Transition Metal Carbonitride MXenes Anchored with Pt Sub-Nanometer Clusters to Achieve High-Performance Hydrogen Evolution Reaction at All pH Range
Highlights Two-dimensional mono- and few-layered Ti3CNTx MXene nanosheets with extremely high nitrogen content were synthesized. Better performance for hydrogen evolution reaction (HER) than Pt/C catalyst in acidic, neutral and alkaline solutions. Exceptional performance of HER in both acidic and al...
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| Format: | Article |
| Language: | English |
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SpringerOpen
2025-01-01
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| Series: | Nano-Micro Letters |
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| Online Access: | https://doi.org/10.1007/s40820-025-01654-y |
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| author | Zhihao Lei Sajjad Ali CI Sathish MuhammadIbrar Ahmed Jiangtao Qu Rongkun Zheng Shibo Xi Xiaojiang Yu M. B. H. Breese Chao Liu Jizhen Zhang Shuai Qi Xinwei Guan Vibin Perumalsamy Mohammed Fawaz Jae-Hun Yang Mohamed Bououdina Kazunari Domen Ajayan Vinu Liang Qiao Jiabao Yi |
| author_facet | Zhihao Lei Sajjad Ali CI Sathish MuhammadIbrar Ahmed Jiangtao Qu Rongkun Zheng Shibo Xi Xiaojiang Yu M. B. H. Breese Chao Liu Jizhen Zhang Shuai Qi Xinwei Guan Vibin Perumalsamy Mohammed Fawaz Jae-Hun Yang Mohamed Bououdina Kazunari Domen Ajayan Vinu Liang Qiao Jiabao Yi |
| author_sort | Zhihao Lei |
| collection | DOAJ |
| description | Highlights Two-dimensional mono- and few-layered Ti3CNTx MXene nanosheets with extremely high nitrogen content were synthesized. Better performance for hydrogen evolution reaction (HER) than Pt/C catalyst in acidic, neutral and alkaline solutions. Exceptional performance of HER in both acidic and alkaline solutions. A large current density (> 500 mA cm−2) has been achieved for HER. |
| format | Article |
| id | doaj-art-92fad12a229f4eb69f3bf92e1e94a527 |
| institution | Kabale University |
| issn | 2311-6706 2150-5551 |
| language | English |
| publishDate | 2025-01-01 |
| publisher | SpringerOpen |
| record_format | Article |
| series | Nano-Micro Letters |
| spelling | doaj-art-92fad12a229f4eb69f3bf92e1e94a5272025-02-02T12:37:37ZengSpringerOpenNano-Micro Letters2311-67062150-55512025-01-0117111510.1007/s40820-025-01654-yTransition Metal Carbonitride MXenes Anchored with Pt Sub-Nanometer Clusters to Achieve High-Performance Hydrogen Evolution Reaction at All pH RangeZhihao Lei0Sajjad Ali1CI Sathish2MuhammadIbrar Ahmed3Jiangtao Qu4Rongkun Zheng5Shibo Xi6Xiaojiang Yu7M. B. H. Breese8Chao Liu9Jizhen Zhang10Shuai Qi11Xinwei Guan12Vibin Perumalsamy13Mohammed Fawaz14Jae-Hun Yang15Mohamed Bououdina16Kazunari Domen17Ajayan Vinu18Liang Qiao19Jiabao Yi20Global Innovative Center of Advanced Nanomaterials, College of Engineering, Science and Environment, University of NewcastleEnergy, Water, and Environment Lab, College of Humanities and Sciences, Prince Sultan UniversityGlobal Innovative Center of Advanced Nanomaterials, College of Engineering, Science and Environment, University of NewcastleGlobal Innovative Center of Advanced Nanomaterials, College of Engineering, Science and Environment, University of NewcastleSchool of Physics, University of SydneySchool of Physics, University of SydneyInstitute of Chemical and Engineering Sciences, A*STARSingapore Synchrotron Light Source, National University of SingaporeSingapore Synchrotron Light Source, National University of SingaporeInstitute for Frontier Materials, Deakin UniversityGuangdong Provincial Key Laboratory