Exploring Community Succession, Assembly Patterns, and Metabolic Functions of Ester-Producing-Related Microbiota during the Production of <i>Nongxiangxing baijiu</i>

Esters are vital flavor compounds in Chinese <i>Nongxiangxing baijiu</i> and greatly affect the quality of <i>baijiu</i>. Microbial communities inhabiting fermented grains (FGs) have a marked impact on esters. However, the specific microorganisms and their assembly patterns r...

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Main Authors: Xiawei Yi, Huan Xia, Ping Huang, Shiyuan Ma, Chongde Wu
Format: Article
Language:English
Published: MDPI AG 2024-10-01
Series:Foods
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Online Access:https://www.mdpi.com/2304-8158/13/19/3169
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author Xiawei Yi
Huan Xia
Ping Huang
Shiyuan Ma
Chongde Wu
author_facet Xiawei Yi
Huan Xia
Ping Huang
Shiyuan Ma
Chongde Wu
author_sort Xiawei Yi
collection DOAJ
description Esters are vital flavor compounds in Chinese <i>Nongxiangxing baijiu</i> and greatly affect the quality of <i>baijiu</i>. Microbial communities inhabiting fermented grains (FGs) have a marked impact on esters. However, the specific microorganisms and their assembly patterns remain unclear. This study utilized high-throughput sequencing and a culture-based method to reveal ester-producing microorganisms. A total of 33 esters were detected, including 19 ethyl esters, 9 linear chain esters, and 2 branched chain esters. A correlation analysis indicated that the bacterial genus <i>Lactobacillus</i> (relative abundance in average: 69.05%) and fungal genera <i>Pichia</i> (2.40%), <i>Aspergillus</i> (11.84%), <i>Wickerhamomyces</i> (0.60%), <i>Thermomyces</i> (3.57%), <i>Saccharomycopsis</i> (7.87%), <i>Issatchenkia</i> (0.96%), and <i>Thermoascus</i> (10.83%) were dominant and associated with esters production and their precursors. The numbers of esters positively correlated with them were 1, 17, 3, 2, 1, 1, 1, and 1, respectively. The modified stochasticity ratio (MST) index and Sloan neutral model revealed that bacteria were predominantly governed by deterministic processes while fungal assemblies were more stochastic. <i>Saturnispora silvae</i> and <i>Zygosaccharomyces bailii</i> were isolated and identified with ester synthesis potential. PICRUSt2 analysis showed that fungi in FG had a high potential for synthesizing ethanol, while 14 enzymes related to esters synthesis were all produced by bacteria, especially enzymes catalyzing the synthesis of acyl-CoA. In addition, ester synthesis was mainly catalyzed by carboxylesterase, acylglycerol lipase and triacylglycerol lipase. These findings may provide insights into ester production mechanism and potential strategies to improve the quality of <i>Nongxiangxing baijiu</i>.
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spelling doaj-art-8e452f2db82e4e45bf474c0b946175b62025-08-20T02:16:50ZengMDPI AGFoods2304-81582024-10-011319316910.3390/foods13193169Exploring Community Succession, Assembly Patterns, and Metabolic Functions of Ester-Producing-Related Microbiota during the Production of <i>Nongxiangxing baijiu</i>Xiawei Yi0Huan Xia1Ping Huang2Shiyuan Ma3Chongde Wu4College of Biomass Science and Engineering, Sichuan University, Chengdu 610065, ChinaCollege of Biomass Science and Engineering, Sichuan University, Chengdu 610065, ChinaCollege of Biomass Science and Engineering, Sichuan University, Chengdu 610065, ChinaCollege of Biomass Science and Engineering, Sichuan University, Chengdu 610065, ChinaCollege of Biomass Science and Engineering, Sichuan University, Chengdu 610065, ChinaEsters are vital flavor compounds in Chinese <i>Nongxiangxing baijiu</i> and greatly affect the quality of <i>baijiu</i>. Microbial communities inhabiting fermented grains (FGs) have a marked impact on esters. However, the specific microorganisms and their assembly patterns remain unclear. This study utilized high-throughput sequencing and a culture-based method to reveal ester-producing microorganisms. A total of 33 esters were detected, including 19 ethyl esters, 9 linear chain esters, and 2 branched chain esters. A correlation analysis indicated that the bacterial genus <i>Lactobacillus</i> (relative abundance in average: 69.05%) and fungal genera <i>Pichia</i> (2.40%), <i>Aspergillus</i> (11.84%), <i>Wickerhamomyces</i> (0.60%), <i>Thermomyces</i> (3.57%), <i>Saccharomycopsis</i> (7.87%), <i>Issatchenkia</i> (0.96%), and <i>Thermoascus</i> (10.83%) were dominant and associated with esters production and their precursors. The numbers of esters positively correlated with them were 1, 17, 3, 2, 1, 1, 1, and 1, respectively. The modified stochasticity ratio (MST) index and Sloan neutral model revealed that bacteria were predominantly governed by deterministic processes while fungal assemblies were more stochastic. <i>Saturnispora silvae</i> and <i>Zygosaccharomyces bailii</i> were isolated and identified with ester synthesis potential. PICRUSt2 analysis showed that fungi in FG had a high potential for synthesizing ethanol, while 14 enzymes related to esters synthesis were all produced by bacteria, especially enzymes catalyzing the synthesis of acyl-CoA. In addition, ester synthesis was mainly catalyzed by carboxylesterase, acylglycerol lipase and triacylglycerol lipase. These findings may provide insights into ester production mechanism and potential strategies to improve the quality of <i>Nongxiangxing baijiu</i>.https://www.mdpi.com/2304-8158/13/19/3169fermentation grainsester formationmicrobial communitymicrobiota assembly
spellingShingle Xiawei Yi
Huan Xia
Ping Huang
Shiyuan Ma
Chongde Wu
Exploring Community Succession, Assembly Patterns, and Metabolic Functions of Ester-Producing-Related Microbiota during the Production of <i>Nongxiangxing baijiu</i>
Foods
fermentation grains
ester formation
microbial community
microbiota assembly
title Exploring Community Succession, Assembly Patterns, and Metabolic Functions of Ester-Producing-Related Microbiota during the Production of <i>Nongxiangxing baijiu</i>
title_full Exploring Community Succession, Assembly Patterns, and Metabolic Functions of Ester-Producing-Related Microbiota during the Production of <i>Nongxiangxing baijiu</i>
title_fullStr Exploring Community Succession, Assembly Patterns, and Metabolic Functions of Ester-Producing-Related Microbiota during the Production of <i>Nongxiangxing baijiu</i>
title_full_unstemmed Exploring Community Succession, Assembly Patterns, and Metabolic Functions of Ester-Producing-Related Microbiota during the Production of <i>Nongxiangxing baijiu</i>
title_short Exploring Community Succession, Assembly Patterns, and Metabolic Functions of Ester-Producing-Related Microbiota during the Production of <i>Nongxiangxing baijiu</i>
title_sort exploring community succession assembly patterns and metabolic functions of ester producing related microbiota during the production of i nongxiangxing baijiu i
topic fermentation grains
ester formation
microbial community
microbiota assembly
url https://www.mdpi.com/2304-8158/13/19/3169
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AT shiyuanma exploringcommunitysuccessionassemblypatternsandmetabolicfunctionsofesterproducingrelatedmicrobiotaduringtheproductionofinongxiangxingbaijiui
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