 10 % in the coarse, ‎medium, and fine sand, respectively. An increasing LNAPL volume with consistent ‎groundwater fluctuations has a limited impact on LNAPL behavior, although a higher LNAPL ‎spill volume can notably depress the capillary fringe. The influence of the three studied factors on ‎the migration and transformation of pollutants, however, remains uncertain, which necessitates further studies on the migration and entrapment of LNAPL in the capillary fringe ‎zone to mitigate LNAPL contamination in the saturated zone. ‎Additionally, future studies should investigate the LNAPL migration in double ‎porous soil and multiple LNAPL injections under groundwater fluctuation.‎ A deeper understanding of these factors is essential for developing predictive models and effective remediation techniques to mitigate groundwater contamination. This review serves as a foundation for future research, guiding efforts toward sustainable contamination management strategies.
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spelling doaj-art-93b3a3a6e7f5437caa5fde17a38ee4932025-08-20T02:32:30ZengElsevierDesalination and Water Treatment1944-39862025-04-0132210109510.1016/j.dwt.2025.101095Review on migration and entrapment of light nonaqueous phase liquids ‎in the subsurface environmentDoaa F. Almaliki0Harris Ramli1Ali Zaiter2Ishmail Sheriff3School of Civil Engineering, Engineering Campus, Universiti Sains Malaysia, 14300 Nibong Tebal, Pulau Pinang, Malaysia; Environment and Pollution Engineering Department, Basrah Engineering Technical College, Southern Technical University, Alzybair Street, Basrah, IraqSchool of Civil Engineering, Engineering Campus, Universiti Sains Malaysia, 14300 Nibong Tebal, Pulau Pinang, Malaysia; Corresponding author.School of Civil Engineering, Engineering Campus, Universiti Sains Malaysia, 14300 Nibong Tebal, Pulau Pinang, MalaysiaSchool of Civil Engineering, Engineering Campus, Universiti Sains Malaysia, 14300 Nibong Tebal, Pulau Pinang, MalaysiaGroundwater contamination by Light Non-aqueous Phase liquids‎ (LNAPLs) has attracted ‎massive research attention over the past decades to ensure a safe environment for living beings. The knowledge of LNAPL distribution and entrapment in the subsurface environment is still scattered, preventing a clear view of the occurring processes. This review discusses ‎the effect of (1) groundwater table fluctuation, (2) sand arrangement and particle size, and (3) spilled LNAPL volume on LNAPL behavior and entrapment in ‎the subsurface. From the available literature, changes in the groundwater table increase LNAPL entrapment in the initial wet soil conditions by ‎over 130 % and reduce trapped LNAPL in saturated soil by 101.65 % promoting the ‎contaminant loss through enhanced dissolution and degradation in the unsaturated zone. ‎Researchers have investigated LNAPL movement in layered heterogeneous sand to ‎understand the effects of local low permeability on the contaminant ‎velocities. It showed that LNAPL displacement was 20.78 %, 20.5 %, and 10 % in the coarse, ‎medium, and fine sand, respectively. An increasing LNAPL volume with consistent ‎groundwater fluctuations has a limited impact on LNAPL behavior, although a higher LNAPL ‎spill volume can notably depress the capillary fringe. The influence of the three studied factors on ‎the migration and transformation of pollutants, however, remains uncertain, which necessitates further studies on the migration and entrapment of LNAPL in the capillary fringe ‎zone to mitigate LNAPL contamination in the saturated zone. ‎Additionally, future studies should investigate the LNAPL migration in double ‎porous soil and multiple LNAPL injections under groundwater fluctuation.‎ A deeper understanding of these factors is essential for developing predictive models and effective remediation techniques to mitigate groundwater contamination. This review serves as a foundation for future research, guiding efforts toward sustainable contamination management strategies.http://www.sciencedirect.com/science/article/pii/S1944398625001110LNAPLsMigrationEntrapmentGroundwater table fluctuationParticle sizeLNAPL volume
spellingShingle Doaa F. Almaliki
Harris Ramli
Ali Zaiter
Ishmail Sheriff
Review on migration and entrapment of light nonaqueous phase liquids ‎in the subsurface environment
Desalination and Water Treatment
LNAPLs
Migration
Entrapment
Groundwater table fluctuation
Particle size
LNAPL volume
title Review on migration and entrapment of light nonaqueous phase liquids ‎in the subsurface environment
title_full Review on migration and entrapment of light nonaqueous phase liquids ‎in the subsurface environment
title_fullStr Review on migration and entrapment of light nonaqueous phase liquids ‎in the subsurface environment
title_full_unstemmed Review on migration and entrapment of light nonaqueous phase liquids ‎in the subsurface environment
title_short Review on migration and entrapment of light nonaqueous phase liquids ‎in the subsurface environment
title_sort review on migration and entrapment of light nonaqueous phase liquids ‎in the subsurface environment
topic LNAPLs
Migration
Entrapment
Groundwater table fluctuation
Particle size
LNAPL volume
url http://www.sciencedirect.com/science/article/pii/S1944398625001110
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