3D‐Printed PDMS/Graphene Sensors with Tunable Sensitivity via Temperature‐Induced Crosslinking for Pressure Applications

Abstract The development of polydimethylsiloxane (PDMS) graphene composites with high graphene content, employed to formulate printing ink for the fabrication of tunable multilayer pressure sensors via 3D printing is presented. This study demonstrates an efficient preparation technique capable of in...

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Main Authors: Chong‐You Chen, Sepidar Sayyar, Johnson Chung, Guan‐Yu Chen, Gordon G. Wallace
Format: Article
Language:English
Published: Wiley-VCH 2025-05-01
Series:Advanced Electronic Materials
Subjects:
Online Access:https://doi.org/10.1002/aelm.202400653
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author Chong‐You Chen
Sepidar Sayyar
Johnson Chung
Guan‐Yu Chen
Gordon G. Wallace
author_facet Chong‐You Chen
Sepidar Sayyar
Johnson Chung
Guan‐Yu Chen
Gordon G. Wallace
author_sort Chong‐You Chen
collection DOAJ
description Abstract The development of polydimethylsiloxane (PDMS) graphene composites with high graphene content, employed to formulate printing ink for the fabrication of tunable multilayer pressure sensors via 3D printing is presented. This study demonstrates an efficient preparation technique capable of incorporating a high loading of edge‐functionalized expanded graphene into PDMS while minimally affecting the inherent crosslinking properties of the matrix. Graphene addition enhances electrical conductivity and rheological investigations reveal improves the printability of PDMS. Three sensor configurations differing in layer order and conductivity through piezoresistive characterization, demonstrating their excellent sensitivity and tunability with a gauge factor of ≈20 are evaluated. This performance is comparable to, and in some cases exceeds, similar structures reported in the literature. The assessment of the real‐world application potential of the PDMS/graphene pressure sensor in monitoring human movements during typical everyday situations reveals promising results. These findings suggest that the sensors developed here hold significant promise for diverse pressure‐sensing applications across various fields, including wearables, medical diagnostics, and industrial automation .
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issn 2199-160X
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publishDate 2025-05-01
publisher Wiley-VCH
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series Advanced Electronic Materials
spelling doaj-art-9367b94ae5184883b50c51de57a2d8fe2025-08-20T01:48:37ZengWiley-VCHAdvanced Electronic Materials2199-160X2025-05-01116n/an/a10.1002/aelm.2024006533D‐Printed PDMS/Graphene Sensors with Tunable Sensitivity via Temperature‐Induced Crosslinking for Pressure ApplicationsChong‐You Chen0Sepidar Sayyar1Johnson Chung2Guan‐Yu Chen3Gordon G. Wallace4Institute of Biomedical Engineering College of Electrical and Computer Engineering National Yang Ming Chiao Tung University Hsinchu 300093 TaiwanARC Centre of Excellence for Electromaterials Science Intelligent Polymer Research Institute AIIM Innovation Campus University of Wollongong Wollongong NSW 2500 AustraliaARC Centre of Excellence for Electromaterials Science Intelligent Polymer Research Institute AIIM Innovation Campus University of Wollongong Wollongong NSW 2500 AustraliaInstitute of Biomedical Engineering College of Electrical and Computer Engineering National Yang Ming Chiao Tung University Hsinchu 300093 TaiwanARC Centre of Excellence for Electromaterials Science Intelligent Polymer Research Institute AIIM Innovation Campus University of Wollongong Wollongong NSW 2500 AustraliaAbstract The development of polydimethylsiloxane (PDMS) graphene composites with high graphene content, employed to formulate printing ink for the fabrication of tunable multilayer pressure sensors via 3D printing is presented. This study demonstrates an efficient preparation technique capable of incorporating a high loading of edge‐functionalized expanded graphene into PDMS while minimally affecting the inherent crosslinking properties of the matrix. Graphene addition enhances electrical conductivity and rheological investigations reveal improves the printability of PDMS. Three sensor configurations differing in layer order and conductivity through piezoresistive characterization, demonstrating their excellent sensitivity and tunability with a gauge factor of ≈20 are evaluated. This performance is comparable to, and in some cases exceeds, similar structures reported in the literature. The assessment of the real‐world application potential of the PDMS/graphene pressure sensor in monitoring human movements during typical everyday situations reveals promising results. These findings suggest that the sensors developed here hold significant promise for diverse pressure‐sensing applications across various fields, including wearables, medical diagnostics, and industrial automation .https://doi.org/10.1002/aelm.2024006533D printingflexible sensorpolydimethylsiloxane (PDMS)/graphene compositepressure sensors
spellingShingle Chong‐You Chen
Sepidar Sayyar
Johnson Chung
Guan‐Yu Chen
Gordon G. Wallace
3D‐Printed PDMS/Graphene Sensors with Tunable Sensitivity via Temperature‐Induced Crosslinking for Pressure Applications
Advanced Electronic Materials
3D printing
flexible sensor
polydimethylsiloxane (PDMS)/graphene composite
pressure sensors
title 3D‐Printed PDMS/Graphene Sensors with Tunable Sensitivity via Temperature‐Induced Crosslinking for Pressure Applications
title_full 3D‐Printed PDMS/Graphene Sensors with Tunable Sensitivity via Temperature‐Induced Crosslinking for Pressure Applications
title_fullStr 3D‐Printed PDMS/Graphene Sensors with Tunable Sensitivity via Temperature‐Induced Crosslinking for Pressure Applications
title_full_unstemmed 3D‐Printed PDMS/Graphene Sensors with Tunable Sensitivity via Temperature‐Induced Crosslinking for Pressure Applications
title_short 3D‐Printed PDMS/Graphene Sensors with Tunable Sensitivity via Temperature‐Induced Crosslinking for Pressure Applications
title_sort 3d printed pdms graphene sensors with tunable sensitivity via temperature induced crosslinking for pressure applications
topic 3D printing
flexible sensor
polydimethylsiloxane (PDMS)/graphene composite
pressure sensors
url https://doi.org/10.1002/aelm.202400653
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AT sepidarsayyar 3dprintedpdmsgraphenesensorswithtunablesensitivityviatemperatureinducedcrosslinkingforpressureapplications
AT johnsonchung 3dprintedpdmsgraphenesensorswithtunablesensitivityviatemperatureinducedcrosslinkingforpressureapplications
AT guanyuchen 3dprintedpdmsgraphenesensorswithtunablesensitivityviatemperatureinducedcrosslinkingforpressureapplications
AT gordongwallace 3dprintedpdmsgraphenesensorswithtunablesensitivityviatemperatureinducedcrosslinkingforpressureapplications