Formation of bovine serum albumin–galangin nanoparticles and their potential to inhibit reactive oxygen species–induced inflammation: Ethanol desolvation versus pH-shifting method

ABSTRACT: The pH-shifting method, as an ecofriendly approach, is a promising alternative to the desolvation method, yet systematic comparison of their properties is still lacking. In this study, BSA-galangin nanoparticles (BSA-GA NP) were designed for alleviating reactive oxygen species (ROS)–mediat...

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Main Authors: Weigang Zhong, Lei Xu, Qi Wang, Xue Shen
Format: Article
Language:English
Published: Elsevier 2025-01-01
Series:Journal of Dairy Science
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Online Access:http://www.sciencedirect.com/science/article/pii/S0022030224012098
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author Weigang Zhong
Lei Xu
Qi Wang
Xue Shen
author_facet Weigang Zhong
Lei Xu
Qi Wang
Xue Shen
author_sort Weigang Zhong
collection DOAJ
description ABSTRACT: The pH-shifting method, as an ecofriendly approach, is a promising alternative to the desolvation method, yet systematic comparison of their properties is still lacking. In this study, BSA-galangin nanoparticles (BSA-GA NP) were designed for alleviating reactive oxygen species (ROS)–mediated macrophage inflammation by the 2 separate methods. Compared with the desolvation method, BSA exhibited a higher loading capacity for GA under the pH-shifting method, which was attributed to the exposure of the binding site leading to enhanced affinity for GA and a more compact particle structure. Further analyses evidenced that the electron arrangement and crystal structure of GA changed with different methods. The content of the random coil of BSA was elevated after the pH-shifting method. Additionally, the smaller size rendered the pH-shifting treated BSA-GA NP easier to be taken up by macrophages, and the enhanced specific surface area conferred excellent ROS scavenging and anti-inflammatory performances. This study may provide new insights into the choice of loading methods.
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issn 0022-0302
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publishDate 2025-01-01
publisher Elsevier
record_format Article
series Journal of Dairy Science
spelling doaj-art-90ea87d6a9fe4f269d7e05ee9b96e0012025-08-20T01:57:20ZengElsevierJournal of Dairy Science0022-03022025-01-01108128229710.3168/jds.2024-25495Formation of bovine serum albumin–galangin nanoparticles and their potential to inhibit reactive oxygen species–induced inflammation: Ethanol desolvation versus pH-shifting methodWeigang Zhong0Lei Xu1Qi Wang2Xue Shen3Department of Food Science, College of Food Science and Engineering, Jilin University, Changchun, Jilin, 130062, ChinaState Key Laboratory for Zoonotic Diseases, Key Laboratory for Zoonosis Research, Ministry of Education, College of Veterinary Medicine, Jilin University, Changchun, Jilin, 130012, ChinaDepartment of Food Science, College of Food Science and Engineering, Jilin University, Changchun, Jilin, 130062, ChinaDepartment of Food Science, College of Food Science and Engineering, Jilin University, Changchun, Jilin, 130062, China; Corresponding authorABSTRACT: The pH-shifting method, as an ecofriendly approach, is a promising alternative to the desolvation method, yet systematic comparison of their properties is still lacking. In this study, BSA-galangin nanoparticles (BSA-GA NP) were designed for alleviating reactive oxygen species (ROS)–mediated macrophage inflammation by the 2 separate methods. Compared with the desolvation method, BSA exhibited a higher loading capacity for GA under the pH-shifting method, which was attributed to the exposure of the binding site leading to enhanced affinity for GA and a more compact particle structure. Further analyses evidenced that the electron arrangement and crystal structure of GA changed with different methods. The content of the random coil of BSA was elevated after the pH-shifting method. Additionally, the smaller size rendered the pH-shifting treated BSA-GA NP easier to be taken up by macrophages, and the enhanced specific surface area conferred excellent ROS scavenging and anti-inflammatory performances. This study may provide new insights into the choice of loading methods.http://www.sciencedirect.com/science/article/pii/S0022030224012098bovine serum albumingalanginethanol desolvationpH-shiftingnanoparticles
spellingShingle Weigang Zhong
Lei Xu
Qi Wang
Xue Shen
Formation of bovine serum albumin–galangin nanoparticles and their potential to inhibit reactive oxygen species–induced inflammation: Ethanol desolvation versus pH-shifting method
Journal of Dairy Science
bovine serum albumin
galangin
ethanol desolvation
pH-shifting
nanoparticles
title Formation of bovine serum albumin–galangin nanoparticles and their potential to inhibit reactive oxygen species–induced inflammation: Ethanol desolvation versus pH-shifting method
title_full Formation of bovine serum albumin–galangin nanoparticles and their potential to inhibit reactive oxygen species–induced inflammation: Ethanol desolvation versus pH-shifting method
title_fullStr Formation of bovine serum albumin–galangin nanoparticles and their potential to inhibit reactive oxygen species–induced inflammation: Ethanol desolvation versus pH-shifting method
title_full_unstemmed Formation of bovine serum albumin–galangin nanoparticles and their potential to inhibit reactive oxygen species–induced inflammation: Ethanol desolvation versus pH-shifting method
title_short Formation of bovine serum albumin–galangin nanoparticles and their potential to inhibit reactive oxygen species–induced inflammation: Ethanol desolvation versus pH-shifting method
title_sort formation of bovine serum albumin galangin nanoparticles and their potential to inhibit reactive oxygen species induced inflammation ethanol desolvation versus ph shifting method
topic bovine serum albumin
galangin
ethanol desolvation
pH-shifting
nanoparticles
url http://www.sciencedirect.com/science/article/pii/S0022030224012098
work_keys_str_mv AT weigangzhong formationofbovineserumalbumingalanginnanoparticlesandtheirpotentialtoinhibitreactiveoxygenspeciesinducedinflammationethanoldesolvationversusphshiftingmethod
AT leixu formationofbovineserumalbumingalanginnanoparticlesandtheirpotentialtoinhibitreactiveoxygenspeciesinducedinflammationethanoldesolvationversusphshiftingmethod
AT qiwang formationofbovineserumalbumingalanginnanoparticlesandtheirpotentialtoinhibitreactiveoxygenspeciesinducedinflammationethanoldesolvationversusphshiftingmethod
AT xueshen formationofbovineserumalbumingalanginnanoparticlesandtheirpotentialtoinhibitreactiveoxygenspeciesinducedinflammationethanoldesolvationversusphshiftingmethod