Development and optimization of a bio-based adhesive from euphorbia trigon latex reinforced with alumina for sustainable wood bonding applications

The environmental and health concerns associated with petroleum-based synthetic adhesives, particularly their non-biodegradability and emission of volatile organic compounds (VOCs), have been widely recognized. As a result, increased attention has been given to the development of sustainable, bio-ba...

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Main Authors: Abdurahman Aman, Kumlachew Yeneneh, Ali Shemsedin, Belachew Zegale, Elias Wakshume
Format: Article
Language:English
Published: Elsevier 2025-09-01
Series:Results in Engineering
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Online Access:http://www.sciencedirect.com/science/article/pii/S259012302502537X
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author Abdurahman Aman
Kumlachew Yeneneh
Ali Shemsedin
Belachew Zegale
Elias Wakshume
author_facet Abdurahman Aman
Kumlachew Yeneneh
Ali Shemsedin
Belachew Zegale
Elias Wakshume
author_sort Abdurahman Aman
collection DOAJ
description The environmental and health concerns associated with petroleum-based synthetic adhesives, particularly their non-biodegradability and emission of volatile organic compounds (VOCs), have been widely recognized. As a result, increased attention has been given to the development of sustainable, bio-based alternatives. However, natural adhesives have often been limited by inadequate mechanical strength, low thermal stability, and poor durability. In this study, a bio-adhesive was formulated from Euphorbia trigon latex, an underutilized, non-edible, and drought-tolerant plant, by reinforcing it with alumina (Al₂O₃) to enhance its performance characteristics. Improvements in structural integrity and thermal resistance were targeted while maintaining environmental sustainability. A Central Composite Design (CCD) under Response Surface Methodology (RSM) was employed to optimize the formulation parameters. The effects of latex concentration, alumina loading, and mixing time were systematically analyzed. An optimized formulation comprising 40 % latex, 30 % alumina, and a mixing time of 30 min was obtained. Under these conditions, a lap shear strength of 7.7 MPa, a viscosity of 3585 mPa·s, and a thermal decomposition temperature exceeding 400 °C were achieved. These results indicate that the developed bio-adhesive can serve as a viable and eco-friendly alternative to synthetic adhesives for wood bonding, particularly in regions where cost-effective and locally sourced materials are desired.
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spelling doaj-art-922d824203ed4d8ebd98bcba125abec62025-08-20T03:08:35ZengElsevierResults in Engineering2590-12302025-09-012710646810.1016/j.rineng.2025.106468Development and optimization of a bio-based adhesive from euphorbia trigon latex reinforced with alumina for sustainable wood bonding applicationsAbdurahman Aman0Kumlachew Yeneneh1Ali Shemsedin2Belachew Zegale3Elias Wakshume4Department of Chemical Engineering, College of Engineering, Ethiopian Defence University, Bishoftu P.O. Box 1041, EthiopiaDepartment of Motor Engineering, College of Engineering, Ethiopian Defence University, Bishoftu P.O. Box 1041, Ethiopia; Correspondence author.Biotechnology and Bioprocess Center of Excellence, Addis Ababa Science and Technology University, Addis Ababa, P.O. Box 16417, EthiopiaBiotechnology and Bioprocess Center of Excellence, Addis Ababa Science and Technology University, Addis Ababa, P.O. Box 16417, EthiopiaDepartment of Production Engineering, College of Engineering, Ethiopian Defence University, Bishoftu P.O. Box 1041, EthiopiaThe environmental and health concerns associated with petroleum-based synthetic adhesives, particularly their non-biodegradability and emission of volatile organic compounds (VOCs), have been widely recognized. As a result, increased attention has been given to the development of sustainable, bio-based alternatives. However, natural adhesives have often been limited by inadequate mechanical strength, low thermal stability, and poor durability. In this study, a bio-adhesive was formulated from Euphorbia trigon latex, an underutilized, non-edible, and drought-tolerant plant, by reinforcing it with alumina (Al₂O₃) to enhance its performance characteristics. Improvements in structural integrity and thermal resistance were targeted while maintaining environmental sustainability. A Central Composite Design (CCD) under Response Surface Methodology (RSM) was employed to optimize the formulation parameters. The effects of latex concentration, alumina loading, and mixing time were systematically analyzed. An optimized formulation comprising 40 % latex, 30 % alumina, and a mixing time of 30 min was obtained. Under these conditions, a lap shear strength of 7.7 MPa, a viscosity of 3585 mPa·s, and a thermal decomposition temperature exceeding 400 °C were achieved. These results indicate that the developed bio-adhesive can serve as a viable and eco-friendly alternative to synthetic adhesives for wood bonding, particularly in regions where cost-effective and locally sourced materials are desired.http://www.sciencedirect.com/science/article/pii/S259012302502537XBio-adhesiveEuphorbia trigon latexAlumina reinforcementSustainable materialsLap shear strengthThermal stability
spellingShingle Abdurahman Aman
Kumlachew Yeneneh
Ali Shemsedin
Belachew Zegale
Elias Wakshume
Development and optimization of a bio-based adhesive from euphorbia trigon latex reinforced with alumina for sustainable wood bonding applications
Results in Engineering
Bio-adhesive
Euphorbia trigon latex
Alumina reinforcement
Sustainable materials
Lap shear strength
Thermal stability
title Development and optimization of a bio-based adhesive from euphorbia trigon latex reinforced with alumina for sustainable wood bonding applications
title_full Development and optimization of a bio-based adhesive from euphorbia trigon latex reinforced with alumina for sustainable wood bonding applications
title_fullStr Development and optimization of a bio-based adhesive from euphorbia trigon latex reinforced with alumina for sustainable wood bonding applications
title_full_unstemmed Development and optimization of a bio-based adhesive from euphorbia trigon latex reinforced with alumina for sustainable wood bonding applications
title_short Development and optimization of a bio-based adhesive from euphorbia trigon latex reinforced with alumina for sustainable wood bonding applications
title_sort development and optimization of a bio based adhesive from euphorbia trigon latex reinforced with alumina for sustainable wood bonding applications
topic Bio-adhesive
Euphorbia trigon latex
Alumina reinforcement
Sustainable materials
Lap shear strength
Thermal stability
url http://www.sciencedirect.com/science/article/pii/S259012302502537X
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