Self-Regulated Bilateral Anchoring Enables Efficient Charge Transport Pathways for High-Performance Rigid and Flexible Perovskite Solar Cells

Highlights Robust interface molecular bridge was constructed by employing self-transforming squaric acid (SA) to reduce residual stress and passivate defects at the buried interface. Attributing to the efficient charge transport pathways, the SA-modified perovskite solar cells demonstrate high photo...

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Main Authors: Haiying Zheng, Guozhen Liu, Xinhe Dong, Feifan Chen, Chao Wang, Hongbo Yu, Zhihua Zhang, Xu Pan
Format: Article
Language:English
Published: SpringerOpen 2025-07-01
Series:Nano-Micro Letters
Subjects:
Online Access:https://doi.org/10.1007/s40820-025-01846-6
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author Haiying Zheng
Guozhen Liu
Xinhe Dong
Feifan Chen
Chao Wang
Hongbo Yu
Zhihua Zhang
Xu Pan
author_facet Haiying Zheng
Guozhen Liu
Xinhe Dong
Feifan Chen
Chao Wang
Hongbo Yu
Zhihua Zhang
Xu Pan
author_sort Haiying Zheng
collection DOAJ
description Highlights Robust interface molecular bridge was constructed by employing self-transforming squaric acid (SA) to reduce residual stress and passivate defects at the buried interface. Attributing to the efficient charge transport pathways, the SA-modified perovskite solar cells demonstrate high photovoltaic performance with power conversion efficiency up to 25.50% (rigid) and 24.92% (flexible). The SA-modified devices demonstrate excellent stability under various environmental stress conditions, including humidity, thermal aging, light irradiation, and bending.
format Article
id doaj-art-9133f333dc88448b8ff98e807dc14e97
institution Kabale University
issn 2311-6706
2150-5551
language English
publishDate 2025-07-01
publisher SpringerOpen
record_format Article
series Nano-Micro Letters
spelling doaj-art-9133f333dc88448b8ff98e807dc14e972025-08-20T04:02:56ZengSpringerOpenNano-Micro Letters2311-67062150-55512025-07-0117111510.1007/s40820-025-01846-6Self-Regulated Bilateral Anchoring Enables Efficient Charge Transport Pathways for High-Performance Rigid and Flexible Perovskite Solar CellsHaiying Zheng0Guozhen Liu1Xinhe Dong2Feifan Chen3Chao Wang4Hongbo Yu5Zhihua Zhang6Xu Pan7School of Materials Science and Engineering, Dalian Jiaotong UniversityState Key Laboratory of Fine Chemicals, School of Chemistry, Dalian University of TechnologyInstitutes of Physical Science and Information Technology, Anhui UniversityInstitutes of Physical Science and Information Technology, Anhui UniversityInstitutes of Physical Science and Information Technology, Anhui UniversitySchool of Materials Science and Engineering, Dalian Jiaotong UniversitySchool of Materials Science and Engineering, Dalian Jiaotong UniversityKey Laboratory of Photovoltaic and Energy Conservation Materials, Institute of Solid State Physics, Hefei Institutes of Physical Science, Chinese Academy of SciencesHighlights Robust interface molecular bridge was constructed by employing self-transforming squaric acid (SA) to reduce residual stress and passivate defects at the buried interface. Attributing to the efficient charge transport pathways, the SA-modified perovskite solar cells demonstrate high photovoltaic performance with power conversion efficiency up to 25.50% (rigid) and 24.92% (flexible). The SA-modified devices demonstrate excellent stability under various environmental stress conditions, including humidity, thermal aging, light irradiation, and bending.https://doi.org/10.1007/s40820-025-01846-6Perovskite solar cellsBuried interfaceBilateral bondingDefects passivationElectron transport pathway
spellingShingle Haiying Zheng
Guozhen Liu
Xinhe Dong
Feifan Chen
Chao Wang
Hongbo Yu
Zhihua Zhang
Xu Pan
Self-Regulated Bilateral Anchoring Enables Efficient Charge Transport Pathways for High-Performance Rigid and Flexible Perovskite Solar Cells
Nano-Micro Letters
Perovskite solar cells
Buried interface
Bilateral bonding
Defects passivation
Electron transport pathway
title Self-Regulated Bilateral Anchoring Enables Efficient Charge Transport Pathways for High-Performance Rigid and Flexible Perovskite Solar Cells
title_full Self-Regulated Bilateral Anchoring Enables Efficient Charge Transport Pathways for High-Performance Rigid and Flexible Perovskite Solar Cells
title_fullStr Self-Regulated Bilateral Anchoring Enables Efficient Charge Transport Pathways for High-Performance Rigid and Flexible Perovskite Solar Cells
title_full_unstemmed Self-Regulated Bilateral Anchoring Enables Efficient Charge Transport Pathways for High-Performance Rigid and Flexible Perovskite Solar Cells
title_short Self-Regulated Bilateral Anchoring Enables Efficient Charge Transport Pathways for High-Performance Rigid and Flexible Perovskite Solar Cells
title_sort self regulated bilateral anchoring enables efficient charge transport pathways for high performance rigid and flexible perovskite solar cells
topic Perovskite solar cells
Buried interface
Bilateral bonding
Defects passivation
Electron transport pathway
url https://doi.org/10.1007/s40820-025-01846-6
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