of Natural Rubber Processing, Agricultural Products Processing Research Institute, Chinese Academy of Tropical Agricultural SciencesCollege of Chemistry Environmental Engineering, Shenzhen UniversityGlobal Innovative Center of Advanced Nanomaterials, College of Engineering, Science and Environment, University of NewcastleGlobal Innovative Center of Advanced Nanomaterials, College of Engineering, Science and Environment, University of NewcastleGlobal Innovative Center of Advanced Nanomaterials, College of Engineering, Science and Environment, University of NewcastleGlobal Innovative Center of Advanced Nanomaterials, College of Engineering, Science and Environment, University of NewcastleGlobal Innovative Center of Advanced Nanomaterials, College of Engineering, Science and Environment, University of NewcastleResearch Initiative for Supra-Materials Interdisciplinary Cluster for Cutting Edge Research, Shinshu UniversityGlobal Innovative Center of Advanced Nanomaterials, College of Engineering, Science and Environment, University of NewcastleSchool of Physics, University of Electronic Science and Technology of ChinaDepartment of Chemical Engineering and Interdisciplinary Research Center for Hydrogen Technologies and Carbon Management (IRC-HTCM), King Fahd University of Petroleum and MineralsHighlights Two-dimensional mono- and few-layered Ti3CNTx MXene nanosheets with extremely high nitrogen content were synthesized. Better performance for hydrogen evolution reaction (HER) than Pt/C catalyst in acidic, neutral and alkaline solutions. Exceptional performance of HER in both acidic and alkaline solutions. A large current density (> 500 mA cm−2) has been achieved for HER.https://doi.org/10.1007/s40820-025-01654-yMXeneHydrogen evolution reactionSingle atomTwo-dimensional nanosheetsDensity functional theory |
| spellingShingle | Zhihao Lei Sajjad Ali CI Sathish MuhammadIbrar Ahmed Jiangtao Qu Rongkun Zheng Shibo Xi Xiaojiang Yu M. B. H. Breese Chao Liu Jizhen Zhang Shuai Qi Xinwei Guan Vibin Perumalsamy Mohammed Fawaz Jae-Hun Yang Mohamed Bououdina Kazunari Domen Ajayan Vinu Liang Qiao Jiabao Yi Transition Metal Carbonitride MXenes Anchored with Pt Sub-Nanometer Clusters to Achieve High-Performance Hydrogen Evolution Reaction at All pH Range Nano-Micro Letters MXene Hydrogen evolution reaction Single atom Two-dimensional nanosheets Density functional theory |
| title | Transition Metal Carbonitride MXenes Anchored with Pt Sub-Nanometer Clusters to Achieve High-Performance Hydrogen Evolution Reaction at All pH Range |
| title_full | Transition Metal Carbonitride MXenes Anchored with Pt Sub-Nanometer Clusters to Achieve High-Performance Hydrogen Evolution Reaction at All pH Range |
| title_fullStr | Transition Metal Carbonitride MXenes Anchored with Pt Sub-Nanometer Clusters to Achieve High-Performance Hydrogen Evolution Reaction at All pH Range |
| title_full_unstemmed | Transition Metal Carbonitride MXenes Anchored with Pt Sub-Nanometer Clusters to Achieve High-Performance Hydrogen Evolution Reaction at All pH Range |
| title_short | Transition Metal Carbonitride MXenes Anchored with Pt Sub-Nanometer Clusters to Achieve High-Performance Hydrogen Evolution Reaction at All pH Range |
| title_sort | transition metal carbonitride mxenes anchored with pt sub nanometer clusters to achieve high performance hydrogen evolution reaction at all ph range |
| topic | MXene Hydrogen evolution reaction Single atom Two-dimensional nanosheets Density functional theory |
| url | https://doi.org/10.1007/s40820-025-01654-y |
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